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Monolithic Metal Dimer-on-Film Structure: New Plasmonic Properties Introduced by the Underlying Metal

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Download Hi-Res ImageDownload to MS-PowerPointCite This:Nano Lett. 2020, 20, 3, 2087-2093
    Letter

    Monolithic Metal Dimer-on-Film Structure: New Plasmonic Properties Introduced by the Underlying Metal
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    • Burak Gerislioglu
      Burak Gerislioglu
      Department of Physics and Astronomy  and  Laboratory for Nanophotonics, Rice University, 6100 Main Street, Houston, Texas 77005, United States
      More by Burak Gerislioglu
      Orcidhttp://orcid.org/0000-0001-8575-7990
    • Liangliang Dong
      Liangliang Dong
      Department of Chemistry  and  Laboratory for Nanophotonics, Rice University, 6100 Main Street, Houston, Texas 77005, United States
      More by Liangliang Dong
    • Arash Ahmadivand
      Arash Ahmadivand
      Department of Electrical and Computer Engineering, Rice University, 6100 Main Street, Houston, Texas 77005, United States
      More by Arash Ahmadivand
      Orcidhttp://orcid.org/0000-0003-0808-8775
    • Huatian Hu
      Huatian Hu
      The Institute for Advanced Studies, Wuhan University, Wuhan 430072, China
      More by Huatian Hu
    • Peter Nordlander*
      Peter Nordlander
      Department of Physics and Astronomy,  Department of Electrical and Computer Engineering  and  Laboratory for Nanophotonics, Rice University, 6100 Main Street, Houston, Texas 77005, United States
      *E-mail: [email protected]
      More by Peter Nordlander
      Orcidhttp://orcid.org/0000-0002-1633-2937
    • Naomi J. Halas*
      Naomi J. Halas
      Department of Physics and Astronomy,  Department of Chemistry,  Department of Electrical and Computer Engineering  and  Laboratory for Nanophotonics, Rice University, 6100 Main Street, Houston, Texas 77005, United States
      *E-mail: [email protected],.
      More by Naomi J. Halas
      Orcidhttp://orcid.org/0000-0002-8461-8494
    Other Access OptionsSupporting Information (1)

    Nano Letters

    Cite this: Nano Lett. 2020, 20, 3, 2087–2093
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    https://doi.org/10.1021/acs.nanolett.0c00075
    Published January 28, 2020
    Copyright © 2020 American Chemical Society
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    Abstract

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    Dimers, two closely spaced metallic nanostructures, are one of the primary nanoscale geometries in plasmonics, supporting high local field enhancements in their interparticle junction under excitation of their hybridized “bonding” plasmon. However, when a dimer is fabricated on a metallic substrate, its characteristics are changed profoundly. Here we examine the properties of a Au dimer on a Au substrate. This structure supports a bright “bonding” dimer plasmon, screened by the metal, and a lower energy magnetic charge transfer plasmon. Changing the dielectric environment of the dimer-on-film structure reveals a broad family of higher-order hybrid plasmons in the visible region of the spectrum. Both of the localized surface plasmons resonances (LSPR) of the individual dimer-on-film structures as well as their collective surface lattice resonances (SLR) show a highly sensitive refractive index sensing response. Implementation of such all-metal magnetic-resonant nanostructures offers a promising route to achieve higher-performance LSPR- and SLR-based plasmonic sensors.

    Copyright © 2020 American Chemical Society

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    • Tilted SEM image, simulations for a fictitious Au film-included geometry, electric-and magnetic-field enhancement, and current density maps of the all-metal unit-cell platform; additional data about the SLR reflection spectra; SEM pictures of the ordered and disordered metasurfaces (PDF)

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    Cited By

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    This article is cited by 106 publications.

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    Cite this: Nano Lett. 2020, 20, 3, 2087–2093
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