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Self-Powered Potentiometric Sensor Based on a Passive Signal Amplifier with Electronic Paper Display
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    Self-Powered Potentiometric Sensor Based on a Passive Signal Amplifier with Electronic Paper Display
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    • Aori Qileng
      Aori Qileng
      Department of Inorganic and Analytical Chemistry, University of Geneva, Quai Ernest-Ansermet 30, CH-1211 Geneva, Switzerland
      Key Laboratory for Biobased Materials and Energy of Ministry of Education, College of Materials and Energy, South China Agricultural University, Guangzhou 510642, China
      More by Aori Qileng
    • Yaotian Wu
      Yaotian Wu
      Department of Inorganic and Analytical Chemistry, University of Geneva, Quai Ernest-Ansermet 30, CH-1211 Geneva, Switzerland
      More by Yaotian Wu
    • Yingju Liu*
      Yingju Liu
      Key Laboratory for Biobased Materials and Energy of Ministry of Education, College of Materials and Energy, South China Agricultural University, Guangzhou 510642, China
      *E-mail: [email protected] (Y. Liu).
      More by Yingju Liu
    • Eric Bakker*
      Eric Bakker
      Department of Inorganic and Analytical Chemistry, University of Geneva, Quai Ernest-Ansermet 30, CH-1211 Geneva, Switzerland
      *E-mail: [email protected] (E. Bakker).
      More by Eric Bakker
    Other Access OptionsSupporting Information (2)

    Analytical Chemistry

    Cite this: Anal. Chem. 2023, 95, 48, 17444–17449
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    https://doi.org/10.1021/acs.analchem.3c04323
    Published November 18, 2023
    Copyright © 2023 American Chemical Society

    Abstract

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    Self-powered potentiometric sensors are attractive because of their simple operation, low cost, fast response, and ability to be integrated with electronic components. Self-powered potentiometric sensors that give a direct colorimetric output are especially interesting, because no power supply is needed, which dramatically reduces waste. Recently reported work from our group using an electronic paper display, however, exhibits limitations, because the visualization of small pH changes is difficult. A self-powered ion-selective potentiometric sensor is introduced here that may amplify the e-paper pixel sensitivity by improving the self-powered circuit. The voltage is amplified by changing the circuit from incorporating parallel to incorporating serial capacitors. With three such capacitors, a greatly improved sensitivity is observed, amplifying the absorbance 3-fold. A portable device is realized that changes the position of the capacitors from parallel to serial through a simple mechanical sliding action. As a result, the pH information on the sample is more easily visualized with a pH uncertainty of about 0.1 when comparing the e-paper output to a color card.

    Copyright © 2023 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.analchem.3c04323.

    • Charging process of the e-paper, optical response of pixel and data of sensor in the detection of real sample (PDF)

    • Video S1: Video showing operation and switching speed (MP4)

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    Cited By

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    This article is cited by 1 publications.

    1. Yaotian Wu, Yupu Zhang, Aori Qileng, Eric Bakker. Self-Powered Potentiometric Sensor with Relational Operation Function to Capture Concentration Excursions. Analytical Chemistry 2024, 96 (46) , 18401-18407. https://doi.org/10.1021/acs.analchem.4c03081

    Analytical Chemistry

    Cite this: Anal. Chem. 2023, 95, 48, 17444–17449
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.analchem.3c04323
    Published November 18, 2023
    Copyright © 2023 American Chemical Society

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