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Download Hi-Res ImageDownload to MS-PowerPointCite This:Chem. Rev. 2024, 124, 7, 4479-4539
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    Phase Engineering of Nanomaterials: Transition Metal Dichalcogenides
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    • Wei Zhai
      Wei Zhai
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Zijian Li
      Zijian Li
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Yongji Wang
      Yongji Wang
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Li Zhai
      Li Zhai
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
      Hong Kong Branch of National Precious Metals Material Engineering Research Center (NPMM), City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Yao Yao
      Yao Yao
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Siyuan Li
      Siyuan Li
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Lixin Wang
      Lixin Wang
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Hua Yang
      Hua Yang
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Banlan Chi
      Banlan Chi
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Jinzhe Liang
      Jinzhe Liang
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Zhenyu Shi
      Zhenyu Shi
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Yiyao Ge
      Yiyao Ge
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
      State Key Laboratory for Advanced Metals and Materials, University of Science and Technology Beijing, Beijing 100083, China
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      Orcidhttps://orcid.org/0000-0002-2546-005X
    • Zhuangchai Lai
      Zhuangchai Lai
      Department of Applied Physics, The Hong Kong Polytechnic University, Hong Kong 999077, China
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      Orcidhttps://orcid.org/0000-0001-8743-6568
    • Qinbai Yun
      Qinbai Yun
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • An Zhang
      An Zhang
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Zhiying Wu
      Zhiying Wu
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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    • Qiyuan He
      Qiyuan He
      Department of Materials Science and Engineering, City University of Hong Kong, Kowloon, Hong Kong 999077, China
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      Orcidhttps://orcid.org/0000-0001-9083-8285
    • Bo Chen
      Bo Chen
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
      State Key Laboratory of Organic Electronics and Information Displays & Jiangsu Key Laboratory for Biosensors, Institute of Advanced Materials (IAM), School of Chemistry and Life Sciences, Nanjing University of Posts and Telecommunications, Nanjing 210023, China
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      Orcidhttps://orcid.org/0000-0001-6743-9251
    • Zhiqi Huang
      Zhiqi Huang
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
      School of Chemistry and Chemical Engineering, Beijing Institute of Technology, Beijing 100081, China
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    • Hua Zhang*
      Hua Zhang
      Department of Chemistry, City University of Hong Kong, Kowloon, Hong Kong 999077, China
      Hong Kong Branch of National Precious Metals Material Engineering Research Center (NPMM), City University of Hong Kong, Kowloon, Hong Kong 999077, China
      Hong Kong Institute for Clean Energy, City University of Hong Kong, Kowloon, Hong Kong 999077, China
      Shenzhen Research Institute, City University of Hong Kong, Shenzhen 518057, China
      *E-mail: [email protected]
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      Orcidhttps://orcid.org/0000-0001-9518-740X
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    Chemical Reviews

    Cite this: Chem. Rev. 2024, 124, 7, 4479–4539
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    https://doi.org/10.1021/acs.chemrev.3c00931
    Published March 29, 2024
    Copyright © 2024 American Chemical Society
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    Abstract

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    Crystal phase, a critical structural characteristic beyond the morphology, size, dimension, facet, etc., determines the physicochemical properties of nanomaterials. As a group of layered nanomaterials with polymorphs, transition metal dichalcogenides (TMDs) have attracted intensive research attention due to their phase-dependent properties. Therefore, great efforts have been devoted to the phase engineering of TMDs to synthesize TMDs with controlled phases, especially unconventional/metastable phases, for various applications in electronics, optoelectronics, catalysis, biomedicine, energy storage and conversion, and ferroelectrics. Considering the significant progress in the synthesis and applications of TMDs, we believe that a comprehensive review on the phase engineering of TMDs is critical to promote their fundamental studies and practical applications. This Review aims to provide a comprehensive introduction and discussion on the crystal structures, synthetic strategies, and phase-dependent properties and applications of TMDs. Finally, our perspectives on the challenges and opportunities in phase engineering of TMDs will also be discussed.

    Copyright © 2024 American Chemical Society

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    Cite this: Chem. Rev. 2024, 124, 7, 4479–4539
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.chemrev.3c00931
    Published March 29, 2024
    Copyright © 2024 American Chemical Society
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