Table of Contents

Journal Cover
December 8, 2004
Volume 126, Issue 48
Pages 15636-15924
For Selected Content:

COMMUNICATIONS

Dendrimers with Both Polar and Apolar Nanocontainer Characteristics

Dharma Rao Vutukuri, Subhadeep Basu, and S. Thayumanavan
pp 15636–15637
Publication Date (Web): November 10, 2004 (Communication)
DOI: 10.1021/ja0449628

Near-Infrared Fluorescence Microscopy of Single-Walled Carbon Nanotubes in Phagocytic Cells

Paul Cherukuri, Sergei M. Bachilo, Silvio H. Litovsky, and R. Bruce Weisman
pp 15638–15639
Publication Date (Web): November 11, 2004 (Communication)
DOI: 10.1021/ja0466311

Microarray Platform for Profiling Enzyme Activities in Complex Proteomes

Stephan A. Sieber, Tony S. Mondala, Steven R. Head, and Benjamin F. Cravatt
pp 15640–15641
Publication Date (Web): November 10, 2004 (Communication)
DOI: 10.1021/ja044286+

A Strong Positive Dendritic Effect in a Peptide Dendrimer-Catalyzed Ester Hydrolysis Reaction

Estelle Delort, Tamis Darbre, and Jean-Louis Reymond
pp 15642–15643
Publication Date (Web): November 11, 2004 (Communication)
DOI: 10.1021/ja044652p

Fluorinated Imidazoles as Proton Carriers for Water-Free Fuel Cell Membranes

Wei-Qiao Deng, Valeria Molinero, and William A. Goddard III
pp 15644–15645
Publication Date (Web): November 11, 2004 (Communication)
DOI: 10.1021/ja046999y

DNA−Nanotube Artificial Ion Channels

C. Chad Harrell, Punit Kohli, Zuzanna Siwy, and Charles R. Martin
pp 15646–15647
Publication Date (Web): November 10, 2004 (Communication)
DOI: 10.1021/ja044948v

Initial Observation of Magnetization Hysteresis and Quantum Tunneling in Mixed Manganese−Lanthanide Single-Molecule Magnets

Abhudaya Mishra, Wolfgang Wernsdorfer, Khalil A. Abboud, and George Christou
pp 15648–15649
Publication Date (Web): November 12, 2004 (Communication)
DOI: 10.1021/ja0452727

Stannylative Cycloaddition of Enynes Catalyzed by Palladium−Iminophosphine

Yoshiaki Nakao, Yasuhiro Hirata, Shinjiro Ishihara, Shinichi Oda, Tomoya Yukawa, Eiji Shirakawa, and Tamejiro Hiyama
pp 15650–15651
Publication Date (Web): November 11, 2004 (Communication)
DOI: 10.1021/ja044429s

Asymmetric α-Alkylation of N‘-tert-Butanesulfinyl Amidines. Application to the Total Synthesis of (6R,7S)-7-Amino-7,8-dihydro-α-bisabolene

Takuya Kochi and Jonathan A. Ellman
pp 15652–15653
Publication Date (Web): November 12, 2004 (Communication)
DOI: 10.1021/ja044753n

Site-Specific Incorporation of the Mucin-Type N-Acetylgalactosamine-α-O-threonine into Protein in Escherichia coli

Ran Xu, Sarah R. Hanson, Zhiwen Zhang, Yu-Ying Yang, Peter G. Schultz, and Chi-Huey Wong
pp 15654–15655
Publication Date (Web): November 11, 2004 (Communication)
DOI: 10.1021/ja044711z

Cell-Specific Delivery of a Chemotherapeutic to Lung Cancer Cells

Xin Zhou, Ya-Ching Chang, Tsukasa Oyama, Michael J. McGuire, and Kathlynn C. Brown
pp 15656–15657
Publication Date (Web): November 10, 2004 (Communication)
DOI: 10.1021/ja0446496

The Hydratase Activity of Malonate Semialdehyde Decarboxylase:  Mechanistic and Evolutionary Implications

Gerrit J. Poelarends, Hector Serrano, William H. Johnson, Jr., David W. Hoffman, and Christian P. Whitman
pp 15658–15659
Publication Date (Web): November 12, 2004 (Communication)
DOI: 10.1021/ja044304n

Direct Observation of Enantiomer Discrimination of Epoxides by Chiral Salen Complexes Using ENDOR

Ian A. Fallis, Damien M. Murphy, David J. Willock, Richard J. Tucker, Robert D. Farley, Robert Jenkins, and Robert R. Strevens
pp 15660–15661
Publication Date (Web): November 12, 2004 (Communication)
DOI: 10.1021/ja045491s

Oxonia-Cope Prins Cyclizations:  A Facile Method for the Synthesis of Tetrahydropyranones Bearing Quaternary Centers

Jackline E. Dalgard and Scott D. Rychnovsky
pp 15662–15663
Publication Date (Web): November 12, 2004 (Communication)
DOI: 10.1021/ja044736y

