A Novel Fountain Photocatalytic Reactor for Water Treatment and Purification:  Modeling and Design

Gianluca Li Puma* and Po Lock Yue
School of Chemical, Environmental and Mining Engineering, The University of Nottingham, University Park, Nottingham NG7 2RD, United Kingdom, and Department of Chemical Engineering, The Hong Kong University of Science & Technology, Clear Water Bay, Kowloon, Hong Kong SAR
Ind. Eng. Chem. Res., 2001, 40 (23), pp 5162–5169
DOI: 10.1021/ie0010316
Publication Date (Web): June 23, 2001
Copyright © 2001 American Chemical Society
*

 Corresponding author. E-mail:  gianluca.li.puma@ nottingham.ac.uk. Fax:  +44 (0) 115 9514115.

,

 The University of Nottingham.

,

 The Hong Kong University of Science & Technology.

Abstract

A novel, thin-film, slurry “fountain” photocatalytic reactor for water treatment and purification is presented. The novelty of the reactor centers on the design of a special nozzle through which water is pumped to create a thin film. The film emerges from the nozzle in the shape of a smooth and radially expanding water fountain. A radiation source (solar or UV lamps) is situated above the fountain. Two dimensionless mathematical models for the photoreactora flat fountain model and a parabolic fountain modeland simulation results under a number of different conditions including the effects of nozzle setting (radius, aperture, and angle), flow rate, and light scattering are presented. The model simulations suggest that optimal photoreactor design is given by fountains with large surface areas. Photocatalysts with scattering albedos smaller than 0.3 result in optimal photoreactor performance. The models presented may be used as a tool for the design, scale-up, and optimization of these types of reactors.

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History

  • Published In Issue November 14, 2001
  • Received for review December 4, 2000
    Revised manuscript received March 23, 2001
    Accepted April 23, 2001

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