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Download Hi-Res ImageDownload to MS-PowerPointCite This:Nano Lett. 2022, 22, 23, 9405-9410
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    Ferroelectric Ordering in Nanosized PbTiO3
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    • Qiang Li*
      Qiang Li
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
      *[email protected]
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      Orcidhttps://orcid.org/0000-0003-4259-6984
    • Jing Sun
      Jing Sun
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
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    • Yuanpeng Zhang
      Yuanpeng Zhang
      Neutron Science Division, Oak Ridge National Laboratory (ORNL), Oak Ridge, Tennessee 37831, United States
      More by Yuanpeng Zhang
    • Tianyu Li
      Tianyu Li
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
      More by Tianyu Li
      Orcidhttps://orcid.org/0000-0001-8857-433X
    • Hui Liu
      Hui Liu
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
      More by Hui Liu
      Orcidhttps://orcid.org/0000-0002-4973-9784
    • Yili Cao
      Yili Cao
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
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    • Qinghua Zhang
      Qinghua Zhang
      Beijing National Laboratory for Condensed Matter Physics, Chinese Academy of Science, Beijing 100190, China
      More by Qinghua Zhang
    • Lin Gu
      Lin Gu
      Beijing National Center for Electron Microscopy and Laboratory of Advanced Materials, Department of Materials Science and Engineering, Tsinghua University, Beijing 100084, China
      More by Lin Gu
    • Takashi Honda
      Takashi Honda
      Institute of Materials Structure Science, High Energy Accelerator Research Organization (KEK), Tsukuba, Ibaraki 305-0801, Japan
      More by Takashi Honda
      Orcidhttps://orcid.org/0000-0003-4121-8957
    • Kazutaka Ikeda
      Kazutaka Ikeda
      Institute of Materials Structure Science, High Energy Accelerator Research Organization (KEK), Tsukuba, Ibaraki 305-0801, Japan
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    • Toshiya Otomo
      Toshiya Otomo
      Institute of Materials Structure Science, High Energy Accelerator Research Organization (KEK), Tsukuba, Ibaraki 305-0801, Japan
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    • Kun Lin
      Kun Lin
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
      More by Kun Lin
      Orcidhttps://orcid.org/0000-0003-4515-3206
    • Jinxia Deng
      Jinxia Deng
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
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    • Xianran Xing*
      Xianran Xing
      Beijing Advanced Innovation Center for Materials Genome Engineering, Institute of Solid State Chemistry, University of Science and Technology Beijing, Beijing 100083, China
      *[email protected]
      More by Xianran Xing
      Orcidhttps://orcid.org/0000-0003-0704-8886
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    Nano Letters

    Cite this: Nano Lett. 2022, 22, 23, 9405–9410
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    https://doi.org/10.1021/acs.nanolett.2c03303
    Published November 21, 2022
    Copyright © 2022 American Chemical Society
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    Abstract

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    The insight into the three-dimensional configuration of ferroelectric ordering in ferroelectric nanomaterials is motivated by the application of the development of functional nanodevices and the structural designing. However, the atomic deciphering of the spatial distribution of ordered structure remains challenging for the limitation of dimension and probing techniques. In this paper, a neutron pair distribution function (nPDF) was utilized to analyze the spontaneous polarization distribution of zero-dimensional PbTiO3 nanoparticles in three dimensions, via the application of reverse Monte Carlo (RMC) modeling. The comprehensive identification with transmission electron microscopy verified the linear characteristics of polarization along the c-axis in the main body, while electric polarization distribution on the surface was enhanced abnormally. In addition, the correlation of dipole vectors extending to three unit cells below the surface is retained. This work shows an application of the micro/macroscale information to effectively decode the polarization structure of nanoferroelectrics, providing new views of designing nanoferroelectric devices.

    Copyright © 2022 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acs.nanolett.2c03303.

    • Real-space refinements of the nPDF of nanosized and bulk PbTiO3, RMC results, c/a mapping based on the STEM image, and statistic graphs for the bulk model (PDF)

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    Cited By

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    This article is cited by 1 publications.

    1. Wojciech A. Sławiński, Christopher J. Kerr, Yuanpeng Zhang, Helen Y. Playford, Martin T. Dove, Anthony E. Phillips, Matthew G. Tucker. RMCProfile7 : reverse Monte Carlo for multiphase systems. Journal of Applied Crystallography 2024, 57 (4) , 1251-1262. https://doi.org/10.1107/S1600576724004175
    2. Lin He, JiaHua Li, Yin Ren, Yunfei He, Sisi Li, Yahong Wang, Peng Ye, Luming Zhou, Rongli Gao, Zhenhua Wang, Wei Cai, Chunlin Fu. Effect of Mn Doping on the Photovoltaic Properties of Multiferroic Composite Nanowire Arrays. 2024https://doi.org/10.2139/ssrn.4805384
    3. Lin He, JiaHua Li, Yin Ren, Yunfei He, Sisi Li, Yahong Wang, Peng Ye, Luming Zhou, Rongli Gao, Zhenhua Wang, Wei Cai, Chunlin Fu. Effect of Mn Doping on the Photovoltaic Properties of Multiferroic Composite Nanowire Arrays. 2024https://doi.org/10.2139/ssrn.4826562
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    Nano Letters

    Cite this: Nano Lett. 2022, 22, 23, 9405–9410
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.nanolett.2c03303
    Published November 21, 2022
    Copyright © 2022 American Chemical Society
    Request reuse permissions

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