Influence of Methane Emissions and Vehicle Efficiency on the Climate Implications of Heavy-Duty Natural Gas TrucksClick to copy article linkArticle link copied!
Abstract
While natural gas produces lower carbon dioxide emissions than diesel during combustion, if enough methane is emitted across the fuel cycle, then switching a heavy-duty truck fleet from diesel to natural gas can produce net climate damages (more radiative forcing) for decades. Using the Technology Warming Potential methodology, we assess the climate implications of a diesel to natural gas switch in heavy-duty trucks. We consider spark ignition (SI) and high-pressure direct injection (HPDI) natural gas engines and compressed and liquefied natural gas. Given uncertainty surrounding several key assumptions and the potential for technology to evolve, results are evaluated for a range of inputs for well-to-pump natural gas loss rates, vehicle efficiency, and pump-to-wheels (in-use) methane emissions. Using reference case assumptions reflecting currently available data, we find that converting heavy-duty truck fleets leads to damages to the climate for several decades: around 70–90 years for the SI cases, and 50 years for the more efficient HPDI. Our range of results indicates that these fuel switches have the potential to produce climate benefits on all time frames, but combinations of significant well-to-wheels methane emissions reductions and natural gas vehicle efficiency improvements would be required.
Introduction
Methods
Results
Discussion
Supporting Information
Further methodological details and results. This material is available free of charge via the Internet at ACS Publications website at DOI: 10.1021/acs.est.5b00412.
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Acknowledgment
For helpful comments and discussions, we thank Andrew Burnham, Steve Hamburg, Klaus Lackner, Michael Levi, Jason Mathers, Christoph Meinrenken, Joe Rudek, and James Winebrake. All remaining errors are our own. This work was partially supported by the Robertson Foundation.
References
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- 1Fuel Competition in Power Generation and Elasticities of Substitution; Energy Information Administration, U.S. Department of Energy: Washington, DC, 2012.There is no corresponding record for this reference.
- 2Alvarez, R. A.; Pacala, S. W.; Winebrake, J. J.; Chameides, W. L.; Hamburg, S. P. Greater Focus Needed on Methane Leakage from Natural Gas Infrastructure Proc. Natl. Acad. Sci. U.S.A. 2012, 109 (17) 6435– 64402https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC38Xmslyjt78%253D&md5=cc313105cb8d7918515e42c622dfe956Greater focus needed on methane leakage from natural gas infrastructureAlvarez, Ramon A.; Pacala, Stephen W.; Winebrake, James J.; Chameides, William L.; Hamburg, Steven P.Proceedings of the National Academy of Sciences of the United States of America (2012), 109 (17), 6435-6440, S6435/1-S6435/7CODEN: PNASA6; ISSN:0027-8424. (National Academy of Sciences)Natural gas is seen by many as the future of American energy: a fuel that can provide energy independence and reduce greenhouse gas emissions in the process. However, there has also been confusion about the climate implications of increased use of natural gas for elec. power and transportation. We propose and illustrate the use of technol. warming potentials as a robust and transparent way to compare the cumulative radiative forcing created by alternative technologies fueled by natural gas and oil or coal by using the best available ests. of greenhouse gas emissions from each fuel cycle (i.e., prodn., transportation and use). We find that a shift to compressed natural gas vehicles from gasoline or diesel vehicles leads to greater radiative forcing of the climate for 80 or 280 yr, resp., before beginning to produce benefits. Compressed natural gas vehicles could produce climate benefits on all time frames if the well-to-wheels CH4 leakage were capped at a level 45-70% below current ests. By contrast, using natural gas instead of coal for elec. power plants can reduce radiative forcing immediately, and reducing CH4 losses from the prodn. and transportation of natural gas would produce even greater benefits. There is a need for the natural gas industry and science community to help obtain better emissions data and for increased efforts to reduce methane leakage in order to minimize the climate footprint of natural gas.
