Table of Contents

Journal Cover
March 7, 2007
Volume 129, Issue 9
Pages 2410-2726
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COMMUNICATIONS

Catalytic Asymmetric Rearrangement of α,α-Disubstituted α-Siloxy Aldehydes to Optically Active Acyloins Using Axially Chiral Organoaluminum Lewis Acids

Takashi Ooi, Kohsuke Ohmatsu, and Keiji Maruoka
pp 2410–2411
Publication Date (Web): February 10, 2007 (Communication)
DOI: 10.1021/ja063051q

Etching Colloidal Gold Nanocrystals with Hyperbranched and Multivalent Polymers:  A New Route to Fluorescent and Water-Soluble Atomic Clusters

Hongwei Duan and Shuming Nie
pp 2412–2413
Publication Date (Web): February 13, 2007 (Communication)
DOI: 10.1021/ja067727t

Slow Conformational Dynamics and Unfolding of the Calmodulin C-Terminal Domain

Yng-Gwei Chen and Gerhard Hummer
pp 2414–2415
Publication Date (Web): February 10, 2007 (Communication)
DOI: 10.1021/ja067791a

Transition of Ionic Liquid [bmim][PF6] from Liquid to High-Melting-Point Crystal When Confined in Multiwalled Carbon Nanotubes

Shimou Chen, Guozhong Wu, Maolin Sha, and Shirong Huang
pp 2416–2417
Publication Date (Web): February 09, 2007 (Communication)
DOI: 10.1021/ja067972c

Enhanced Sensitized NIR Luminescence from Gold Nanoparticles via Energy Transfer from Surface-Bound Fluorophores

Marco Montalti, Nelsi Zaccheroni, Luca Prodi, Niamh O'Reilly, and Stuart L. James
pp 2418–2419
Publication Date (Web): February 08, 2007 (Communication)
DOI: 10.1021/ja068095d

Heterogeneously Catalyzed Living Cationic Polymerization of Isobutyl Vinyl Ether Using Iron(III) Oxide

Arihiro Kanazawa, Shokyoku Kanaoka, and Sadahito Aoshima
pp 2420–2421
Publication Date (Web): February 09, 2007 (Communication)
DOI: 10.1021/ja068124k

Dynamic Recompartmentalization of Supported Lipid Bilayers Using Focused Femtosecond Laser Pulses

Andreia M. Smith, Thomas Huser, and Atul N. Parikh
pp 2422–2423
Publication Date (Web): February 09, 2007 (Communication)
DOI: 10.1021/ja065626p

Formation of a Cobalt(III) Imido from a Cobalt(II) Amido Complex. Evidence for Proton-Coupled Electron Transfer

Ryan E. Cowley, Ranko P. Bontchev, John Sorrell, Orcino Sarracino, Yanhua Feng, Haobin Wang, and Jeremy M. Smith
pp 2424–2425
Publication Date (Web): February 09, 2007 (Communication)
DOI: 10.1021/ja066899n

Design, Synthesis, and Characterization of Binuclear Ni(II) Complexes with Inherent Helical Chirality

Vadim A. Soloshonok and Hisanori Ueki
pp 2426–2427
Publication Date (Web): February 08, 2007 (Communication)
DOI: 10.1021/ja0671215

A Dramatic Effect of Lewis-Acid Catalysts on Nickel-Catalyzed Carbocyanation of Alkynes

Yoshiaki Nakao, Akira Yada, Shiro Ebata, and Tamejiro Hiyama
pp 2428–2429
Publication Date (Web): February 13, 2007 (Communication)
DOI: 10.1021/ja067364x

Gd-Loaded Liposomes as T1, Susceptibility, and CEST Agents, All in One

Silvio Aime, Daniela Delli Castelli, Dale Lawson, and Enzo Terreno
pp 2430–2431
Publication Date (Web): February 09, 2007 (Communication)
DOI: 10.1021/ja0677867

Isotropic Bicelles Stabilize the Functional Form of a Small Multidrug-Resistance Pump for NMR Structural Studies

Sébastien F. Poget, Sean M. Cahill, and Mark E. Girvin
pp 2432–2433
Publication Date (Web): February 07, 2007 (Communication)
DOI: 10.1021/ja0679836

