A Rare Earth Metal Catalyzed Aerobic Dehydrogenation of N-Heterocycles
- Ting ZhangTing ZhangInstitute of Advanced Synthesis, School of Chemistry and Molecular Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University, Nanjing, 211816, ChinaMore by Ting Zhang
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- Yongheng LvYongheng LvInstitute of Advanced Synthesis, School of Chemistry and Molecular Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University, Nanjing, 211816, ChinaMore by Yongheng Lv
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- Zhenguo ZhangZhenguo ZhangDivision of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore, 637371, SingaporeMore by Zhenguo Zhang
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- Zhenhua Jia*Zhenhua Jia*Email: [email protected]Institute of Advanced Synthesis, School of Chemistry and Molecular Engineering, Jiangsu National Synergetic Innovation Center for Advanced Materials, Nanjing Tech University, Nanjing, 211816, ChinaMore by Zhenhua Jia
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- Teck-Peng Loh*Teck-Peng Loh*Email: [email protected]Division of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, Singapore, 637371, SingaporeMore by Teck-Peng Loh
Abstract
Rare earth metals exhibit high catalytic activity and selectivity in various organic reactions due to their unique electronic properties. Among them, praseodymium has shown high catalytic activity under mild reaction conditions compared with transitional metals. Here, we report a strategy of Pr-catalyzed aerobic dehydrogenative aromatization of saturated N-heterocycles to produce 7 classes of products with a broad substrate scope.
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