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Applications of Plasmon-Enhanced Nanocatalysis to Organic Transformations

  • Alexandra Gellé
    Alexandra Gellé
    Centre for Green Chemistry and Catalysis, Department of Chemistry, McGill University, 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada
  • Tony Jin
    Tony Jin
    Centre for Green Chemistry and Catalysis, Department of Chemistry, McGill University, 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada
    More by Tony Jin
  • Luis de la Garza
    Luis de la Garza
    Centre for Green Chemistry and Catalysis, Department of Chemistry, McGill University, 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada
  • Gareth D. Price
    Gareth D. Price
    Centre for Green Chemistry and Catalysis, Department of Chemistry, McGill University, 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada
  • Lucas V. Besteiro
    Lucas V. Besteiro
    Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 610054, China
    Centre Énergie Matériaux et Télécommunications, Institut National de la Recherche Scientifique, 1650 Boul. Lionel Boulet, Varennes, Quebec J3X 1S2, Canada
  • , and 
  • Audrey Moores*
    Audrey Moores
    Centre for Green Chemistry and Catalysis, Department of Chemistry, McGill University, 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada
    Department of Materials Engineering, McGill University, 3610 University Street, Montreal, Quebec H3A 0C5, Canada
    *Audrey Moores E-mail: [email protected]
Cite this: Chem. Rev. 2020, 120, 2, 986–1041
Publication Date (Web):November 14, 2019
https://doi.org/10.1021/acs.chemrev.9b00187
Copyright © 2019 American Chemical Society

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    Abstract

    Abstract Image

    Localized surface plasmon resonance (LSPR) is a physical phenomenon exhibited by nanoparticles of metals including coinage metals, alkali metals, aluminum, and some semiconductors which translates into electromagnetic, thermal, and chemical properties. In the past decade, LSPR has been taken advantage of in the context of catalysis. While plasmonic nanoparticles (PNPs) have been successfully applied toward enhancing catalysis of inorganic reactions such as water splitting, they have also demonstrated exciting performance in the catalysis of organic transformations with potential applications in synthesis of molecules from commodity to pharmaceutical compounds. The advantages of this approach include improved selectivity, enhanced reaction rates, and milder reaction conditions. This review provides the basics of LSPR theory, details the mechanisms at play in plasmon-enhanced nanocatalysis, sheds light onto such nanocatalyst design, and finally systematically presents the breadth of organic reactions hence catalyzed.

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