Synthetic Macrolides that Inhibit Breast Cancer Cell Migration in Vitro

Belhu B. Metaferia, Lin Chen, Heather L. Baker, Xin-Yun Huang, and Carole A. Bewley
pp 2434–2435
Publication Date (Web): February 13, 2007 (Communication)
DOI: 10.1021/ja068538d

Interplay of EnE‘3-nC Valence Isomers (E, E‘ = Si, Ge):  Bicyclo[1.1.0]butanes with Very Short Bridging Bonds and Their Isomerization to Alkyl-Substituted Cyclopropenes

Vladimir Ya. Lee, Hiroyuki Yasuda, and Akira Sekiguchi
pp 2436–2437
Publication Date (Web): February 13, 2007 (Communication)
DOI: 10.1021/ja068229n

Spirodiepoxide Reaction with Cuprates

Partha Ghosh, Stephen D. Lotesta, and Lawrence J. Williams
pp 2438–2439
Publication Date (Web): February 09, 2007 (Communication)
DOI: 10.1021/ja068813w

Self-Assembly and Self-Metallization of Porphyrin Nanosheets

Zhongchun Wang, Zhiyong Li, Craig J. Medforth, and John A. Shelnutt
pp 2440–2441
Publication Date (Web): February 10, 2007 (Communication)
DOI: 10.1021/ja068250o

Luminescence from Neptunyl(VI) Species in Solution

Catherine Talbot-Eeckelaers, Simon J. A. Pope, Amanda J. Hynes, Roy Copping, Chris J. Jones, Robin J. Taylor, Stephen Faulkner, Daniel Sykes, Francis R. Livens, and Iain May
pp 2442–2443
Publication Date (Web): February 13, 2007 (Communication)
DOI: 10.1021/ja068522n

Critical Importance of Length-Scale Dependence in Implicit Modeling of Hydrophobic Interactions

Jianhan Chen and Charles L. Brooks III
pp 2444–2445
Publication Date (Web): February 09, 2007 (Communication)
DOI: 10.1021/ja068383+

Electrochemical Oxidation of Water by an Adsorbed μ-Oxo-Bridged Ru Complex

Feng Liu, Thomas Cardolaccia, Brooks J. Hornstein, Jon R. Schoonover, and Thomas J. Meyer
pp 2446–2447
Publication Date (Web): February 07, 2007 (Communication)
DOI: 10.1021/ja068630+

Noncovalent Functionalization of Carbon Nanotubes by Fluorescein−Polyethylene Glycol:  Supramolecular Conjugates with pH-Dependent Absorbance and Fluorescence

Nozomi Nakayama-Ratchford, Sarunya Bangsaruntip, Xiaoming Sun, Kevin Welsher, and Hongjie Dai
pp 2448–2449
Publication Date (Web): February 07, 2007 (Communication)
DOI: 10.1021/ja068684j

Rectangular Nanostructuring of Au(111) Surfaces by Self-Assembly of Size-Selected Thiacrown Ether Macrocycles

Aymeric Nion, Peng Jiang, Alexandre Popoff, and Denis Fichou
pp 2450–2451
Publication Date (Web): February 13, 2007 (Communication)
DOI: 10.1021/ja068709e

Gold(I)-Catalyzed Enantioselective Intramolecular Hydroamination of Allenes

Rebecca L. LaLonde, Benjamin D. Sherry, Eun Joo Kang, and F. Dean Toste
pp 2452–2453
Publication Date (Web): February 10, 2007 (Communication)
DOI: 10.1021/ja068819l

Facile Activation of Hydrogen by an Unsaturated Platinum−Osmium Cluster Complex

Richard D. Adams, Burjor Captain, and Lei Zhu
pp 2454–2455
Publication Date (Web): February 10, 2007 (Communication)
DOI: 10.1021/ja0688272

Reactivation of the p53 Tumor Suppressor Pathway by a Stapled p53 Peptide

Federico Bernal, Andrew F. Tyler, Stanley J. Korsmeyer, Loren D. Walensky, and Gregory L. Verdine
pp 2456–2457
Publication Date (Web): February 07, 2007 (Communication)
DOI: 10.1021/ja0693587

ARTICLES

Thermodynamic Stability of Boron:  The Role of Defects and Zero Point Motion

Michiel J. van Setten, Matthé A. Uijttewaal, Gilles A. de Wijs, and Robert A. de Groot
pp 2458–2465
Publication Date (Web): February 13, 2007 (Article)
DOI: 10.1021/ja0631246

