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Ultrafast Hydrogen Migration in Photoionized Glycine

  • M. C. Castrovilli*
    M. C. Castrovilli
    Istituto Struttura della Materia, ISM-CNR, 00016 Monterotondo Scalo, Roma, Italy
    Institute for Photonics and Nanotechnologies, IFN-CNR, 20133 Milano, Italy
    *E-mail: [email protected]
  • A. Trabattoni
    A. Trabattoni
    Department of Physics, Politecnico di Milano, 20133 Milano, Italy
    CFEL-DESY, Notkerstrasse 85, 22607 Hamburg, Germany
  • P. Bolognesi
    P. Bolognesi
    Istituto Struttura della Materia, ISM-CNR, 00016 Monterotondo Scalo, Roma, Italy
    More by P. Bolognesi
  • P. O’Keeffe
    P. O’Keeffe
    Istituto Struttura della Materia, ISM-CNR, 00016 Monterotondo Scalo, Roma, Italy
  • L. Avaldi
    L. Avaldi
    Istituto Struttura della Materia, ISM-CNR, 00016 Monterotondo Scalo, Roma, Italy
    More by L. Avaldi
  • M. Nisoli
    M. Nisoli
    Department of Physics, Politecnico di Milano, 20133 Milano, Italy
    Institute for Photonics and Nanotechnologies, IFN-CNR, 20133 Milano, Italy
    More by M. Nisoli
  • F. Calegari
    F. Calegari
    CFEL-DESY, Notkerstrasse 85, 22607 Hamburg, Germany
    Department of Physics, University of Hamburg, 20355 Hamburg, Germany
    Institute for Photonics and Nanotechnologies, IFN-CNR, 20133 Milano, Italy
    More by F. Calegari
  • , and 
  • R. Cireasa
    R. Cireasa
    Institut des Sciences Moléculaires d’Orsay, CNRS, Université Paris Sud, 91400 Orsay, France
    More by R. Cireasa
Cite this: J. Phys. Chem. Lett. 2018, 9, 20, 6012–6016
Publication Date (Web):September 25, 2018
https://doi.org/10.1021/acs.jpclett.8b02089
Copyright © 2018 American Chemical Society

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    Abstract

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    Hydrogen migration in the glycine cation has been investigated using a combination of a short train of attosecond extreme ultraviolet pulses with few-optical-cycle near-infrared pulses. The yield of the photofragments produced has been measured as a function of pump–probe delay. These time-dependent measurements reveal the presence of a hydrogen migration process occurring in 48 fs. Previous mass spectrometric experiments and theoretical calculations have allowed us to identify the conformations and cation states involved in the process induced by the broad band extreme ultraviolet radiation.

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    Cited By

    This article is cited by 16 publications.

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