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Power-to-Gas through High Temperature Electrolysis and Carbon Dioxide Methanation: Reactor Design and Process Modeling

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Download Hi-Res ImageDownload to MS-PowerPointCite This:Ind. Eng. Chem. Res. 2018, 57, 11, 4007-4018
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    Power-to-Gas through High Temperature Electrolysis and Carbon Dioxide Methanation: Reactor Design and Process Modeling
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    • Emanuele Giglio
      Emanuele Giglio
      Department of Applied Science and Technology (DISAT), Politecnico di Torino, Corso Duca degli Abruzzi 24, 10129 Torino, Italy
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    • Fabio Alessandro Deorsola
      Fabio Alessandro Deorsola
      Department of Applied Science and Technology (DISAT), Politecnico di Torino, Corso Duca degli Abruzzi 24, 10129 Torino, Italy
      More by Fabio Alessandro Deorsola
    • Manuel Gruber
      Manuel Gruber
      Engler-Bunte-Institute, Division of Combustion Technology, Karlsruhe Institute of Technology, Engler-Bunte-Ring 7, 76131 Karlsruhe, Germany
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    • Stefan Raphael Harth
      Stefan Raphael Harth
      Engler-Bunte-Institute, Division of Combustion Technology, Karlsruhe Institute of Technology, Engler-Bunte-Ring 7, 76131 Karlsruhe, Germany
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    • Eduard Alexandru Morosanu
      Eduard Alexandru Morosanu
      Department of Applied Science and Technology (DISAT), Politecnico di Torino, Corso Duca degli Abruzzi 24, 10129 Torino, Italy
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    • Dimosthenis Trimis
      Dimosthenis Trimis
      Engler-Bunte-Institute, Division of Combustion Technology, Karlsruhe Institute of Technology, Engler-Bunte-Ring 7, 76131 Karlsruhe, Germany
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    • Samir Bensaid*
      Samir Bensaid
      Department of Applied Science and Technology (DISAT), Politecnico di Torino, Corso Duca degli Abruzzi 24, 10129 Torino, Italy
      *E-mail: [email protected]
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      Orcidhttp://orcid.org/0000-0001-9634-266X
    • Raffaele Pirone
      Raffaele Pirone
      Department of Applied Science and Technology (DISAT), Politecnico di Torino, Corso Duca degli Abruzzi 24, 10129 Torino, Italy
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    Industrial & Engineering Chemistry Research

    Cite this: Ind. Eng. Chem. Res. 2018, 57, 11, 4007–4018
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    https://doi.org/10.1021/acs.iecr.8b00477
    Published March 7, 2018
    Copyright © 2018 American Chemical Society
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    Abstract

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    This work deals with the coupling between high temperature steam electrolysis using solid oxide cells (SOEC) and carbon dioxide methanation to produce a synthetic natural gas (SNG) directly injectable in the natural gas distribution grid via a power-to-gas (P2G) pathway. An intrinsic kinetics obtained from the open literature has been used as the basis for a plug flow reactor model applied to a series of cooled multitube fixed bed reactors for methane synthesis. Evaporating water has been considered as coolant, ensuring a high heat transfer coefficient within the shell side of the reactor. A methanation section has been designed and optimized in order to moderate the maximum temperature within the catalytic bed and to minimize the catalyst load. Then, process modeling of a plant coupling high temperature electrolysis and methanation is presented: the main goal of this analysis is the calculation of overall plant efficiency (in terms of electricity-to-SNG chemical energy). Plant size has been set considering a 10 MWel SOEC-based electrolysis unit; heat produced from the exothermal methanation is entirely used for water evaporation before the steam electrolysis. A heat exchanger network (HEN) has been designed in order to reduce the number of components, resulting in an external heat requirement equal to 185 kW (≈1.9% of the electrolysis power). The SOEC-based power-to-gas system presented a higher heating value based efficiency equal to ≈86% (≈77% if evaluated on lower heating value basis).

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.iecr.8b00477.

    • Description of the kinetic model used in this work, including Table S1 and eqs S1–S3 (PDF)

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    Cite this: Ind. Eng. Chem. Res. 2018, 57, 11, 4007–4018
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