- 3Howarth, R. W.; Santoro, R.; Ingraffea, A. CH4 and the Greenhouse-Gas Footprint of Natural Gas from Shale Formations Clim. Chang. 2011, 106 (4) 679– 6903https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC3MXlslKitrY%253D&md5=c9560e099a6d1300153d8a9d533bc8e2Methane and the greenhouse-gas footprint of natural gas from shale formationsHowarth, Robert W.; Santoro, Renee; Ingraffea, AnthonyClimatic Change (2011), 106 (4), 679-690CODEN: CLCHDX; ISSN:0165-0009. (Springer)We evaluate the greenhouse gas footprint of natural gas obtained by high-vol. hydraulic fracturing from shale formations, focusing on methane emissions. Natural gas is composed largely of methane, and 3.6% to 7.9% of the methane from shale-gas prodn. escapes to the atm. in venting and leaks over the life-time of a well. These methane emissions are at least 30% more than and perhaps more than twice as great as those from conventional gas. The higher emissions from shale gas occur at the time wells are hydraulically fractured-as methane escapes from flow-back return fluids-and during drill out following the fracturing. Methane is a powerful greenhouse gas, with a global warming potential that is far greater than that of carbon dioxide, particularly over the time horizon of the first few decades following emission. Methane contributes substantially to the greenhouse gas footprint of shale gas on shorter time scales, dominating it on a 20-yr time horizon. The footprint for shale gas is greater than that for conventional gas or oil when viewed on any time horizon, but particularly so over 20 years. Compared to coal, the footprint of shale gas is at least 20% greater and perhaps more than twice as great on the 20-yr horizon and is comparable when compared over 100 years.
- 4Myhrvold, N. P.; Caldeira, K. Greenhouse Gases, Climate Change and the Transition from Coal to Low-Carbon Electricity Environ. Res. Lett. 2012, 7014019There is no corresponding record for this reference.
- 5Moore, C. W.; Zielinska, B.; Pétron, G.; Jackson, R. B. Air Impacts of Increased Natural Gas Acquisition, Processing, and Use: A Critical Review Environ. Sci. Technol. 2014, 48 (15) 8349– 8359 DOI: 10.1021/es40534725https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC2cXjsVSitr4%253D&md5=71090b083be22e7118fadff76d56f05cAir Impacts of Increased Natural Gas Acquisition, Processing, and Use: A Critical ReviewMoore, Christopher W.; Zielinska, Barbara; Petron, Gabrielle; Jackson, Robert B.Environmental Science & Technology (2014), 48 (15), 8349-8359CODEN: ESTHAG; ISSN:0013-936X. (American Chemical Society)A review concerning the current understanding of local and regional air quality impacts of conventional vs. unconventional natural gas extn., prodn., distribution, and use is given. Over the past 10 yr, US and Canadian technol. advancements led to rapid, intensive development of many unconventional natural gas extn. technologies (e.g., shale gas, tight sand gas, coal-bed CH4), raising concerns about environmental impacts. Topics discussed include: ests. life cycle CH4 leaks from natural gas; air quality impacts of the first 2 life cycle changes (pre-prodn., prodn., and other stages); potential air quality benefits of increased natural gas use; regulations; and recommendations.
- 6Brandt, A. R.; Heath, G. A.; Kort, E. A.; O’Sullivan, F.; Pétron, G.; Jordaan, S. M.; Tans, P.; Wilcox, J.; Gopstein, A. M.; Arent, D. Methane Leaks from North American Natural Gas Systems Science 2014, 343, 733– 735 DOI: 10.1126/science.12470456https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC2cXjvVOiuro%253D&md5=919ddc43ceb2719af54e1d6c4217c995Methane leaks from North American natural gas systemsBrandt, A. R.; Heath, G. A.; Kort, E. A.; O'Sullivan, F.; Petron, G.; Jodraan, S. M.; Tans, P.; Wilcox, J.; Gopstein, A. M.; Arent, D.; Wofsy, S.; Brown, N. J.; Bradley, R.; Stucky, G. D.; Eardley, D.; Harriss, R.Science (Washington, DC, United States) (2014), 343 (6172), 733-735CODEN: SCIEAS; ISSN:0036-8075. (American Association for the Advancement of Science)There is no expanded citation for this reference.
