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    Organic Flow Batteries: Recent Progress and Perspectives
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    • Jianyu Cao
      Jianyu Cao
      Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China
      More by Jianyu Cao
      Orcidhttp://orcid.org/0000-0003-2716-7663
    • Junya Tian
      Junya Tian
      Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China
      More by Junya Tian
    • Juan Xu*
      Juan Xu
      Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology, School of Petrochemical Engineering, Changzhou University, Changzhou 213164, China
      *(J.X.) Email: [email protected]
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    • Yonggang Wang*
      Yonggang Wang
      Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials, Institute of New Energy, iChEM (Collaborative Innovation Centre of Chemistry for Energy Materials), Fudan University, Shanghai 200433, China
      *(Y.W.) Email: [email protected]
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      Orcidhttp://orcid.org/0000-0002-2447-4679
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    Energy & Fuels

    Cite this: Energy Fuels 2020, 34, 11, 13384–13411
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    https://doi.org/10.1021/acs.energyfuels.0c02855
    Published October 20, 2020
    Copyright © 2020 American Chemical Society
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    Abstract

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    As a necessary supplement to clean renewable energy, aqueous flow batteries have become one of the most promising next-generation energy storage and conversion devices because of their excellent safety, high efficiency, flexibility, low cost, and particular capability of being scaled severally in light of energy and power density. The water-soluble redox-active electrolytes are the core components of aqueous flow batteries. The redox-active organic molecules have leaped to the more important electrolytes than conventional inorganic species because of their structural diversity, tailorability, and potential low cost. Much research work was conducted on organic electrolytes for designing high-performance aqueous flow batteries. The motivation of this review is to summarize and present the structure features, property evaluation methods, performance improvement schemes and battery design principles. The detailed functionalization methods to improve the physical and chemical performances of organic electrolytes including redox potential, reaction kinetic rate, solubility, and permeability have been emphatically provided and analyzed. Meanwhile, the further development prospect of aqueous organic electrolytes was put forward.

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    Cite this: Energy Fuels 2020, 34, 11, 13384–13411
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    https://doi.org/10.1021/acs.energyfuels.0c02855
    Published October 20, 2020
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