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Higher Fine Particle Fraction in Sediment Increased Phosphorus Flux to Estuary in Restored Yellow River Basin

  • Yidi Wang
    Yidi Wang
    School of Environment, State Key Laboratory of Water Environment Simulation, Beijing Normal University, Beijing 100875, P.R. China
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  • Wei Ouyang*
    Wei Ouyang
    School of Environment, State Key Laboratory of Water Environment Simulation, Beijing Normal University, Beijing 100875, P.R. China
    *Email: [email protected]. Phone: +86 10 58804585. Fax: +86 10 58804585.
    More by Wei Ouyang
  • Chunye Lin
    Chunye Lin
    School of Environment, State Key Laboratory of Water Environment Simulation, Beijing Normal University, Beijing 100875, P.R. China
    More by Chunye Lin
  • Weihong Zhu
    Weihong Zhu
    School of Geography and Ocean Science, Changbai Mountain Key Laboratory of Biological Resources and Functional Molecules, Yanbian University, Yanji 133003, P.R. China
    More by Weihong Zhu
  • Andrea Critto
    Andrea Critto
    Department of Environmental Sciences, Informatics and Statistics, University Ca’ Foscari Venice, Venice I-30170, Italy
  • Mats Tysklind
    Mats Tysklind
    Department of Chemistry, Umeå University, Umeå SE-901 87, Sweden
  • Xuelei Wang
    Xuelei Wang
    Satellite Environment Center, Ministry of Ecology and Environment, Beijing 100094, P.R. China
    More by Xuelei Wang
  • Mengchang He
    Mengchang He
    School of Environment, State Key Laboratory of Water Environment Simulation, Beijing Normal University, Beijing 100875, P.R. China
    More by Mengchang He
  • Baodong Wang
    Baodong Wang
    First Institute of Oceanography, Ministry of Natural Resources, 6 Xianxialing Road, Qingdao 266061, P.R. China
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  • , and 
  • Haotian Wu
    Haotian Wu
    School of Environment, State Key Laboratory of Water Environment Simulation, Beijing Normal University, Beijing 100875, P.R. China
    More by Haotian Wu
Cite this: Environ. Sci. Technol. 2021, 55, 10, 6783–6790
Publication Date (Web):May 4, 2021
https://doi.org/10.1021/acs.est.1c00135
Copyright © 2021 American Chemical Society

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    Abstract

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    River delta-front estuaries (DEs) are vital interfaces for fluxes between terrestrial and marine environments. However, deep uncertainty exists in estimating the sedimentary pollutant flux from terrestrial environments in DEs due, in part, to a lack of direct measurements in these dynamic and complicated regions and uncertainty in the calculation method. Due to its high sediment content, the Yellow River (YR) has a strong ability to adsorb phosphorus; therefore, it reliably reflects estuarine sedimentary processes. Here, through the comprehensive analysis of field samples, monitoring data and remote sensing images, we conclude that riverine fine particles control the deltaic estuary pollution status and that particle size is the key factor. Based on the stable relationships between phosphorus and heavy metals, with r2 values of 0.990, 0.992, and 0.639 for As, Cd, and Cr, respectively, we estimated that the P flux reached 22.68 g/m2 yr in 2017. Analysis of the YR high-silt sediment load, which has a strong phosphorus adsorption ability and constitutes a substantial fraction of global fluvial sediment transport, revealed a negative correlation between the riverine sediment load and the estuarine phosphorus flux.

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.est.1c00135.

    • CRS model; MFA and RDA methods; sediment sampling, analysis, and related equipment information; and correlation analysis between P, Fe, and Mn in the B2 core (n = 22) (PDF)

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