Exploring the Subtleties of Drug−Receptor Interactions:  The Case of Matrix Metalloproteinases

Ivano Bertini, Vito Calderone, Marco Fragai, Andrea Giachetti, Mauro Loconte, Claudio Luchinat, Massimiliano Maletta, Cristina Nativi, and Kwon Joo Yeo
pp 2466–2475
Publication Date (Web): February 02, 2007 (Article)
DOI: 10.1021/ja065156z

Energy-Resolved Collision-Induced Dissociation Cross Sections of 2:1 Bis-oxazoline Copper Complexes. Nonbonded Interactions and Nonlinear Effects

Eva Zocher, Rolf Dietiker, and Peter Chen
pp 2476–2481
Publication Date (Web): February 09, 2007 (Article)
DOI: 10.1021/ja065390p

Reactive Nature of Dopamine as a Surface Functionalization Agent in Iron Oxide Nanoparticles

Michael D. Shultz, J. Ulises Reveles, Shiv N. Khanna, and Everett E. Carpenter
pp 2482–2487
Publication Date (Web): February 10, 2007 (Article)
DOI: 10.1021/ja0651963

Effect of Deuterium on the Kinetics of 1,5-Hydrogen Shifts:  5-Dideuteriomethylene-2,4,6,7,9-pentamethyl-11,11a- dihydro-12H-naphthacene

William von E. Doering and Edmund J. Keliher
pp 2488–2495
Publication Date (Web): February 09, 2007 (Article)
DOI: 10.1021/ja066018c

Surface Chemistry of Aerosolized Silicon Nanoparticles:  Evolution and Desorption of Hydrogen from 6-nm Diameter Particles

Jason Holm and Jeffrey T. Roberts
pp 2496–2503
Publication Date (Web): February 07, 2007 (Article)
DOI: 10.1021/ja0658970

Effect of Field Direction on Electrowetting in a Nanopore

Dusan Bratko, Christopher D. Daub, Kevin Leung, and Alenka Luzar
pp 2504–2510
Publication Date (Web): February 07, 2007 (Article)
DOI: 10.1021/ja0659370

Hierarchical Chiral Framework Based on a Rigid Adamantane Tripod on Au(111)

Satoshi Katano, Yousoo Kim, Hiroaki Matsubara, Toshikazu Kitagawa, and Maki Kawai
pp 2511–2515
Publication Date (Web): February 06, 2007 (Article)
DOI: 10.1021/ja065893v

Hydrogen-Induced Transition from Dissociative to Molecular Chemisorption of CO on Vanadium Clusters

Ingmar Swart, André Fielicke, Britta Redlich, Gerard Meijer, Bert M. Weckhuysen, and Frank M. F. de Groot
pp 2516–2520
Publication Date (Web): January 31, 2007 (Article)
DOI: 10.1021/ja066261b

“Amide Resonance” Correlates with a Breadth of C−N Rotation Barriers

Carl R. Kemnitz and Mark J. Loewen
pp 2521–2528
Publication Date (Web): February 13, 2007 (Article)
DOI: 10.1021/ja0663024

Reactions of Monomeric [1,2,4-(Me3C)3C5H2]2CeH and CO with or without H2:  An Experimental and Computational Study

Evan L. Werkema, Laurent Maron, Odile Eisenstein, and Richard A. Andersen
pp 2529–2541
Publication Date (Web): February 08, 2007 (Article)
DOI: 10.1021/ja066482h

Concerted Molecular Displacements in a Thermally-Induced Solid-State Transformation in Crystals of DL-Norleucine

Jamshed Anwar, Sigrid C. Tuble, and John Kendrick
pp 2542–2547
Publication Date (Web): February 08, 2007 (Article)
DOI: 10.1021/ja066686y

Cyclic Modular β-Sheets

R. Jeremy Woods, Justin O. Brower, Elena Castellanos, Mehrnoosh Hashemzadeh, Omid Khakshoor, Wade A. Russu, and James S. Nowick
pp 2548–2558
Publication Date (Web): February 13, 2007 (Article)
DOI: 10.1021/ja0667965