- 7Karion, A.; Sweeney, C.; Pétron, G.; Frost, G.; Hardesty, R. M.; Kofler, J.; Miller, B. R.; Newberger, T.; Wolter, S.; Banta, R. Methane Emissions Estimate from Airborne Measurements over a Western United States Natural Gas Field Geophys. Res. Lett. 2013, 40 (16) 4393– 4397 DOI: 10.1002/grl.508117https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC3sXhsVKgsrvP&md5=05e893c9e2415cd0fde399ce2aa3ac6bMethane emissions estimate from airborne measurements over a western United States natural gas fieldKarion, Anna; Sweeney, Colm; Petron, Gabrielle; Frost, Gregory; Michael Hardesty, R.; Kofler, Jonathan; Miller, Ben R.; Newberger, Tim; Wolter, Sonja; Banta, Robert; Brewer, Alan; Dlugokencky, Ed; Lang, Patricia; Montzka, Stephen A.; Schnell, Russell; Tans, Pieter; Trainer, Michael; Zamora, Robert; Conley, StephenGeophysical Research Letters (2013), 40 (16), 4393-4397CODEN: GPRLAJ; ISSN:1944-8007. (Wiley-Blackwell)Methane (CH4) emissions from natural gas prodn. are not well quantified and have the potential to offset the climate benefits of natural gas over other fossil fuels. We use atm. measurements in a mass balance approach to est. CH4 emissions of 55 ± 15 × 103 kg h-1 from a natural gas and oil prodn. field in Uintah County, Utah, on 1 day: 3 Feb. 2012. This emission rate corresponds to 6.2%-11.7% (1σ) of av. hourly natural gas prodn. in Uintah County in the month of Feb. This study demonstrates the mass balance technique as a valuable tool for estg. emissions from oil and gas prodn. regions and illustrates the need for further atm. measurements to det. the representativeness of our single-day est. and to better assess inventories of CH4 emissions.
- 8Pétron, G.; Karion, A.; Sweeney, C.; Miller, B. R.; Montzka, S. A.; Frost, G.; Trainer, M.; Tans, P.; Andrews, A.; Kofler, J. A New Look at Methane and Non-Methane Hydrocarbon Emissions from Oil and Natural Gas Operations in the Colorado Denver-Julesburg Basin J. Geophys. Res. Atmos. 2014, 119 (11) 6386– 6852 DOI: 10.1002/2013JD021272There is no corresponding record for this reference.
- 9Peischl, J.; Ryerson, T. B.; Aikin, K. C.; de Gouw, J. A.; Gilman, J. B.; Holloway, J. S.; Lerner, B. M.; Nadkarni, R.; Neuman, J. A.; Nowak, J. B. Quantifying Atmospheric Methane Emissions from the Haynesville, Fayetteville, and Northeastern Marcellus Shale Gas Production Regions J. Geophys. Res. Atmos. 2015, 120 (5) 2119– 2139 DOI: 10.1002/2014JD0226979https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC2MXltVWmtL4%253D&md5=1a060b067d6f67778177a0f72fca8920Quantifying atmospheric methane emissions from the Haynesville, Fayetteville, and northeastern Marcellus shale gas production regionsPeischl, J.; Ryerson, T. B.; Aikin, K. C.; de Gouw, J. A.; Gilman, J. B.; Holloway, J. S.; Lerner, B. M.; Nadkarni, R.; Neuman, J. A.; Nowak, J. B.; Trainer, M.; Warneke, C.; Parrish, D. D.Journal of Geophysical Research: Atmospheres (2015), 120 (5), 2119-2139CODEN: JGRDE3; ISSN:2169-8996. (Wiley-Blackwell)We present measurements of methane (CH4) taken aboard a NOAA WP-3D research aircraft in 2013 over the Haynesville shale region in eastern Texas/northwestern Louisiana, the Fayetteville shale region in Arkansas, and the northeastern Pennsylvania portion of the Marcellus shale region, which accounted for the majority of Marcellus shale gas prodn. that year. We calc. emission rates from the horizontal CH4 flux in the planetary boundary layer downwind of each region after subtracting the CH4 flux entering the region upwind. We find 1 day CH4 emissions of (8.0 ± 2.7) × 107 g/h from the Haynesville region, (3.9 ± 1.8) × 107 g/h from the Fayetteville region, and (1.5 ± 0.6) × 107 g/h from the Marcellus region in northeastern Pennsylvania. Finally, we compare the CH4 emissions to the total vol. of natural gas extd. from each region to derive a loss rate from prodn. operations of 1.0-2.1% from the Haynesville region, 1.0-2.8% from the Fayetteville region, and 0.18-0.41% from the Marcellus region in northeastern Pennsylvania. The climate impact of CH4 loss from shale gas prodn. depends upon the total leakage from all prodn. regions. The regions investigated in this work represented over half of the U.S. shale gas prodn. in 2013, and we find generally lower loss rates than those reported in earlier studies of regions that made smaller contributions to total prodn. Hence, the national av. CH4 loss rate from shale gas prodn. may be lower than values extrapolated from the earlier studies.
