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Multilayered Carbon Nanotube/Polymer Composite Based Thermoelectric Fabrics

Center for Nanotechnology, Wake Forest University, Winston Salem, North Carolina 27105, United States
MacDiarmid Institute for Advanced Materials and Nanotechnology, SCPS, Victoria University of Wellington, Wellington 6140, New Zealand
§ School of Electrical Engineering, WCU Flexible Nanosystems, Korea University, Seoul, Korea
NanoTechLabs, Yadkinville, North Carolina 27055, United States
Nano Lett., 2012, 12 (3), pp 1307–1310
DOI: 10.1021/nl203806q
Publication Date (Web): February 8, 2012
Copyright © 2012 American Chemical Society

Abstract

Abstract Image

Thermoelectrics are materials capable of the solid-state conversion between thermal and electrical energy. Carbon nanotube/polymer composite thin films are known to exhibit thermoelectric effects, however, have a low figure of merit (ZT) of 0.02. In this work, we demonstrate individual composite films of multiwalled carbon nanotubes (MWNT)/polyvinylidene fluoride (PVDF) that are layered into multiple element modules that resemble a felt fabric. The thermoelectric voltage generated by these fabrics is the sum of contributions from each layer, resulting in increased power output. Since these fabrics have the potential to be cheaper, lighter, and more easily processed than the commonly used thermoelectric bismuth telluride, the overall performance of the fabric shows promise as a realistic alternative in a number of applications such as portable lightweight electronics.

Effect of temperature gradient profile on VTEP and power generated. This material is available free of charge via the Internet at http://pubs.acs.org.

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History

  • Published In Issue March 14, 2012
  • Article ASAPFebruary 16, 2012
  • Just Accepted ManuscriptFebruary 08, 2012
  • Received: October 28, 2011
    Revised: January 24, 2012

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