Total Synthesis of (±)-Pentacycloanammoxic Acid

Vincent Mascitti and E. J. Corey
pp 15664–15665
Publication Date (Web): November 11, 2004 (Communication)
DOI: 10.1021/ja044089a

Stille Coupling of Stereochemically Defined α-Sulfonamidoorganostannanes

Kevin W. Kells and J. Michael Chong
pp 15666–15667
Publication Date (Web): November 11, 2004 (Communication)
DOI: 10.1021/ja044354s

ARTICLES

Correlated C−C and C−O Bond Conformations in Saccharide Hydroxymethyl Groups:  Parametrization and Application of Redundant 1H−1H, 13C−1H, and 13C−13C NMR J-Couplings

Christophe Thibaudeau, Roland Stenutz, Brian Hertz, Thomas Klepach, Shikai Zhao, Qingquan Wu, Ian Carmichael, and Anthony S. Serianni
pp 15668–15685
Publication Date (Web): November 11, 2004 (Article)
DOI: 10.1021/ja0306718

Isolation of Fast Purine Nucleotide Synthase Ribozymes

Matthew W. L. Lau, Kelly E. C. Cadieux, and Peter J. Unrau
pp 15686–15693
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja045387a

Kinetics and Mechanism of •NO2 Reacting with Various Oxidation States of Myoglobin

Sara Goldstein, Gabor Merenyi, and Amram Samuni
pp 15694–15701
Publication Date (Web): November 11, 2004 (Article)
DOI: 10.1021/ja046186+

Dynamics of Hemoglobin in Human Erythrocytes and in Solution:  Influence of Viscosity Studied by Ultrafast Vibrational Echo Experiments

Brian L. McClain, Ilya J. Finkelstein, and M. D. Fayer
pp 15702–15710
Publication Date (Web): November 10, 2004 (Article)
DOI: 10.1021/ja0454790

Loop-Contraction Mutagenesis of Type 1 Copper Sites

Sachiko Yanagisawa and Christopher Dennison
pp 15711–15719
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja047295r

Promoting Vibrations in Human Purine Nucleoside Phosphorylase. A Molecular Dynamics and Hybrid Quantum Mechanical/Molecular Mechanical Study

Sara Núñez, Dimitri Antoniou, Vern L. Schramm, and Steven D. Schwartz
pp 15720–15729
Publication Date (Web): November 5, 2004 (Article)
DOI: 10.1021/ja0457563

A Proficient Enzyme:  Insights on the Mechanism of Orotidine Monophosphate Decarboxylase from Computer Simulations

Simone Raugei, Michele Cascella, and Paolo Carloni
pp 15730–15737
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja0455143

Probing the Hydrophobic Cavity of Lipid Transfer Protein from Nicotiana tabacum through Xenon-Based NMR Spectroscopy

Lionel Dubois, Pedro Da Silva, Céline Landon, J. Gaspard Huber, Michel Ponchet, Françoise Vovelle, Patrick Berthault, and Hervé Desvaux
pp 15738–15746
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja046195i

Synthetic Ion Channel Activity Documented by Electrophysiological Methods in Living Cells

W. Matthew Leevy, James E. Huettner, Robert Pajewski, Paul H. Schlesinger, and George W. Gokel
pp 15747–15753
Publication Date (Web): November 10, 2004 (Article)
DOI: 10.1021/ja046626x

Assembly of Well-Aligned Multiwalled Carbon Nanotubes in Confined Polyacrylonitrile Environments:  Electrospun Composite Nanofiber Sheets

Jason J. Ge, Haoqing Hou, Qing Li, Matthew J. Graham, Andreas Greiner, Darrell H. Reneker, Frank W. Harris, and Stephen Z. D. Cheng
pp 15754–15761
Publication Date (Web): November 10, 2004 (Article)
DOI: 10.1021/ja048648p

Control of Peptide Structure and Recognition by Fe(III)-Induced Helix Destabilization

Shiroh Futaki, Tatsuto Kiwada, and Yukio Sugiura
pp 15762–15769
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja046870o

N-Halosuccinimide/BF3−H2O, Efficient Electrophilic Halogenating Systems for Aromatics

G. K. Surya Prakash, Thomas Mathew, Dushyanthi Hoole, Pierre M. Esteves, Qi Wang, Golam Rasul, and George A. Olah
pp 15770–15776
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja0465247

Hydration of Pyridylketenes:  Formation of Acid Enol and Dihydropyridine (Eneaminone) Transients

Annette D. Allen, Andrei V. Fedorov, Thomas T. Tidwell, and Sinisa Vukovic
pp 15777–15783
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja047623n

Hybridization of Oligonucleotide-Modified Silver and Gold Nanoparticles in Aqueous Dispersions and on Gold Films

Iryna Tokareva and Eliza Hutter
pp 15784–15789
Publication Date (Web): November 11, 2004 (Article)
DOI: 10.1021/ja046779k

Direct Measurement of the Hydrogen-Bonding Effect on the Intrinsic Redox Potentials of [4Fe−4S] Cubane Complexes

Xin Yang, Shuqiang Niu, Toshiko Ichiye, and Lai-Sheng Wang
pp 15790–15794
Publication Date (Web): November 6, 2004 (Article)
DOI: 10.1021/ja045709a

A New Type of Intermediate, C+(BCH3)11- ↔ C(BCH3)11, in a Grob Fragmentation Coupled with Intramolecular Hydride Transfer. A Nonclassical Carbocation Ylide or a Carbenoid?

