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Investigation of Mass Transfer Characteristics of SO2 Absorption into NaOH in a Multichannel Ceramic Membrane Contactor

  • Xiangli Kong
    Xiangli Kong
    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No.30 South Puzhu Road, Nanjing 211816, P.R. China
    More by Xiangli Kong
  • Dawei Gong
    Dawei Gong
    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No.30 South Puzhu Road, Nanjing 211816, P.R. China
    More by Dawei Gong
  • Wei Ke
    Wei Ke
    Nanjing Membrane Industrial Technology Research Institute Co., Ltd, No.1 Yuansi Road, Nanjing 211800, P.R. China
    More by Wei Ke
  • Minghui Qiu
    Minghui Qiu
    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No.30 South Puzhu Road, Nanjing 211816, P.R. China
    More by Minghui Qiu
  • Kaiyun Fu
    Kaiyun Fu
    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No.30 South Puzhu Road, Nanjing 211816, P.R. China
    More by Kaiyun Fu
  • Peng Xu
    Peng Xu
    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No.30 South Puzhu Road, Nanjing 211816, P.R. China
    More by Peng Xu
  • Xianfu Chen
    Xianfu Chen
    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No.30 South Puzhu Road, Nanjing 211816, P.R. China
    More by Xianfu Chen
  • , and 
  • Yiqun Fan*
    Yiqun Fan
    State Key Laboratory of Materials-Oriented Chemical Engineering, College of Chemical Engineering, Nanjing Tech University, No.30 South Puzhu Road, Nanjing 211816, P.R. China
    *Email: [email protected]. Phone: +86 25 83172277. Fax: +86 25 83172292.
    More by Yiqun Fan
Cite this: Ind. Eng. Chem. Res. 2020, 59, 23, 11054–11062
Publication Date (Web):May 22, 2020
https://doi.org/10.1021/acs.iecr.0c01327
Copyright © 2020 American Chemical Society

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    Abstract

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    A ceramic membrane with multichannels generally has a higher specific area and larger throughput compared to that with a single channel, which is beneficial to the industrialization of ceramic membrane contactors for SO2 absorption. In this work, the mass transfer performance of SO2 absorption into NaOH solution was investigated at various gas and liquid operating conditions in a membrane contactor packed with a 19-channel hydrophilic membrane. The results showed that increasing the NaOH concentration can offset the effect of membrane thickness. To analyze the mass transfer process, a 3D mass transfer model was developed to simulate the concentration distribution of the components. The simulated SO2 fluxes were consistent with the experimental results. Additionally, the mass transfer model was applied to optimize the structure of channels in multichannel ceramic membranes. The operational mode of the multichannel ceramic membrane is optimized by blocking some inside channels to reduce the mass transfer resistance.

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