An efficient photochemical approach to the trans-bicyclo[5.1.0]octene ring system

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  • Asymmetric Synthesis of Functionalized Cyclopentanones via a Multicatalytic Secondary Amine/N-Heterocyclic Carbene Catalyzed Cascade Sequence

    Stephen P. Lathrop and Tomislav Rovis
    Journal of the American Chemical Society 2009 131 (38), pp 13628–13630

    Abstract: A one-pot, asymmetric multicatalytic formal [3+2] reaction between 1,3-dicarbonyls and α,β-unsaturated aldehydes is described. The multicatalytic process involves a secondary amine catalyzed Michael addition followed by a N-heterocyclic carbene catalyzed ...

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