Environ. Sci. Technol., 41 (7), 2131 -2137, 2007. 10.1021/es061791t S0013-936X(06)01791-3
Web Release Date: February 14, 2007

Copyright © 2007 American Chemical Society

Atmospheric Methane: Trends and Cycles of Sources and Sinks

M. Aslam Khan Khalil,* Christopher L. Butenhoff, and Reinhold A. Rasmussen

Department of Physics, Portland State University, P.O. Box 751, Portland, Oregon 97207, and Department of Environmental Science, Oregon Graduate Institute, Beaverton, Oregon 97006

Received for review July 27, 2006

Revised manuscript received January 10, 2007

Accepted January 13, 2007

Abstract:

For more than 20 years the global emissions and the lifetime of methane have probably been constant, so the buildup of methane in the atmosphere has been slowing down for as long. During this time, there have been periodic events occurring every seven to eight years, when global methane concentrations increased by some 10 ppb and later fell back, in some cases due to temporary increases of emissions from the northern tropics that spread to the global scale. These conclusions are derived from the accumulated global observations that now span 23 years and define the role of human activities in the recent cycle of atmospheric methane.


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