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Mallopenins A–E, Antibacterial Phenolic Derivatives from the Fruits of Mallotus philippensis
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    Mallopenins A–E, Antibacterial Phenolic Derivatives from the Fruits of Mallotus philippensis
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    • Sarot Cheenpracha*
      Sarot Cheenpracha
      Division of Chemistry, School of Science, University of Phayao, Phayao 56000, Thailand
      *Tel (S. Cheenpracha): +66-5446-6666. Fax: +66-5446-6664. E-mail: [email protected]
    • Stephen G. Pyne
      Stephen G. Pyne
      School of Chemistry and Molecular Biosciences, University of Wollongong, Wollongong, New South Wales 2522, Australia
    • Brian O. Patrick
      Brian O. Patrick
      Department of Chemistry and Earth, Ocean & Atmospheric Sciences, University of British Columbia, 2036 Main Mall, Vancouver, British Columbia, Canada V6T 1Z1
    • Raymond J. Andersen
      Raymond J. Andersen
      Department of Chemistry and Earth, Ocean & Atmospheric Sciences, University of British Columbia, 2036 Main Mall, Vancouver, British Columbia, Canada V6T 1Z1
    • Wisanu Maneerat
      Wisanu Maneerat
      Center of Chemical Innovation for Sustainability (CIS)  and  School of Science, Mae Fah Luang University, Chiang Rai 57100, Thailand
    • Surat Laphookhieo
      Surat Laphookhieo
      Center of Chemical Innovation for Sustainability (CIS)  and  School of Science, Mae Fah Luang University, Chiang Rai 57100, Thailand
    Other Access OptionsSupporting Information (2)

    Journal of Natural Products

    Cite this: J. Nat. Prod. 2019, 82, 8, 2174–2180
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    https://doi.org/10.1021/acs.jnatprod.9b00182
    Published July 18, 2019
    Copyright © 2019 American Chemical Society and American Society of Pharmacognosy

    Abstract

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    The chromatographic separation of the components of the acetone extract of Mallotus philippensis fruits yielded five new phenolic compounds including two chalcones, 1 and 3, a functionalized phloroglucinol, 2, two flavanones, 4 and 5, and six known compounds. The structures of 15 were confirmed by NMR and mass analyses. Racemic compounds 1 and 2 were separated by chiral-phase HPLC, and the absolute configuration of (+)-1 was confirmed by X-ray diffraction studies and ECD spectroscopic data. The configurations of the enantiomers of 2 were defined by comparison of its ECD data with those of (+)-1. Compounds 6 and 7 exhibited significant antibacterial activities, with MIC values ranging from 3.8 to 15.5 μM.

    Copyright © 2019 American Chemical Society and American Society of Pharmacognosy

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    Supporting Information

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.jnatprod.9b00182.

    • 1D and 2D NMR, HRTOFESIMS spectra of 15 (PDF)

    • X-ray crystallography for 1 (CIF)

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    Cited By

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    This article is cited by 12 publications.