Syntheses and Electronic Structures of One-Electron-Oxidized Group 10 Metal(II)−(Disalicylidene)diamine Complexes (Metal = Ni, Pd, Pt)

Yuichi Shimazaki, Tatsuo Yajima, Fumito Tani, Satoru Karasawa, Koichi Fukui, Yoshinori Naruta, and Osamu Yamauchi
pp 2559–2568
Publication Date (Web): February 10, 2007 (Article)
DOI: 10.1021/ja067022r

Methyl Chloride Production from Methane over Lanthanum-Based Catalysts

Simon G. Podkolzin, Eric E. Stangland, Mark E. Jones, Elvira Peringer, and Johannes A. Lercher
pp 2569–2576
Publication Date (Web): February 13, 2007 (Article)
DOI: 10.1021/ja066913w
Sponsored Access Sponsored Access

Classification of Water Molecules in Protein Binding Sites

Caterina Barillari, Justine Taylor, Russell Viner, and Jonathan W. Essex
pp 2577–2587
Publication Date (Web): February 09, 2007 (Article)
DOI: 10.1021/ja066980q

Spectroscopic Observation of Conformation-Dependent Charge Distribution in a Molecular Cation

Kang Taek Lee, Hyung Min Kim, Kyu Young Han, Jiha Sung, Kwang Jun Lee, and Seong Keun Kim
pp 2588–2592
Publication Date (Web): February 07, 2007 (Article)
DOI: 10.1021/ja0670308

Layer-Engineering of High-Tc Superconductors:  (Cu,Mo)Sr2(Ce,Y)4Cu2O13+δ with a Quadruple-Fluorite-Layer Block Between CuO2 Planes

Inga Grigoraviciute, Hisao Yamauchi, and Maarit Karppinen
pp 2593–2596
Publication Date (Web): February 07, 2007 (Article)
DOI: 10.1021/ja0671316

Ultrafast Study of p-Biphenylyldiazoethane. The Chemistry of the Diazo Excited State and the Relaxed Carbene

Jin Wang, Gotard Burdzinski, Terry L. Gustafson, and Matthew S. Platz
pp 2597–2606
Publication Date (Web): February 10, 2007 (Article)
DOI: 10.1021/ja067213u

Three-Dimensional Porous Coordination Polymer Functionalized with Amide Groups Based on Tridentate Ligand:  Selective Sorption and Catalysis

Shinpei Hasegawa, Satoshi Horike, Ryotaro Matsuda, Shuhei Furukawa, Katsunori Mochizuki, Yoshinori Kinoshita, and Susumu Kitagawa
pp 2607–2614
Publication Date (Web): February 09, 2007 (Article)
DOI: 10.1021/ja067374y

Crystal Nucleation, Growth, and Morphology of the Synthetic Malaria Pigment β-Hematin and the Effect Thereon by Quinoline Additives:  The Malaria Pigment as a Target of Various Antimalarial Drugs

Inna Solomonov, Maria Osipova, Yishay Feldman, Carsten Baehtz, Kristian Kjaer, Ian K. Robinson, Grant T. Webster, Don McNaughton, Bayden R. Wood, Isabelle Weissbuch, and Leslie Leiserowitz
pp 2615–2627
Publication Date (Web): February 10, 2007 (Article)
DOI: 10.1021/ja0674183

Size-Sorted Anionic Iron Oxide Nanomagnets as Colloidal Mediators for Magnetic Hyperthermia

Jean-Paul Fortin, Claire Wilhelm, Jacques Servais, Christine Ménager, Jean-Claude Bacri, and Florence Gazeau
pp 2628–2635
Publication Date (Web): February 01, 2007 (Article)
DOI: 10.1021/ja067457e

Mechanical Stabilization Effect of Water on a Membrane-like System

Matteo Castronovo, Fouzia Bano, Simone Raugei, Denis Scaini, Martina Dell'Angela, Robert Hudej, Loredana Casalis, and Giacinto Scoles
pp 2636–2641
Publication Date (Web): February 09, 2007 (Article)
DOI: 10.1021/ja067462i

Origin of Oxide Sensitivity in Gold-Based Catalysts:  A First Principle Study of CO Oxidation over Au Supported on Monoclinic and Tetragonal ZrO2

Chuan-Ming Wang, Kang-Nian Fan, and Zhi-Pan Liu
pp 2642–2647
Publication Date (Web): February 10, 2007 (Article)
DOI: 10.1021/ja067510z

