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Strong Field Double Ionization of Formaldehyde Investigated Using Momentum Resolved Covariance Imaging and Trajectory Surface Hopping

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Download Hi-Res ImageDownload to MS-PowerPointCite This:J. Phys. Chem. A 2022, 126, 40, 7399-7406
    A: New Tools and Methods in Experiment and Theory

    Strong Field Double Ionization of Formaldehyde Investigated Using Momentum Resolved Covariance Imaging and Trajectory Surface Hopping
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    • Chuan Cheng
      Chuan Cheng
      Department of Physics and Astronomy, Stony Brook University, Stony Brook, New York11794-3800, United States
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    • Vaibhav Singh
      Vaibhav Singh
      Department of Chemistry, Temple University, Philadelphia, Pennsylvania19122, United States
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    • Spiridoula Matsika
      Spiridoula Matsika
      Department of Chemistry, Temple University, Philadelphia, Pennsylvania19122, United States
      More by Spiridoula Matsika
      Orcidhttps://orcid.org/0000-0003-2773-3979
    • Thomas Weinacht*
      Thomas Weinacht
      Department of Physics and Astronomy, Stony Brook University, Stony Brook, New York11794-3800, United States
      More by Thomas Weinacht
      Orcidhttps://orcid.org/0000-0001-9343-7276
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    The Journal of Physical Chemistry A

    Cite this: J. Phys. Chem. A 2022, 126, 40, 7399–7406
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    https://doi.org/10.1021/acs.jpca.2c04650
    Published September 30, 2022
    Copyright © 2022 American Chemical Society
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    Abstract

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    We use covariance velocity map imaging of fragment ions from the strong field double ionization of formaldehyde in conjunction with trajectory surface hopping calculations to determine the ionization yields to different singlet and triplet states of the dication. The calculated kinetic energy release for trajectories initiated on different electronic states is compared with the experimental values based on momentum resolved covariance measurements. We determine the state resolved double ionization yields as a function of laser intensity and pulse duration down to 6 fs (two optical cycles).

    Copyright © 2022 American Chemical Society

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    The Journal of Physical Chemistry A

    Cite this: J. Phys. Chem. A 2022, 126, 40, 7399–7406
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.jpca.2c04650
    Published September 30, 2022
    Copyright © 2022 American Chemical Society
    Request reuse permissions

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