ACS Publications. Most Trusted. Most Cited. Most Read

OR SEARCH CITATIONS

My Activity
Publications
CONTENT TYPES

Figure 1Loading Img
Download Hi-Res ImageDownload to MS-PowerPointCite This:J. Phys. Chem. C 2019, 123, 43, 26509-26515
RETURN TO ISSUEPREVArticleNEXT

Propagating Hybrid Tamm Exciton Polaritons in Organic Microcavity

  • Bin Liu
    Bin Liu
    Department of Physics, City College of New York, New York, New York 10031, United States
    More by Bin Liu
  • , 
  • Rong Wu
    Rong Wu
    Department of Physics, City College of New York, New York, New York 10031, United States
    Department of Physics, Graduate Center of the City University of New York (CUNY), New York, New York 10016, United States
    More by Rong Wu
  • , and 
  • Vinod M. Menon*
    Vinod M. Menon
    Department of Physics, City College of New York, New York, New York 10031, United States
    Department of Physics, Graduate Center of the City University of New York (CUNY), New York, New York 10016, United States
    *E-mail: [email protected]
    More by Vinod M. Menon
    Orcidhttp://orcid.org/0000-0002-9725-6445
Cite this: J. Phys. Chem. C 2019, 123, 43, 26509–26515
Publication Date (Web):October 11, 2019
https://doi.org/10.1021/acs.jpcc.9b06383
Copyright © 2019 American Chemical Society
Request reuse permissions

    Article Views

    946

    Altmetric

    -

    Citations

    19
    LEARN ABOUT THESE METRICS
    Read OnlinePDF (5 MB)
    Get e-Alerts
    Supporting Info (1)»
    SUBJECTS:

    Abstract

    Abstract Image

    Strong coupling between Tamm plasmons and organic cavity polaritons is observed at room temperature. Angle-resolved reflectometry experiments unambiguously indicate the anticrossing in the dispersion relations, which is characteristic of the strong coupling regime, and the Tamm plasmon–cavity polariton hybrid states can be energetically manipulated by tuning the Tamm plasmons. The experimental data are in good agreement with calculations based on the transfer matrix method. Emission from the lower energy Tamm plasmon–cavity polariton hybrid states is observed, and the propagation property of the hybrid Tamm plasmon polariton is also studied. The real-space imaging experiments reveal that the propagation distance is larger when the Tamm plasmon and cavity polariton are strongly coupled in comparison to both the exciton of the uncoupled organic neat film and the cavity polaritons. Moreover, the propagation length of the hybrid polaritons increases as the fraction of Tamm plasmon component in the hybrid states increases.

    Supporting Information

    ARTICLE SECTIONS
    Jump To

    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.jpcc.9b06383.

    • Optical spectroscopy characterization; electric field intensity distribution profile simulation; exponential fitting for the real-space PL intensity; Hopfield coefficients; power-dependent angle-resolved photoluminescence; parameters for the coupled oscillator model (PDF)

    Terms & Conditions

    Most electronic Supporting Information files are available without a subscription to ACS Web Editions. Such files may be downloaded by article for research use (if there is a public use license linked to the relevant article, that license may permit other uses). Permission may be obtained from ACS for other uses through requests via the RightsLink permission system: http://pubs.acs.org/page/copyright/permissions.html.

    Cited By

    This article is cited by 19 publications.