Total Syntheses, Fragmentation Studies, and Antitumor/Antiproliferative Activities of FR901464 and Its Low Picomolar Analogue

Brian J. Albert, Ananthapadmanabhan Sivaramakrishnan, Tadaatsu Naka, Nancy L. Czaicki, and Kazunori Koide
pp 2648–2659
Publication Date (Web): February 06, 2007 (Article)
DOI: 10.1021/ja067870m
Sponsored Access Sponsored Access

Minimization of a Protein−DNA Dimerizer

Ryan L. Stafford, Hans-Dieter Arndt, Mary L. Brezinski, Aseem Z. Ansari, and Peter B. Dervan
pp 2660–2668
Publication Date (Web): February 10, 2007 (Article)
DOI: 10.1021/ja067971k

Organically Modified Silica Nanoparticles Co-encapsulating Photosensitizing Drug and Aggregation-Enhanced Two-Photon Absorbing Fluorescent Dye Aggregates for Two-Photon Photodynamic Therapy

Sehoon Kim, Tymish Y. Ohulchanskyy, Haridas E. Pudavar, Ravindra K. Pandey, and Paras N. Prasad
pp 2669–2675
Publication Date (Web): February 09, 2007 (Article)
DOI: 10.1021/ja0680257

Charge Density of Divalent Metal Cations Determines RNA Stability

Eda Koculi, Changbong Hyeon, D. Thirumalai, and Sarah A. Woodson
pp 2676–2682
Publication Date (Web): February 13, 2007 (Article)
DOI: 10.1021/ja068027r

Self-Assembled Heterotrimeric Collagen Triple Helices Directed through Electrostatic Interactions

Varun Gauba and Jeffrey D. Hartgerink
pp 2683–2690
Publication Date (Web): February 13, 2007 (Article)
DOI: 10.1021/ja0683640

The Participation of Alkynylboronates in Inverse Electron Demand [4 + 2] Cycloadditions:  A Mechanistic Study

Enrique Gomez-Bengoa, Matthew D. Helm, Andrew Plant, and Joseph P. A. Harrity
pp 2691–2699
Publication Date (Web): February 10, 2007 (Article)
DOI: 10.1021/ja068527k

Shapes and Noncovalent Interactions of Oligomers:  The Rotational Spectrum of the Difluoromethane Trimer

Susana Blanco, Sonia Melandri, Paolo Ottaviani, and Walther Caminati
pp 2700–2703
Publication Date (Web): February 09, 2007 (Article)
DOI: 10.1021/ja068599b

Does Aromaticity in a Reaction Product Increase or Decrease the Intrinsic Barrier? Kinetics of the Reversible Deprotonation of Benzofuran-3(2H)-one and Benzothiophene-3(2H)-one

Claude F. Bernasconi and Moisés Pérez-Lorenzo
pp 2704–2712
Publication Date (Web): February 14, 2007 (Article)
DOI: 10.1021/ja067118l

Carbocyclization by Radical Closure onto O-Trityl Oximes:  Dramatic Effect of Diphenyl Diselenide

Derrick L. J. Clive, Mai P. Pham, and Rajendra Subedi
pp 2713–2717
Publication Date (Web): February 07, 2007 (Article)
DOI: 10.1021/ja067117t

Ligand-Dependent Catalytic Cycle and Role of Styrene in Nickel-Catalyzed Anhydride Cross-Coupling:  Evidence for Turnover-Limiting Reductive Elimination

Jeffrey B. Johnson, Eric A. Bercot, John M. Rowley, Geoffrey W. Coates, and Tomislav Rovis
pp 2718–2725
Publication Date (Web): February 13, 2007 (Article)
DOI: 10.1021/ja067845g

BOOK REVIEWS

Heterocyclic Antitumor Antibiotics. Topics in Heterocyclic Chemistry, 02 Edited by Moses Lee (Hope College, Holland, MI). Series Edited by R. R. Gupta. Springer:  Berlin, Heidelberg, New York. 2006. xiv + 252 pp. $149.00. ISBN 3-540-30982-9.

Gary I. Dmitrienko
p 2726
Publication Date (Web): February 09, 2007 (Book Review)
DOI: 10.1021/ja0697830
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