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Reducing Circuit Depth in Adaptive Variational Quantum Algorithms via Effective Hamiltonian Theories
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    Quantum Electronic Structure

    Reducing Circuit Depth in Adaptive Variational Quantum Algorithms via Effective Hamiltonian Theories
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    Journal of Chemical Theory and Computation

    Cite this: J. Chem. Theory Comput. 2022, 18, 8, 4795–4805
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    https://doi.org/10.1021/acs.jctc.2c00341
    Published July 6, 2022
    Copyright © 2022 American Chemical Society

    Abstract

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    The electronic structure is an anticipated application for quantum computers. However, quantum circuits required to represent the highly entangled electronic wave functions within the variational quantum eigensolver (VQE) framework are far beyond the capacity of current quantum devices. To adapt the VQE algorithms to near-term quantum hardware, it has been suggested to incorporate a part of the electronic correlation into an effective Hamiltonian, leaving the wave function in a less entangled form. We propose a new scheme to construct the effective Hamiltonian with the transformation in the form of a product of linear combinations of excitation operators. This new scheme promises a quadratic multiplicative growth of the effective Hamiltonian. We integrate this effective Hamiltonian method into the adaptive VQE algorithms to maintain constant-size quantum circuits. The new computational scheme is assessed by performing numerical simulations for small molecules. A milli-Hartree accuracy in a minimal basis is achieved with a much shallower circuit depth.

    Copyright © 2022 American Chemical Society

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    Cited By

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    This article is cited by 5 publications.

    1. Francesco A. Evangelista, Victor S. Batista. Editorial: Quantum Computing for Chemistry. Journal of Chemical Theory and Computation 2023, 19 (21) , 7435-7436. https://doi.org/10.1021/acs.jctc.3c01043
    2. Robert A. Lang, Aadithya Ganeshram, Artur F. Izmaylov. Growth Reduction of Similarity-Transformed Electronic Hamiltonians in Qubit Space. Journal of Chemical Theory and Computation 2023, 19 (19) , 6656-6667. https://doi.org/10.1021/acs.jctc.3c00712
    3. Yi Fan, Jie Liu, Zhenyu Li, Jinlong Yang. Quantum Circuit Matrix Product State Ansatz for Large-Scale Simulations of Molecules. Journal of Chemical Theory and Computation 2023, 19 (16) , 5407-5417. https://doi.org/10.1021/acs.jctc.3c00068
    4. Zhenyu Li, Jie Liu, Xiangjian Shen, Feixue Gao. Challenges and opportunities of quantum-computational chemistry. SCIENTIA SINICA Chimica 2023, 53 (2) , 119-128. https://doi.org/10.1360/SSC-2022-0222
    5. Burak Mete, Martin Schulz, Martin Ruefenacht. Predicting the Optimizability for Workflow Decisions. 2022, 68-74. https://doi.org/10.1109/QCS56647.2022.00013

    Journal of Chemical Theory and Computation

    Cite this: J. Chem. Theory Comput. 2022, 18, 8, 4795–4805
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jctc.2c00341
    Published July 6, 2022
    Copyright © 2022 American Chemical Society

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