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Investigation of Plant-Level Volatile Organic Compound Emissions from Chemical Industry Highlights the Importance of Differentiated Control in China
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    Investigation of Plant-Level Volatile Organic Compound Emissions from Chemical Industry Highlights the Importance of Differentiated Control in China
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    • Jinling He
      Jinling He
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      More by Jinling He
    • Huizhong Shen*
      Huizhong Shen
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      *Email: [email protected]
    • Tianyang Lei
      Tianyang Lei
      Department of Earth System Sciences, Tsinghua University, Beijing 100080, China
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    • Yilin Chen
      Yilin Chen
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      School of Urban Planning and Design, Shenzhen Graduate School, Peking University, Shenzhen 518055, China
      More by Yilin Chen
    • Jing Meng
      Jing Meng
      The Bartlett School of Sustainable Construction, University College London, London WC1E 7HB, U.K.
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    • Haitong Sun
      Haitong Sun
      Yusuf Hamied Department of Chemistry, University of Cambridge, Cambridge CB2 1 EW, U.K.
      Centre for Sustainable Medicine, Yong Loo Lin School of Medicine, National University of Singapore, Singapore 117609, Republic of Singapore
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    • Mei Li
      Mei Li
      Institute of Mass Spectrometry and Atmospheric Environment, Guangdong Provincial Engineering Research Center for On-line Source Apportionment System of Air Pollution, Jinan University, Guangzhou 510632, China
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    • Chen Wang
      Chen Wang
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      More by Chen Wang
    • Jianhuai Ye
      Jianhuai Ye
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      More by Jianhuai Ye
    • Lei Zhu
      Lei Zhu
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      More by Lei Zhu
    • Zhihua Zhou
      Zhihua Zhou
      Shenzhen Ecological and Environmental Monitoring Center of Guangdong Province, Shenzhen 518055, China
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    • Guofeng Shen
      Guofeng Shen
      College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
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    • Dabo Guan
      Dabo Guan
      Department of Earth System Sciences, Tsinghua University, Beijing 100080, China
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    • Tzung-May Fu
      Tzung-May Fu
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      More by Tzung-May Fu
    • Xin Yang
      Xin Yang
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      More by Xin Yang
    • Shu Tao
      Shu Tao
      Guangdong Provincial Observation and Research Station for Coastal Atmosphere and Climate of the Greater Bay Area, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      Shenzhen Key Laboratory of Precision Measurement and Early Warning Technology for Urban Environmental Health Risks, School of Environmental Science and Engineering, Southern University of Science and Technology, Shenzhen 518055, China
      College of Urban and Environmental Sciences, Peking University, Beijing 100871, China
      Institute of Carbon Neutrality, Peking University, Beijing 100871, China
      More by Shu Tao
    Other Access OptionsSupporting Information (2)

    Environmental Science & Technology

    Cite this: Environ. Sci. Technol. 2023, 57, 50, 21295–21305
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    https://doi.org/10.1021/acs.est.3c08570
    Published December 8, 2023
    Copyright © 2023 American Chemical Society

    Abstract

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    The chemical industry is a significant source of nonmethane volatile organic compounds (NMVOCs), pivotal precursors to ambient ozone (O3), and secondary organic aerosol (SOA). Despite their importance, precise estimation of these emissions remains challenging, impeding the implementation of NMVOC controls. Here, we present the first comprehensive plant-level assessment of NMVOC emissions from the chemical industry in China, encompassing 3461 plants, 127 products, and 50 NMVOC compounds from 2010 to 2019. Our findings revealed that the chemical industry in China emitted a total of 3105 (interquartile range: 1179–8113) Gg of NMVOCs in 2019, with a few specific products accounting for the majority of the emissions. Generally, plants engaged in chemical fibers production or situated in eastern China pose a greater risk to public health due to their higher formation potentials of O3 and SOA or their proximity to residential areas or both. We demonstrated that targeting these high-risk plants for emission reduction could enhance health benefits by 7–37% per unit of emission reduction on average compared to the current situation. Consequently, this study provides essential insights for developing effective plant-specific NMVOC control strategies within China’s chemical industry.

    Copyright © 2023 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.est.3c08570.

    • Emission factors adopted in this study, provincial-level emission estimates, and comparisons with previous studies (PDF)

    • Estimated emissions and health impact potentials of the top 5% plants with the highest HPO3, HPSOA, and HPTOX (XLSX)

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    This article is cited by 2 publications.

    1. Hanyang Man, Xiaohan Shao, Wenying Cai, Kai Wang, Zhitao Cai, Ming Xue, Huan Liu. Utilizing a optimized method for evaluating vapor recovery equipment control efficiency and estimating evaporative VOC emissions from urban oil depots via an extensive survey. Journal of Hazardous Materials 2024, 479 , 135710. https://doi.org/10.1016/j.jhazmat.2024.135710
    2. Xuan Yang, Cuncun Duan, Bin Chen, Saige Wang. Does stricter sewage treatment targets policy exacerbate the contradiction between effluent water quality improvement and carbon emissions mitigation? An evidence from China. Global Environmental Change 2024, 87 , 102881. https://doi.org/10.1016/j.gloenvcha.2024.102881

    Environmental Science & Technology

    Cite this: Environ. Sci. Technol. 2023, 57, 50, 21295–21305
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.est.3c08570
    Published December 8, 2023
    Copyright © 2023 American Chemical Society

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