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Download Hi-Res ImageDownload to MS-PowerPointCite This:Chem. Rev. 2019, 119, 13, 7848-7939
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    Understanding Glass through Differential Scanning Calorimetry
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    • Qiuju Zheng
      Qiuju Zheng
      School of Materials Science and Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China
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    • Yanfei Zhang
      Yanfei Zhang
      School of Materials Science and Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China
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    • Maziar Montazerian
      Maziar Montazerian
      Vitreous Materials Laboratory (LaMaV), Department of Materials Engineering (DEMa), Federal University of São Carlos (UFSCar), 13.565-905 São Carlos, SP, Brazil
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      Orcidhttp://orcid.org/0000-0002-1409-9182
    • Ozgur Gulbiten
      Ozgur Gulbiten
      Science and Technology Division, Corning Incorporated, Corning, New York 14831, United States
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      Orcidhttp://orcid.org/0000-0001-9156-7659
    • John C. Mauro
      John C. Mauro
      School of Materials Science and Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China
      Department of Materials Science and Engineering, The Pennsylvania State University, University Park, Pennsylvania 16802, United States
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      Orcidhttp://orcid.org/0000-0002-4319-3530
    • Edgar D. Zanotto
      Edgar D. Zanotto
      Vitreous Materials Laboratory (LaMaV), Department of Materials Engineering (DEMa), Federal University of São Carlos (UFSCar), 13.565-905 São Carlos, SP, Brazil
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    • Yuanzheng Yue*
      Yuanzheng Yue
      School of Materials Science and Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, China
      State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology, Wuhan 430070, China
      Department of Chemistry and Bioscience, Aalborg University, DK-9220 Aalborg, Denmark
      *E-mail: [email protected]
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      Orcidhttp://orcid.org/0000-0002-6048-5236
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    Cite this: Chem. Rev. 2019, 119, 13, 7848–7939
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    https://doi.org/10.1021/acs.chemrev.8b00510
    Published May 23, 2019
    Copyright © 2019 American Chemical Society
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    Abstract

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    Differential scanning calorimetry (DSC) is a powerful tool to address some of the most challenging issues in glass science and technology, such as the nonequilibrium nature of the glassy state and the detailed thermodynamics and kinetics of glass-forming systems during glass transition, relaxation, rejuvenation, polyamorphic transition, and crystallization. The utility of the DSC technique spans across all glass-forming chemistries, including oxide, chalcogenide, metallic, and organic systems, as well as recently discovered metal–organic framework glass-forming systems. Here we present a comprehensive review of the many applications of DSC in glass science with focus on glass transition, relaxation, polyamorphism, and crystallization phenomena. We also emphasize recent advances in DSC characterization technology, including flash DSC and temperature-modulated DSC. This review demonstrates how DSC studies have led to a multitude of relevant advances in the understanding of glass physics, chemistry, and even technology.

    Copyright © 2019 American Chemical Society

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    Cite this: Chem. Rev. 2019, 119, 13, 7848–7939
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