Kamesh Vyakaranam, Stefanie Körbe, Hana Divišová, and Josef Michl
pp 15795–15801
Publication Date (Web): November 11, 2004 (Article)
DOI: 10.1021/ja0466558

Linear Rheology of Water-Soluble Reversible Neodymium(III) Coordination Polymers

Tina Vermonden, Mies J. van Steenbergen, Nicolaas A. M. Besseling, Antonius T. M. Marcelis, Wim E. Hennink, Ernst J. R. Sudhölter, and Martien A. Cohen Stuart
pp 15802–15808
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja0458928

Difference RuleA New Thermodynamic Principle:  Prediction of Standard Thermodynamic Data for Inorganic Solvates

H. Donald Brooke Jenkins and Leslie Glasser
pp 15809–15817
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja040137f

Synthetic, Structural, and Mechanistic Aspects of an Amine Activation Process Mediated at a Zwitterionic Pd(II) Center

Connie C. Lu and Jonas C. Peters
pp 15818–15832
Publication Date (Web): November 10, 2004 (Article)
DOI: 10.1021/ja046415s

Insignificance of P−H···P Hydrogen Bonding:  Structural Chemistry of Neutral and Protonated 1,8-Di(phosphinyl)naphthalene

Stephan A. Reiter, Stefan D. Nogai, Konstantin Karaghiosoff, and Hubert Schmidbaur
pp 15833–15843
Publication Date (Web): November 10, 2004 (Article)
DOI: 10.1021/ja045460x

Dynamic and Redox Active Pillared Bilayer Open Framework:  Single-Crystal-to-Single-Crystal Transformations upon Guest Removal, Guest Exchange, and Framework Oxidation

Hye Jin Choi and Myunghyun Paik Suh
pp 15844–15851
Publication Date (Web): November 10, 2004 (Article)
DOI: 10.1021/ja0466715

Self-Assembly and Molecular Recognition of a Luminescent Gold Rectangle

Ronger Lin, John H. K. Yip, Ke Zhang, Lip Lin Koh, Kwok-Yin Wong, and Kam Piu Ho
pp 15852–15869
Publication Date (Web): November 11, 2004 (Article)
DOI: 10.1021/ja0456508

Tuning the Hemolytic and Antibacterial Activities of Amphiphilic Polynorbornene Derivatives

M. Firat Ilker, Klaus Nüsslein, Gregory N. Tew, and E. Bryan Coughlin
pp 15870–15875
Publication Date (Web): November 13, 2004 (Article)
DOI: 10.1021/ja045664d

Nitrile-Functionalized Pyridinium Ionic Liquids:  Synthesis, Characterization, and Their Application in Carbon−Carbon Coupling Reactions

Dongbin Zhao, Zhaofu Fei, Tilmann J. Geldbach, Rosario Scopelliti, and Paul J. Dyson
pp 15876–15882
Publication Date (Web): November 13, 2004 (Article)
DOI: 10.1021/ja0463482

Contiguous versus Segmented Hydrophobicity in Micellar Systems

Fredric M. Menger and Ashley L. Galloway
pp 15883–15889
Publication Date (Web): November 11, 2004 (Article)
DOI: 10.1021/ja040105s

Surface Reaction of Alkynes and Alkenes with H-Si(111):  A Density Functional Theory Study

Noboru Takeuchi, Yosuke Kanai, and Annabella Selloni
pp 15890–15896
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja046702w

Molecular Conductance:  Chemical Trends of Anchoring Groups

San-Huang Ke, Harold U. Baranger, and Weitao Yang
pp 15897–15904
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja047367e

Structure and Dynamics of a Molecular Hydrogel Derived from a Tripodal Cholamide

Samrat Mukhopadhyay, Uday Maitra, Ira, Guruswamy Krishnamoorthy, Judith Schmidt, and Yeshayahu Talmon
pp 15905–15914
Publication Date (Web): November 10, 2004 (Article)
DOI: 10.1021/ja046788t

Consistent Experimental and Theoretical Evidence for Long-Lived Intermediate Radicals in Living Free Radical Polymerization

Achim Feldermann, Michelle L. Coote, Martina H. Stenzel, Thomas P. Davis, and Christopher Barner-Kowollik
pp 15915–15923
Publication Date (Web): November 12, 2004 (Article)
DOI: 10.1021/ja046292b

ADDITIONS AND CORRECTIONS

Identification of Inhibitors for UDP-Galactopyranose Mutase [J. Am. Chem. Soc. 2004, 126, 10532−10533].

Michelle Soltero-Higgin, Erin E. Carlson, John H. Phillips, and Laura L. Kiessling
p 15924
Publication Date (Web): November 11, 2004 (Addition/Correction)
DOI: 10.1021/ja040825z
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