- 10Schwietzke, S.; Griffin, W. M.; Matthews, H. S.; Bruhwiler, L. M. P. Natural Gas Fugitive Emissions Rates Constrained by Global Atmospheric Methane and Ethane Environ. Sci. Technol. 2014, 48 (14) 7714– 7722 DOI: 10.1021/es501204c10https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC2cXhtVSmu7nJ&md5=497f1e27bea54958a142a1617d8292b0Natural Gas Fugitive Emissions Rates Constrained by Global Atmospheric Methane and EthaneSchwietzke, Stefan; Griffin, W. Michael; Matthews, H. Scott; Bruhwiler, Lori M. P.Environmental Science & Technology (2014), 48 (14), 7714-7722CODEN: ESTHAG; ISSN:0013-936X. (American Chemical Society)The amt. of methane emissions released by the natural gas (NG) industry is a crit. and uncertain value for various industry and policy decisions, such as for detg. the climate implications of using NG over coal. Previous studies have estd. fugitive emissions rates (FER)-the fraction of produced NG (mainly methane and ethane) escaped to the atm.-between 1 and 9%. Most of these studies rely on few and outdated measurements, and some may represent only temporal/regional NG industry snapshots. This study ests. NG industry representative FER using global atm. methane and ethane measurements over three decades, and literature ranges of (i) tracer gas atm. lifetimes, (ii) non-NG source ests., and (iii) fossil fuel fugitive gas hydrocarbon compns. The modeling suggests an upper bound global av. FER of 5% during 2006-2011, and a most likely FER of 2-4% since 2000, trending downward. These results do not account for highly uncertain natural hydrocarbon seepage, which could lower the FER. Further emissions redns. by the NG industry may be needed to ensure climate benefits over coal during the next few decades.
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- 23Meyer, P. E.; Green, E. H.; Corbett, J. J.; Mas, C.; Winebrake, J. J. Total fuel-cycle analysis of heavy-duty vehicles using biofuels and natural gas-based alternative fuels J. Air Waste Manage. Assoc. 2011, 61, 285– 29423https://chemport.cas.org/services/resolver?origin=ACS&resolution=options&coi=1%3ACAS%3A528%3ADC%252BC3MXktFant78%253D&md5=6723120d19f3516bdf0b078e81f93f7cTotal fuel-cycle analysis of heavy-duty vehicles using biofuels and natural gas-based alternative fuelsMeyer, Patrick E.; Green, Erin H.; Corbett, James J.; Mas, Carl; Winebrake, James J.Journal of the Air & Waste Management Association (2011), 61 (3), 285-294CODEN: JAWAFC; ISSN:1096-2247. (Air & Waste Management Association)Heavy-duty vehicles (HDVs) present a growing energy and environmental concern worldwide. These vehicles rely almost entirely on diesel fuel for propulsion and create problems assocd. with local pollution, climate change, and energy security. Given these problems and the expected global expansion of HDVs in transportation sectors, industry and governments are pursuing biofuels and natural gas as potential alternative fuels for HDVs. Using recent lifecycle datasets, this paper evaluates the energy and emissions impacts of these fuels in the HDV sector by conducting a total fuel-cycle (TFC) anal. for Class 8 HDVs for six fuel pathways: (1) petroleum to ultra low sulfur diesel; (2) petroleum and soyoil to biodiesel (Me soy ester); (3) petroleum, ethanol, and oxygenate to e-diesel; (4) petroleum and natural gas to Fischer-Tropsch diesel; (5) natural gas to compressed natural gas; and (6) natural gas to liquefied natural gas. TFC emissions are evaluated for three greenhouse gases (GHGs) (carbon dioxide, nitrous oxide, and methane) and five other pollutants (volatile org. compds., carbon monoxide, nitrogen oxides, particulate matter, and sulfur oxides), along with ests. of total energy and petroleum consumption assocd. with each of the six fuel pathways. Results show definite advantages with biodiesel and compressed natural gas for most pollutants, negligible benefits for e-diesel, and increased GHG emissions for liquefied natural gas and Fischer-Tropsch diesel (from natural gas).
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