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Improving the Efficiency of Mn-CeOx/Cordierite Catalysts for Nonmethane Hydrocarbon Oxidation in Cooking Oil Fumes

  • Honghong Yi
    Honghong Yi
    Department of Environmental Engineering, School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
    Beijing Key Laboratory of Resource-oriented Treatment of Industrial Pollutants, Beijing 100083, P. R. China
    More by Honghong Yi
  • Yonghai Huang
    Yonghai Huang
    Department of Environmental Engineering, School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
  • Xiaolong Tang*
    Xiaolong Tang
    Department of Environmental Engineering, School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
    Beijing Key Laboratory of Resource-oriented Treatment of Industrial Pollutants, Beijing 100083, P. R. China
    *Tel./Fax:+86 010 62332747. E-mail: [email protected]
  • Shunzheng Zhao
    Shunzheng Zhao
    Department of Environmental Engineering, School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
    Beijing Key Laboratory of Resource-oriented Treatment of Industrial Pollutants, Beijing 100083, P. R. China
  • Fengyu Gao
    Fengyu Gao
    Department of Environmental Engineering, School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
    More by Fengyu Gao
  • Jiangen Wang
    Jiangen Wang
    Department of Environmental Engineering, School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
    More by Jiangen Wang
  • , and 
  • Zhongyu Yang
    Zhongyu Yang
    Department of Environmental Engineering, School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, P. R. China
    More by Zhongyu Yang
Cite this: Ind. Eng. Chem. Res. 2018, 57, 12, 4186–4194
Publication Date (Web):March 7, 2018
https://doi.org/10.1021/acs.iecr.7b04904
Copyright © 2018 American Chemical Society

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    Abstract

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    Cooking oil fumes (COFs) are considered to be one of the important pollution sources in urban areas, and nonmethane hydrocarbon (NMHC) can be an index of volatile organic compounds (VOCs) from COFs. In this paper, cordierite supported Mn-CeOx catalysts were used for NMHC oxidation in COFs. The results showed that the catalytic oxidation activity of Mn-CeOx/cordierite was obviously improved by adding an appropriate proportion of Ce. The catalytic activity of Mn4Ce1/C was obviously better than catalysts with other molar ratios of Mn/Ce and Mn/C because of the extra adsorbed oxygen species and high ratio of Ce4+/Ce3+ according to the XPS analysis. The physisorption of N2 and SEM-EDS revealed that the structure of catalysts prepared by a sol–gel method presented a higher BET specific surface area, more abundant pore structure, and better dispersion of catalysts’ active components which were favorable for catalytic oxidation reaction of NMHC.

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    Cited By

    This article is cited by 12 publications.

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    2. Siyu Zhang, Xinjun Shen, Lixiang Zhu, Jing Zhang. Study on degradation of cooking fume by compound filter material and UV photodegradation. Environmental Science and Pollution Research 2023, 30 (27) , 70649-70660. https://doi.org/10.1007/s11356-023-27491-3
    3. Yuanyuan Zhang, Qingjun Yu, Xiaolong Tang, Shunzheng Zhao, Fengyu Gao, Yuting Yuan, Jie Zhang, Jinghui Wei, Honghong Yi. Reduction of non-methane hydrocarbons in cooking oil fumes via adsorption on MFI: Effect of zeolitic framework composition. Separation and Purification Technology 2022, 300 , 121687. https://doi.org/10.1016/j.seppur.2022.121687
    4. Caiqing He, Yunnen Chen, Lin Guo, Ruoyu Yin, Tingsheng Qiu. Catalytic ozonation of NH4+-N in wastewater over composite metal oxide catalyst. Journal of Rare Earths 2022, 40 (1) , 73-84. https://doi.org/10.1016/j.jre.2020.11.003
    5. Yuanyuan Zhang, Qingjun Yu, Xiaolong Tang, Shunzheng Zhao, Fengyu Gao, Yuting Yuan, Jie Zhang, Jinghui Wei, Honghong Yi. Reduction of Nmhc in Cooking Oil Fumes Via Adsorption on Mfi: Effect of Zeolitic Framework Composition. SSRN Electronic Journal 2022, 145 https://doi.org/10.2139/ssrn.4118425
    6. Jian Li, Yingjie Shi, Xiaoheng Fu, Yun Shu, Jiayu Huang, Jinwei Zhu, Gang Tian, Jingnan Hu. Effects of Ni substitution on active oxygen species and electronic interactions over La0.8Ce0.2MnO3/mesoporous ZSM-5 for oxidizing C6H14. Molecular Catalysis 2021, 499 , 111309. https://doi.org/10.1016/j.mcat.2020.111309
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    8. Yu-An Ho, Shan-Yu Wang, Wei-Hung Chiang, Van-Huy Nguyen, Jun-Long Chiu, Jeffrey C.S. Wu. Moderate-temperature catalytic incineration of cooking oil fumes using hydrophobic honeycomb supported Pt/CNT catalyst. Journal of Hazardous Materials 2019, 379 , 120750. https://doi.org/10.1016/j.jhazmat.2019.120750
    9. Jian Li, Yingjie Shi, Xiaoheng Fu, Jiayu Huang, Yanping Zhang, Shuang Deng, Fan Zhang. Hierarchical ZSM-5 based on fly ash for the low-temperature purification of odorous volatile organic compound in cooking fumes. Reaction Kinetics, Mechanisms and Catalysis 2019, 128 (1) , 289-314. https://doi.org/10.1007/s11144-019-01633-6
    10. Zhaxi Cuo, Dongdong Wang, Yan Gong, Feng Zhao, Haidi Liu, Yunfa Chen. A Novel Porous Ceramic Membrane Supported Monolithic Cu-Doped Mn–Ce Catalysts for Benzene Combustion. Catalysts 2019, 9 (8) , 652. https://doi.org/10.3390/catal9080652
    11. Honghong Yi, Yonghai Huang, Xiaolong Tang, Shunzheng Zhao, Fengyu Gao, Xizhou Xie, Jiangen Wang, Zhongyu Yang. Mn-CeOx/MeOx(Ti, Al)/cordierite preparation with ultrasound-assisted for non-methane hydrocarbon removal from cooking oil fumes. Ultrasonics Sonochemistry 2019, 53 , 126-133. https://doi.org/10.1016/j.ultsonch.2018.12.043
    12. Honghong Yi, Yonghai Huang, Xiaolong Tang, Shunzheng Zhao, Fengyu Gao, Xizhou Xie, Jiangen Wang, Zhongyu Yang. Synthesis of Mn-CeOx/cordierite catalysts using various coating materials and pore-forming agents for non-methane hydrocarbon oxidation in cooking oil fumes. Ceramics International 2018, 44 (13) , 15472-15477. https://doi.org/10.1016/j.ceramint.2018.05.203

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