    1. Fazlurrahman Khan, Nazia Tabassum, Nilushi Indika Bamunuarachchi, Young-Mog Kim. Phloroglucinol and Its Derivatives: Antimicrobial Properties toward Microbial Pathogens. Journal of Agricultural and Food Chemistry 2022, 70 (16) , 4817-4838. https://doi.org/10.1021/acs.jafc.2c00532
    2. Yan Huang, Ping Hou, Liwei Pan, Jian Li, Xiaoqin Liang, Chenyang Ren, Liuting Peng, Chunqiu Gan, Weifeng Xu, Ruiyun Yang, Jun Li, Xinlan Guan. Lignans and phenols with potential anti-inflammatory effect from the stems of Mallotus paxii Pamp. Fitoterapia 2024, 179 , 106253. https://doi.org/10.1016/j.fitote.2024.106253
    3. Yeqi Chen, Wenlin Zheng, Xun Song, Dabo Pan, Yue Zhuo, Zhenzhen Yang, Qi Wang, Yan Wu, Jihong Gu. Structurally diverse phenylpropanoyl phloroglucinol derivatives from Mallotus philippensis and their anti-bacterial activities. Bioorganic Chemistry 2024, 153 , 107918. https://doi.org/10.1016/j.bioorg.2024.107918
    4. Ahmad Ali, Hangping Chen, He Xu, Shuo Wang, Shun Yao. Accessing the Medicinal Potential of Mallotus philippensis: Comprehensive Exploration of Antioxidant and Antibacterial Properties through Phytochemical Analysis and Extraction Techniques. Separations 2024, 11 (6) , 165. https://doi.org/10.3390/separations11060165
    5. Waseem Rizvi, Syed Shariq Naeem, Ompal Singh, Shagufta Moin, Kafil Akhtar, Syed Najmul Hejaz Azmi, Zubair Ahmed, Monowarul Mobin Siddique, Zainul Amiruddin Zakaria, Qamar Uddin Ahmed. Mechanistic insights into the hepatoprotective properties of Mallotus phillipensis fruit: Targeting proinflammatory cytokines and free radicals using isolated compound. Journal of King Saud University - Science 2024, 36 (5) , 103192. https://doi.org/10.1016/j.jksus.2024.103192
    6. Andromachi Tzani, Eftichia Kritsi, Lamprini Tsamantioti, Ioanna Kostopoulou, Maria-Anna Karadendrou, Panagiotis Zoumpoulakis, Anastasia Detsi. Synthesis, Conformational Analysis and ctDNA Binding Studies of Flavonoid Analogues Possessing the 3,5-di-tert-butyl-4-hydroxyphenyl Moiety. Antioxidants 2022, 11 (11) , 2273. https://doi.org/10.3390/antiox11112273
    7. Nguyen Hoang Anh, SeonJu Park, Do Thi Trang, Duong Thi Hai Yen, Bui Huu Tai, Pham Hai Yen, Phan Van Kiem, Pham The Chinh, Nguyen Xuan Nhiem. Genus mallotus (euphorbiaceae): a review on traditional medicinal use, phytochemistry and biological activities. Vietnam Journal of Science and Technology 2022, 60 (2) , 141-174. https://doi.org/10.15625/2525-2518/16634
    8. Jin-Hai Yu, Zhi-Pu Yu, Robert J. Capon, Hua Zhang. Natural Enantiomers: Occurrence, Biogenesis and Biological Properties. Molecules 2022, 27 (4) , 1279. https://doi.org/10.3390/molecules27041279
    9. Kang Zhou, Song Yang, Shu-Ming Li. Naturally occurring prenylated chalcones from plants: structural diversity, distribution, activities and biosynthesis. Natural Product Reports 2021, 38 (12) , 2236-2260. https://doi.org/10.1039/D0NP00083C
    10. Xiao-Feng He, Ji-Jun Chen, Xiao-Yan Huang, Jing Hu, Xu-Ke Zhang, Yuan-Qiang Guo, Xue-Mei Zhang, Chang-An Geng. The antidiabetic potency of Amomum tsao-ko and its active flavanols, as PTP1B selective and α-glucosidase dual inhibitors. Industrial Crops and Products 2021, 160 , 112908. https://doi.org/10.1016/j.indcrop.2020.112908
    11. Hang Li, Alastair E. Lacey, Si Shu, John A. Kalaitzis, Daniel Vuong, Andrew Crombie, Jinyu Hu, Cameron L. M. Gilchrist, Ernest Lacey, Andrew M. Piggott, Yit-Heng Chooi. Hancockiamides: phenylpropanoid piperazines from Aspergillus hancockii are biosynthesised by a versatile dual single-module NRPS pathway. Organic & Biomolecular Chemistry 2021, 19 (3) , 587-595. https://doi.org/10.1039/D0OB02243H
    12. Yvan Anderson Ngandjui Tchangoue, Joseph Tchamgoue, Paul Keilah Lunga, Janosch Knepper, Ramona Paltinean, Kerstin Ibrom, Gianina Crișan, Simeon Fogue Kouam, Muhammad Shaiq Ali, Stefan Schulz. Antibacterial phloroglucinols derivatives from the leaves of Mallotus oppositifolius (Geisler) Müll. Arg. (Euphorbiaceae). Fitoterapia 2020, 142 , 104527. https://doi.org/10.1016/j.fitote.2020.104527

    Journal of Natural Products

    Cite this: J. Nat. Prod. 2019, 82, 8, 2174–2180
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jnatprod.9b00182
    Published July 18, 2019
    Copyright © 2019 American Chemical Society and American Society of Pharmacognosy

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