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    Quantum Optics with Near-Lifetime-Limited Quantum-Dot Transitions in a Nanophotonic Waveguide
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    • Henri Thyrrestrup*
      Henri Thyrrestrup
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
      *E-mail: [email protected]
      More by Henri Thyrrestrup
      Orcidhttp://orcid.org/0000-0001-8922-4462
    • Gabija Kiršanskė
      Gabija Kiršanskė
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
      More by Gabija Kiršanskė
    • Hanna Le Jeannic
      Hanna Le Jeannic
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
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    • Tommaso Pregnolato
      Tommaso Pregnolato
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
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    • Liang Zhai
      Liang Zhai
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
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    • Laust Raahauge
      Laust Raahauge
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
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    • Leonardo Midolo
      Leonardo Midolo
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
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    • Nir Rotenberg
      Nir Rotenberg
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
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    • Alisa Javadi
      Alisa Javadi
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
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    • Rüdiger Schott
      Rüdiger Schott
      Lehrstuhl für Angewandte Festkörperphysik, Ruhr-Universität Bochum, Universitätsstrasse 150, D-44780 Bochum, Germany
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    • Andreas D. Wieck
      Andreas D. Wieck
      Lehrstuhl für Angewandte Festkörperphysik, Ruhr-Universität Bochum, Universitätsstrasse 150, D-44780 Bochum, Germany
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    • Arne Ludwig
      Arne Ludwig
      Lehrstuhl für Angewandte Festkörperphysik, Ruhr-Universität Bochum, Universitätsstrasse 150, D-44780 Bochum, Germany
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    • Matthias C. Löbl
      Matthias C. Löbl
      Department of Physics, University of Basel, Klingelbergstrasse 82, CH-4056 Basel, Switzerland
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    • Immo Söllner
      Immo Söllner
      Department of Physics, University of Basel, Klingelbergstrasse 82, CH-4056 Basel, Switzerland
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    • Richard J. Warburton
      Richard J. Warburton
      Department of Physics, University of Basel, Klingelbergstrasse 82, CH-4056 Basel, Switzerland
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    • Peter Lodahl*
      Peter Lodahl
      Niels Bohr Institute, University of Copenhagen, Blegdamsvej 17, DK-2100 Copenhagen, Denmark
      *E-mail: [email protected]. Phone: +4535325306.
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    Nano Letters

    Cite this: Nano Lett. 2018, 18, 3, 1801–1806
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    https://doi.org/10.1021/acs.nanolett.7b05016
    Published March 1, 2018
    Copyright © 2018 American Chemical Society
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    Abstract

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    Establishing a highly efficient photon-emitter interface where the intrinsic linewidth broadening is limited solely by spontaneous emission is a key step in quantum optics. It opens a pathway to coherent light–matter interaction for, e.g., the generation of highly indistinguishable photons, few-photon optical nonlinearities, and photon-emitter quantum gates. However, residual broadening mechanisms are ubiquitous and need to be combated. For solid-state emitters charge and nuclear spin noise are of importance, and the influence of photonic nanostructures on the broadening has not been clarified. We present near-lifetime-limited linewidths for quantum dots embedded in nanophotonic waveguides through a resonant transmission experiment. It is found that the scattering of single photons from the quantum dot can be obtained with an extinction of 66 ± 4%, which is limited by the coupling of the quantum dot to the nanostructure rather than the linewidth broadening. This is obtained by embedding the quantum dot in an electrically contacted nanophotonic membrane. A clear pathway to obtaining even larger single-photon extinction is laid out; i.e., the approach enables a fully deterministic and coherent photon-emitter interface in the solid state that is operated at optical frequencies.

    Copyright © 2018 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.nanolett.7b05016.

    • Additional calculations and figures including COMSOL images, coupling efficiency and emission enhancement as a function of emitter displacement, and electron microscope image of the entire nanophotonic device (PDF)

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    Cited By

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    This article is cited by 51 publications.

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    Nano Letters

    Cite this: Nano Lett. 2018, 18, 3, 1801–1806
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acs.nanolett.7b05016
    Published March 1, 2018
    Copyright © 2018 American Chemical Society
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