    1. Bin Liu, Jason Lynch, Haonan Zhao, Ben R. Conran, Clifford McAleese, Deep Jariwala, Stephen R. Forrest. Long-Range Propagation of Exciton-Polaritons in Large-Area 2D Semiconductor Monolayers. ACS Nano 2023, 17 (15) , 14442-14448. https://doi.org/10.1021/acsnano.3c03485
    2. Nikhil Puthiya Purayil, Athulya Kadeprath Satheesan, Shiju Edappadikkunnummal, Chandrasekharan Keloth. Coupling of the Tamm Plasmon to the BODIPY Fluorophore in Photonic Crystals for Nonlinear Optical Applications. The Journal of Physical Chemistry C 2023, 127 (2) , 1244-1250. https://doi.org/10.1021/acs.jpcc.2c07579
    3. Hui-Hsin Hsiao, Chu-Han Huang, Bo-Ting Xu, Guan-Ting Chen, Po-Wei Ho. Triple Narrowband Mid-Infrared Thermal Emitter Based on a Au Grating-Assisted Nanoscale Germanium/Titanium Dioxide Distributed Bragg Reflector: Implications for Molecular Sensing. ACS Applied Nano Materials 2021, 4 (9) , 9344-9352. https://doi.org/10.1021/acsanm.1c01818
    4. Chen Ye, Suman Mallick, Manuel Hertzog, Markus Kowalewski, Karl Börjesson. Direct Transition from Triplet Excitons to Hybrid Light–Matter States via Triplet–Triplet Annihilation. Journal of the American Chemical Society 2021, 143 (19) , 7501-7508. https://doi.org/10.1021/jacs.1c02306
    5. Konstantin M. Morozov, Konstantin A. Ivanov, Alexey V. Belonovski, Elizaveta I. Girshova, Daniel de Sa Pereira, Christopher Menelaou, Piotr Pander, Larissa G. Franca, Andrew P. Monkman, Galia Pozina, Daniil A. Livshits, Nikita V. Selenin, Mikhail A. Kaliteevski. Efficient UV Luminescence from Organic-Based Tamm Plasmon Structures Emitting in the Strong-Coupling Regime. The Journal of Physical Chemistry C 2020, 124 (39) , 21656-21663. https://doi.org/10.1021/acs.jpcc.0c05091
    6. Gregory V. Hartland, (Deputy Editor, The Journal of Physical Chemistry C)Gregory D. Scholes (Editor-in-Chief, The Journal of Physical Chemistry Letters). Virtual Issue on Polaritons in Physical Chemistry. The Journal of Physical Chemistry C 2020, 124 (37) , 19875-19879. https://doi.org/10.1021/acs.jpcc.0c07359
    7. Gregory V. Hartland, (Deputy Editor, The Journal of Physical Chemistry C)Gregory D. Scholes (Editor-in-Chief, The Journal of Physical Chemistry Letters). Virtual Issue on Polaritons in Physical Chemistry. The Journal of Physical Chemistry Letters 2020, 11 (18) , 7920-7924. https://doi.org/10.1021/acs.jpclett.0c02457
    8. Bin Liu, Vinod M. Menon, Matthew Y. Sfeir. The Role of Long-Lived Excitons in the Dynamics of Strongly Coupled Molecular Polaritons. ACS Photonics 2020, 7 (8) , 2292-2301. https://doi.org/10.1021/acsphotonics.0c00895
    9. Chinmaya Kar, Shuvendu Jena, Dinesh V. Udupa, K. Divakar Rao. Tamm plasmon polariton in planar structures: A brief overview and applications. Optics & Laser Technology 2023, 159 , 108928. https://doi.org/10.1016/j.optlastec.2022.108928
    10. Bin Liu, Xinjing Huang, Shaocong Hou, Dejiu Fan, Stephen R. Forrest. Photocurrent generation following long-range propagation of organic exciton–polaritons. Optica 2022, 9 (9) , 1029. https://doi.org/10.1364/OPTICA.461025
    11. Sitakanta Satapathy, Bin Liu, Prathmesh Deshmukh, Paul M. Molinaro, Florian Dirnberger, Mandeep Khatoniar, Ronald L. Koder, Vinod M. Menon. Thermalization of Fluorescent Protein Exciton–Polaritons at Room Temperature. Advanced Materials 2022, 34 (15) https://doi.org/10.1002/adma.202109107
    12. J. Paul, H. Rose, E. Swagel, T. Meier, J. K. Wahlstrand, A. D. Bristow. Coherent contributions to population dynamics in a semiconductor microcavity. Physical Review B 2022, 105 (11) https://doi.org/10.1103/PhysRevB.105.115307
    13. Wen-Hui Xu, Yu-Hsun Chou, Zih-Ying Yang, Yi-Yun Liu, Min-Wen Yu, Chen-Hang Huang, Chun-Tse Chang, Chen-Yu Huang, Tien-Chang Lu, Tzy-Rong Lin, Kuo-Ping Chen. Tamm Plasmon‐Polariton Ultraviolet Lasers. Advanced Photonics Research 2022, 3 (1) https://doi.org/10.1002/adpr.202100120
    14. Chenran Xu, Han Cai, Da-Wei Wang. Vibrational strong coupling between Tamm phonon polaritons and organic molecules. Journal of the Optical Society of America B 2021, 38 (5) , 1505. https://doi.org/10.1364/JOSAB.419042
    15. Mona Kliem, Thomas Kiel, Malin Kück, Stefan Meister, Andreas Mischok, Hartmut Fröb, Kurt Busch, Karl Leo. Defect‐State Lasing in Photonic Lattices of Metal–Organic Microcavities. Advanced Photonics Research 2021, 2 (3) https://doi.org/10.1002/adpr.202000116
    16. Bin Liu, Vinod M. Menon, Matthew Y. Sfeir. Ultrafast thermal modification of strong coupling in an organic microcavity. APL Photonics 2021, 6 (1) https://doi.org/10.1063/5.0031560
    17. D. N. Basov, Ana Asenjo-Garcia, P. James Schuck, Xiaoyang Zhu, Angel Rubio. Polariton panorama. Nanophotonics 2020, 10 (1) , 549-577. https://doi.org/10.1515/nanoph-2020-0449
    18. A. Putintsev, A. Zasedatelev, K. E. McGhee, T. Cookson, K. Georgiou, D. Sannikov, D. G. Lidzey, P. G. Lagoudakis. Nano-second exciton-polariton lasing in organic microcavities. Applied Physics Letters 2020, 117 (12) https://doi.org/10.1063/5.0019195
    19. Kun Zhang, Yan Liu, Feng Xia, Shixia Li, Weijin Kong. Tuning of the polariton modes induced by longitudinal strong coupling in the graphene hybridized DBR cavity. Optics Letters 2020, 45 (13) , 3669. https://doi.org/10.1364/OL.397342
    Download PDF

    Pair your accounts.

    Export articles to Mendeley

    Get article recommendations from ACS based on references in your Mendeley library.

    Pair your accounts.

    Export articles to Mendeley

    Get article recommendations from ACS based on references in your Mendeley library.

    You’ve supercharged your research process with ACS and Mendeley!

    STEP 1:
    Click to create an ACS ID

    Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

    Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

    Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

    MENDELEY PAIRING EXPIRED
    Your Mendeley pairing has expired. Please reconnect