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Spontaneous Recurrence of Deposition and Dissolution of a Solid Layer on a Solution Surface

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Department of Physics, Graduate School of Science, Chiba University, 1-33 Yayoi-cho, Inage-ku, Chiba 263-8522, Japan
‡ § Graduate School of Advanced Mathematical Sciences and §Meiji Institute of Advanced Study of Mathematical Sciences, Meiji University, 4-21-1 Nakano, Tokyo 164-8525, Japan
Cite this: J. Phys. Chem. B 2015, 119, 30, 9970–9974
Publication Date (Web):July 1, 2015
https://doi.org/10.1021/acs.jpcb.5b03413
Copyright © 2015 American Chemical Society

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    Abstract

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    We investigated the spontaneous recurrence of deposition and dissolution of camphor layer on the surface of camphor methanol solution. This recurrence is a novel rhythmic process concerned with solid–liquid phase transition. To elucidate the underlying mechanism, we measured the solution temperature at different times, and found that the temperature increased and decreased repetitively, correlating with the camphor layer’s deposition and dissolution. These experimental results show that the solution temperature plays an important role in recurrence of deposition and dissolution.

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    Supporting Information

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    This material includes (i) measurement of periods between adjacent dissolutions of the camphor layer, (ii) observation of wetting dynamics of a methanol droplet placed on a camphor disk, and (iii) the movie (jp5b03413_si_002.mpg, 10 times faster than real time) of the spontaneous recurrence of deposition and dissolution of the camphor layer corresponding to Figure 1 and the movie (jp5b03413_si_003.mpg, in real time) of the spontaneous recurrence observed for a droplet on a lab bench. The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.jpcb.5b03413.

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    Cited By

    This article is cited by 1 publications.

    1. Nobuhiko J. Suematsu, Junpei Iwamoto, Yuya Ishii, Akira Yamamoto. Dendrite Pattern Formation of Sodium Chloride Crystal. Materials 2021, 14 (16) , 4434. https://doi.org/10.3390/ma14164434

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