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Review and Analysis of Thermophysical Properties of a Sulfuric Acid–Water Electrolyte
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    Review and Analysis of Thermophysical Properties of a Sulfuric Acid–Water Electrolyte
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    Journal of Chemical & Engineering Data

    Cite this: J. Chem. Eng. Data 2018, 63, 9, 3572–3583
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    https://doi.org/10.1021/acs.jced.8b00466
    Published September 4, 2018
    Copyright © 2018 American Chemical Society

    Abstract

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    In this work, we have performed a critical review of the thermophysical properties of sulfuric acid–water mixtures. The thermophysical properties analyzed are density, viscosity, refraction index, thermal expansion coefficient, and mass expansion coefficient. The density of the sulfuric acid–water mixture has been measured for different mass fractions (w = 0.1–0.4) over a broad temperature range (T = 273.15–333.15 K). A new parametrization of the density has been performed using a least-squares method. In this parametrization, the number of coefficients has been reduced with respect to previous works. Moreover, this new equation has been analyzed in an extended region of temperature and concentration in the following ranges: w = 0–0.1, T = (233.15–373.15 K). The coefficients of thermal and mass expansion have also been calculated experimentally, and a linear relation of the density has been determined as a function of the variations in temperature and concentration. In addition, viscosity and refraction index measurements have been performed at 298.15 and 293.15 K, respectively. Our results have been checked against measurements in the literature (review) and show good correspondence.

    Copyright © 2018 American Chemical Society

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    Cited By

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    This article is cited by 5 publications.

    1. J. David Bazak, Allison R. Wong, Kaining Duanmu, Kee Sung Han, David Reed, Vijayakumar Murugesan. Concentration-Dependent Solvation Structure and Dynamics of Aqueous Sulfuric Acid Using Multinuclear NMR and DFT. The Journal of Physical Chemistry B 2021, 125 (19) , 5089-5099. https://doi.org/10.1021/acs.jpcb.1c01177
    2. Elizabeth Asher, Alexandre Baron, Pengfei Yu, Michael Todt, Penny Smale, Ben Liley, Richard Querel, Tetsu Sakai, Isamu Morino, Yoshitaka Jin, Tomohiro Nagai, Osamu Uchino, Emrys Hall, Patrick Cullis, Bryan Johnson, Troy D. Thornberry. Balloon Baseline Stratospheric Aerosol Profiles (B 2 SAP)—Perturbations in the Southern Hemisphere, 2019–2022. Journal of Geophysical Research: Atmospheres 2024, 129 (22) https://doi.org/10.1029/2024JD041581
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    4. Manuel Baumgartner, Christian Rolf, Jens-Uwe Grooß, Julia Schneider, Tobias Schorr, Ottmar Möhler, Peter Spichtinger, Martina Krämer. New investigations on homogeneous ice nucleation: the effects of water activity and water saturation formulations. Atmospheric Chemistry and Physics 2022, 22 (1) , 65-91. https://doi.org/10.5194/acp-22-65-2022
    5. Tuomas Vielma, Lubomir Hnedkovsky, Glenn Hefter. Chemical speciation effects on the volumetric properties of aqueous sulfuric acid solutions. The Journal of Chemical Thermodynamics 2021, 158 , 106408. https://doi.org/10.1016/j.jct.2021.106408

    Journal of Chemical & Engineering Data

    Cite this: J. Chem. Eng. Data 2018, 63, 9, 3572–3583
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jced.8b00466
    Published September 4, 2018
    Copyright © 2018 American Chemical Society

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