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A Fano Cavity–Photon Interface for Directional Suppression of Spectral Diffusion of a Single Perovskite Nanoplatelet
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    A Fano Cavity–Photon Interface for Directional Suppression of Spectral Diffusion of a Single Perovskite Nanoplatelet
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    • Yuqing Huang*
      Yuqing Huang
      Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore637371, Singapore
      *Email for Y.H.: [email protected]
      More by Yuqing Huang
    • Rui Su
      Rui Su
      Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore637371, Singapore
      School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore637371, Singapore
      More by Rui Su
    • Yubin Wang
      Yubin Wang
      State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing100084, People’s Republic of China
      More by Yubin Wang
    • Chao Zhu
      Chao Zhu
      SEU-FEI Nano-Pico Center, Key Laboratory of MEMS of Ministry of Education, Collaborative Innovation Center for Micro/Nano Fabrication, Device and System, Southeast University, Nanjing210096, People’s Republic of China
      More by Chao Zhu
    • Jiangang Feng
      Jiangang Feng
      Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore637371, Singapore
    • Jiaxin Zhao
      Jiaxin Zhao
      Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore637371, Singapore
      More by Jiaxin Zhao
    • Zheng Liu
      Zheng Liu
      School of Materials Science and Engineering, Nanyang Technological University, Singapore639798, Singapore
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    • Qihua Xiong*
      Qihua Xiong
      State Key Laboratory of Low-Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing100084, People’s Republic of China
      Frontier Science Center for Quantum Information, Beijing100084, People’s Republic of China
      Collaborative Innovation Center of Quantum Matter, Beijing100871, People’s Republic of China
      Beijing Academy of Quantum Information Sciences, Beijing100193, P.R. China
      *Email for Q.X.: [email protected]
      More by Qihua Xiong
    Other Access OptionsSupporting Information (1)

    Nano Letters

    Cite this: Nano Lett. 2022, 22, 20, 8274–8280
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    https://doi.org/10.1021/acs.nanolett.2c03073
    Published October 5, 2022
    Copyright © 2022 American Chemical Society

    Abstract

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    Colloidal nanocrystals that are capable of mass production with wet chemical synthesis have long been proposed as color-tunable, scalable quantum emitters for information processing and communication. However, they constantly suffer from spectral diffusion due to being exposed to a noisy electrostatic environment. Herein we demonstrate a cavity–photon interface (CPI) which effectively suppresses the temperature-activated spectral diffusion (SD) of a single perovskite nanoplatelet (NPL) up to 40 K. The spectrally stabilized single-photon emission is achieved at a specific emission direction corresponding to an inhibited dipole moment of the NPL as the result of the Fano coupling between the two photon dissipation channels of the NPL. Our results shed light on the nature of the SD of perovskite nanocrystals and offer a general cavity quantum electrodynamic scheme that controls the brightness and spectral dynamics of a single-photon emitter.

    Copyright © 2022 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.nanolett.2c03073.

    • Methods, TEM images of the perovskite nanoplatelet, schematics of the device fabrication process, excitation power dependence of TRPL spectra of nanoplatelets, temperature-dependent PL spectra of nanoplatelets, estimation of Q-factor and Purcell enhancement, Voigt fitting of the spectral line shape, and fitting parameters of the angle-resolved PL and angle-resolved reflectance spectra (PDF)

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    Cited By

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    This article is cited by 7 publications.

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    2. Hao A. Nguyen, Grant Dixon, Florence Y. Dou, Shaun Gallagher, Stephen Gibbs, Dylan M. Ladd, Emanuele Marino, Justin C. Ondry, James P. Shanahan, Eugenia S. Vasileiadou, Stephen Barlow, Daniel R. Gamelin, David S. Ginger, David M. Jonas, Mercouri G. Kanatzidis, Seth R. Marder, Daniel Morton, Christopher B. Murray, Jonathan S. Owen, Dmitri V. Talapin, Michael F. Toney, Brandi M. Cossairt. Design Rules for Obtaining Narrow Luminescence from Semiconductors Made in Solution. Chemical Reviews 2023, 123 (12) , 7890-7952. https://doi.org/10.1021/acs.chemrev.3c00097
    3. Guangxin Liu, Wenjie Zhou, Dmitrii Gromyko, Ding Huang, Zhaogang Dong, Renming Liu, Juanfeng Zhu, Jingfeng Liu, Cheng-Wei Qiu, Lin Wu. Single-photon generation and manipulation in quantum nanophotonics. Applied Physics Reviews 2025, 12 (1) https://doi.org/10.1063/5.0227350
    4. Yubin Wang, Huawen Xu, Xinyi Deng, Timothy C. H. Liew, Sanjib Ghosh, Qihua Xiong. Topological single-photon emission from quantum emitter chains. npj Quantum Information 2024, 10 (1) https://doi.org/10.1038/s41534-024-00807-y
    5. Martin Esmann, Stephen C. Wein, Carlos Antón‐Solanas. Solid‐State Single‐Photon Sources: Recent Advances for Novel Quantum Materials. Advanced Functional Materials 2024, 34 (30) https://doi.org/10.1002/adfm.202315936
    6. Hui Zhang, Feifei Cai, Bo Huang, Huichao Zhang, Shitong Li. Emission variation and spontaneous deformation of CsPbBr 3 perovskite nanoplatelets at low concentrations. Journal of Materials Chemistry C 2023, 12 (1) , 301-310. https://doi.org/10.1039/D3TC02178E
    7. Yifei Geng, Kazuki Nomoto. Ultrafast spectral diffusion of GaN defect single photon emitters. Applied Physics Letters 2023, 123 (17) https://doi.org/10.1063/5.0171855

    Nano Letters

    Cite this: Nano Lett. 2022, 22, 20, 8274–8280
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.nanolett.2c03073
    Published October 5, 2022
    Copyright © 2022 American Chemical Society

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