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Interpenetrated Luminescent Metal–Organic Frameworks based on 1H-Indazole-5-carboxylic Acid
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    Interpenetrated Luminescent Metal–Organic Frameworks based on 1H-Indazole-5-carboxylic Acid
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    Crystal Growth & Design

    Cite this: Cryst. Growth Des. 2020, 20, 7, 4550–4560
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    https://doi.org/10.1021/acs.cgd.0c00345
    Published May 13, 2020
    Copyright © 2020 American Chemical Society

    Abstract

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    Herein we report the formation and characterization of two novel Zn-based multifunctional metal–organic frameworks (MOFs) based on 1H-indazole-5-carboxylic acid and bipyridine-like linkers, synthesized by soft solvothermal routes. These materials possess isoreticular 2-fold interpenetrated three-dimensional structures that afford a flexible character and allow porosity modulation of the MOFs as confirmed by CO2 sorption measurements. Apart from this attractive structural feature, the MOFs exhibit fascinating luminescent properties involving both luminescence thermometry and long-lasting phosphorescence.

    Copyright © 2020 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.cgd.0c00345.

    • Additional figures of crystal structures and data, thermogravimetric analysis, powder X-ray diffraction analyses, photoluminescence spectra and lifetimes, TD-DFT computational results (PDF)

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    CCDC 19420131942014 contain the supplementary crystallographic data for this paper. These data can be obtained free of charge via www.ccdc.cam.ac.uk/data_request/cif, or by emailing [email protected], or by contacting The Cambridge Crystallographic Data Centre, 12 Union Road, Cambridge CB2 1EZ, UK; fax: +44 1223 336033.

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    Cited By

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    This article is cited by 9 publications.

    1. Yashuang Li, Hao Li, Shuixiang Zou, Yuanzheng Liu, Hengbo Li, Zhenyu Ji, Zhengyi Di, Cheng Chen, Mingyan Wu. Anion-Induced Structural Transformation of a Cage-Based Metal–Organic Framework. Crystal Growth & Design 2023, 23 (4) , 2264-2271. https://doi.org/10.1021/acs.cgd.2c01315
    2. Ceyhun Kucuk, Sibel Celik, Senay Yurdakul, Namık Özdemir, Hakan Bülbül. Characterization of the synthesized diaqua-bis(indazole-κN2)bis(nitrato-κO)zinc(II) complex and DFT calculations. Journal of Molecular Structure 2024, 1304 , 137666. https://doi.org/10.1016/j.molstruc.2024.137666
    3. Hongfei Jiang, Qiuyu Gong, Renshuai Zhang, Hongye Yuan. Tetrazine-based metal-organic frameworks. Coordination Chemistry Reviews 2024, 499 , 215501. https://doi.org/10.1016/j.ccr.2023.215501
    4. Oier Pajuelo-Corral, Iñigo J. Vitorica-Yrezabal, Antonio Rodríguez-Diéguez, Jose M. Seco, Javier Cepeda. A magnetic Ni-based metal-organic framework with interesting transformation dynamics. Inorganic Chemistry Communications 2023, 27 , 111872. https://doi.org/10.1016/j.inoche.2023.111872
    5. Oskar G. Wood, Chris S. Hawes. Fused aza-heterocyclic ligands: expanding the MOF chemist's toolbox. CrystEngComm 2022, 24 (47) , 8197-8207. https://doi.org/10.1039/D2CE01475K
    6. O. Pajuelo-Corral, S. Pérez-Yáñez, I.J. Vitorica-Yrezabal, G. Beobide, A. Zabala-Lekuona, A. Rodríguez-Diéguez, J.M. Seco, J. Cepeda. A metal-organic framework based on Co(II) and 3-aminoisonicotinate showing specific and reversible colourimetric response to solvent exchange with variable magnet behaviour. Materials Today Chemistry 2022, 24 , 100794. https://doi.org/10.1016/j.mtchem.2022.100794
    7. Amelia M. Swarbrook, Rohan J. Weekes, Jack W. Goodwin, Chris S. Hawes. Ligand isomerism fine-tunes structure and stability in zinc complexes of fused pyrazolopyridines. Dalton Transactions 2022, 51 (3) , 1056-1069. https://doi.org/10.1039/D1DT04007C
    8. Chris S. Hawes. Coordination sphere hydrogen bonding as a structural element in metal–organic Frameworks. Dalton Transactions 2021, 50 (18) , 6034-6049. https://doi.org/10.1039/D1DT00675D
    9. Antonio A. García-Valdivia, Estitxu Echenique-Errandonea, Gloria B. Ramírez-Rodríguez, José M. Delgado-López, Belén Fernández, Sara Rojas, Javier Cepeda, Antonio Rodríguez-Diéguez. Photoluminescent Coordination Polymers Based on Group 12 Metals and 1H-Indazole-6-Carboxylic Acid. Inorganics 2021, 9 (3) , 20. https://doi.org/10.3390/inorganics9030020

    Crystal Growth & Design

    Cite this: Cryst. Growth Des. 2020, 20, 7, 4550–4560
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.cgd.0c00345
    Published May 13, 2020
    Copyright © 2020 American Chemical Society

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