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Investigation of Thermodynamic Properties on CO2 Absorbents Blended with Ammonia, Amino Acids, and Corrosion Inhibitors at 313.15, 333.15, and 353.15 K

  • Yunsung Yoo
    Yunsung Yoo
    Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul 03722, Republic of Korea
    More by Yunsung Yoo
  • Dongwoo Kang
    Dongwoo Kang
    Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul 03722, Republic of Korea
    More by Dongwoo Kang
  • Injun Kim
    Injun Kim
    Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul 03722, Republic of Korea
    More by Injun Kim
  • , and 
  • Jinwon Park*
    Jinwon Park
    Department of Chemical and Biomolecular Engineering, Yonsei University, 50 Yonsei-ro, Seodaemun-gu, Seoul 03722, Republic of Korea
    *(J.P.) E-mail: [email protected]. Tel: +82 2-364-1807.
    More by Jinwon Park
Cite this: J. Chem. Eng. Data 2018, 63, 8, 2856–2867
Publication Date (Web):July 20, 2018
https://doi.org/10.1021/acs.jced.8b00175
Copyright © 2018 American Chemical Society

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    Abstract

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    The wet absorption method is currently one of the key technologies employed for the capture of carbon dioxide. In this method, the selection of an optimal absorbent is of particular importance. As such, we herein propose a series of novel and efficient absorbents based on a 7 wt % NH3 solution containing 3 wt % amino acid (β-alanine or l-arginine) and 1 wt % corrosion inhibitor (imidazole or 1,2,3-benzotriazole). To investigate the thermodynamic properties including density, viscosity, diffusivity of CO2, kinetic constant, rate equation, and physical and chemical CO2 solubility data on capturing carbon dioxide in these absorbents, various experiments were conducted on each absorbent at 313.15, 333.15, and 353.15 K. All of the proposed absorbents showed better capacity than monoethanolamine which has been most widely used as a wet absorbent. Among them, the absorbents with added l-arginine were found to be superior to absorbents with added β-alanine.

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