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Electronic Structure and Enhanced Charge-Density Wave Order of Monolayer VSe2

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Download Hi-Res ImageDownload to MS-PowerPointCite This:Nano Lett. 2018, 18, 7, 4493-4499
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    Electronic Structure and Enhanced Charge-Density Wave Order of Monolayer VSe2
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    • Jiagui Feng
      Jiagui Feng
      SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom
      Suzhou Institute of Nano-Technology and Nanobionics (SINANO), CAS, 398 Ruoshui Road, SEID, SIP, Suzhou 215123, China
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      Deepnarayan Biswas
      SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom
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      Akhil Rajan
      SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom
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      Matthew D. Watson
      SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom
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      Federico Mazzola
      SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom
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      Oliver J. Clark
      SUPA, School of Physics and Astronomy, University of St. Andrews, St. Andrews KY16 9SS, United Kingdom
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      Max Planck Institute for Chemical Physics of Solids, Nöthnitzer Straße 40, 01187 Dresden, Germany
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      David M. Burn
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      Department of Physics, University of Warwick, Coventry CV4 7AL, United Kingdom
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    Nano Letters

    Cite this: Nano Lett. 2018, 18, 7, 4493–4499
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    https://doi.org/10.1021/acs.nanolett.8b01649
    Published June 18, 2018
    Copyright © 2018 American Chemical Society
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    Abstract

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    How the interacting electronic states and phases of layered transition-metal dichalcogenides evolve when thinned to the single-layer limit is a key open question in the study of two-dimensional materials. Here, we use angle-resolved photoemission to investigate the electronic structure of monolayer VSe2 grown on bilayer graphene/SiC. While the global electronic structure is similar to that of bulk VSe2, we show that, for the monolayer, pronounced energy gaps develop over the entire Fermi surface with decreasing temperature below Tc = 140 ± 5 K, concomitant with the emergence of charge-order superstructures evident in low-energy electron diffraction. These observations point to a charge-density wave instability in the monolayer that is strongly enhanced over that of the bulk. Moreover, our measurements of both the electronic structure and of X-ray magnetic circular dichroism reveal no signatures of a ferromagnetic ordering, in contrast to the results of a recent experimental study as well as expectations from density functional theory. Our study thus points to a delicate balance that can be realized between competing interacting states and phases in monolayer transition-metal dichalcogenides.

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acs.nanolett.8b01649.

    • Figures showing equivalent measurements to those shown in the main text for samples grown on HOPG substrates and additional growth and materials characterization from reflection high-energy electron diffraction and atomic force microscopy. (PDF)

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    Cited By

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    This article is cited by 205 publications.

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    Cite this: Nano Lett. 2018, 18, 7, 4493–4499
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