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Ising Superconductivity and Quantum Phase Transition in Macro-Size Monolayer NbSe2

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    Ising Superconductivity and Quantum Phase Transition in Macro-Size Monolayer NbSe2
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    † International Center for Quantum Materials, School of Physics, Peking University, Beijing 100871, China
    ‡ State Key Laboratory of Low-Dimensional Quantum Physics, Department of Physics, Tsinghua University, Beijing 100084, China
    § High Magnetic Field Laboratory, Chinese Academy of Sciences, Hefei 230031, China
    ∥ Beijing Key Laboratory of Optical Detection Technology for Oil and Gas, China University of Petroleum, Beijing 102249, China
    ⊥ Department of Physics, Beijing Normal University, Beijing 100875, China
    # Collaborative Innovation Center of Quantum Matter, Beijing 100871, China
    *E-mail: [email protected]
    *E-mail: [email protected]
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    Nano Letters

    Cite this: Nano Lett. 2017, 17, 11, 6802–6807
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    https://doi.org/10.1021/acs.nanolett.7b03026
    Published October 2, 2017
    Copyright © 2017 American Chemical Society
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    Abstract

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    Two-dimensional (2D) transition metal dichalcogenides (TMDs) have a range of unique physics properties and could be used in the development of electronics, photonics, spintronics, and quantum computing devices. The mechanical exfoliation technique of microsize TMD flakes has attracted particular interest due to its simplicity and cost effectiveness. However, for most applications, large-area and high-quality films are preferred. Furthermore, when the thickness of crystalline films is down to the 2D limit (monolayer), exotic properties can be expected due to the quantum confinement and symmetry breaking. In this paper, we have successfully prepared macro-size atomically flat monolayer NbSe2 films on bilayer graphene terminated surface of 6H-SiC(0001) substrates by a molecular beam epitaxy (MBE) method. The films exhibit an onset superconducting critical transition temperature (Tconset) above 6 K and the zero resistance superconducting critical transition temperature (Tczero) up to 2.40 K. Simultaneously, the transport measurements at high magnetic fields and low temperatures reveal that the parallel characteristic field Bc//(T = 0) is above 5 times of the paramagnetic limiting field, consistent with Zeeman-protected Ising superconductivity mechanism. Besides, by ultralow temperature electrical transport measurements, the monolayer NbSe2 film shows the signature of quantum Griffiths singularity (QGS) when approaching the zero-temperature quantum critical point.

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    • Sample preparation, transport measurements and BKT-like transition, theoretical calculations, finite size scaling analysis (PDF)

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    Cite this: Nano Lett. 2017, 17, 11, 6802–6807
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    https://doi.org/10.1021/acs.nanolett.7b03026
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