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Enhanced Uptake and Endosomal Release of LbL Microcarriers Functionalized with Reversible Fusion Proteins
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    Enhanced Uptake and Endosomal Release of LbL Microcarriers Functionalized with Reversible Fusion Proteins
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    • Kira Scheffler
      Kira Scheffler
      Institute for Medical Physics and Biophysics, Faculty of Medicine, University of Leipzig, D-04107 Leipzig, Germany
    • Nicole C. Bilz
      Nicole C. Bilz
      Institute of Virology, Faculty of Medicine, University of Leipzig, 04103 Leipzig, Germany
    • Mandy Brueckner
      Mandy Brueckner
      Institute for Medical Physics and Biophysics, Faculty of Medicine, University of Leipzig, D-04107 Leipzig, Germany
    • Megan L. Stanifer
      Megan L. Stanifer
      Schaller Research Group at CellNetworks, Department of Infectious Diseases, Virology, Heidelberg University Hospital, 69120 Heidelberg, Germany
    • Steeve Boulant
      Steeve Boulant
      Schaller Research Group at CellNetworks, Department of Infectious Diseases, Virology, Heidelberg University Hospital, 69120 Heidelberg, Germany
      Research Group “Cellular Polarity and Viral Infection” (F140), German Cancer Research Center (DKFZ), 69120 Heidelberg, Germany
    • Claudia Claus
      Claudia Claus
      Institute of Virology, Faculty of Medicine, University of Leipzig, 04103 Leipzig, Germany
    • Uta Reibetanz*
      Uta Reibetanz
      Institute for Medical Physics and Biophysics, Faculty of Medicine, University of Leipzig, D-04107 Leipzig, Germany
      *E-mail: [email protected]
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    ACS Applied Bio Materials

    Cite this: ACS Appl. Bio Mater. 2020, 3, 3, 1553–1567
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    https://doi.org/10.1021/acsabm.9b01168
    Published February 6, 2020
    Copyright © 2020 American Chemical Society

    Abstract

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    The efficient application of smart drug-delivery systems requires further improvement of their cellular uptake and in particular their release from endolysosomal compartments into the cytoplasm of target cells. The usage of virus proteins allows for such developments, as viruses have evolved efficient entry mechanisms into the cell, mediated by their fusion proteins. In our investigations, the transferability of the glycoprotein G which is a fusion protein of the vesicular stomatitis virus (VSV-G) onto the surface of a layer-by-layer (LbL) designed microcarrier was investigated. The assembly of VSV-G as a reversible viral fusion protein onto LbL microcarriers indeed induced an enhanced uptake rate on Vero cells as well as a fast and efficient release of the intact carriers from endolysosomes into the cytoplasm. Additionally, neither virus-associated effects on cellular viability nor activation of an interferon response were detected. Our study emphasizes the suitability of VSV-G as an efficient surface functionalization of drug-delivery systems.

    Copyright © 2020 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acsabm.9b01168.

    • Quantification of the lipid bilayer within cells, chemical stability of the fluorescent lipid label, the influence of covered and uncovered SiO2 microparticles on apoptosis, two different forms of intracellular progress of the lipid bilayer, the fusion of the VSV microcarriers with the endolysosomal membrane, CLSM images of the time-dependent processing of the lipid bilayer and the endolysosomal release of VSV-LbL and SLB-LbL microcarriers, endosomal acidification-dependent transport of microparticles with VSV surface functionalization to nucleus (PDF)

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    Cited By

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    This article is cited by 5 publications.

    1. Daniel B. Lawrence, Jordan A. Greco, Robert R. Birge, Nicole L. Wagner. Layer‐by‐Layer Deposition in Microgravity for Enhanced Thin‐Film Production. 2022, 285-301. https://doi.org/10.1002/9783527830909.ch15
    2. E. Barchiesi, T. Wareing, L. Desmond, A. N. Phan, P. Gentile, G. Pontrelli. Characterization of the Shells in Layer-By-Layer Nanofunctionalized Particles: A Computational Study. Frontiers in Bioengineering and Biotechnology 2022, 10 https://doi.org/10.3389/fbioe.2022.888944
    3. Huimin Gao, Pengpeng Hu, Gaoqi Sun, Lei Wang, Yu Tian, Hong Mo, Cheng Liu, Jun Zhang, Jian Shen. Decellularized scaffold-based poly(ethylene glycol) biomimetic vascular patches modified with polyelectrolyte multilayer of heparin and chitosan: preparation and vascular tissue engineering applications in a porcine model. Journal of Materials Chemistry B 2022, 10 (7) , 1077-1084. https://doi.org/10.1039/D1TB02631C
    4. Anna S. Vikulina, Jack Campbell. Biopolymer-Based Multilayer Capsules and Beads Made via Templating: Advantages, Hurdles and Perspectives. Nanomaterials 2021, 11 (10) , 2502. https://doi.org/10.3390/nano11102502
    5. Claudia Claus, Robert Fritz, Erik Schilling, Uta Reibetanz. The Metabolic Response of Various Cell Lines to Microtubule-Driven Uptake of Lipid- and Polymer-Coated Layer-by-Layer Microcarriers. Pharmaceutics 2021, 13 (9) , 1441. https://doi.org/10.3390/pharmaceutics13091441

    ACS Applied Bio Materials

    Cite this: ACS Appl. Bio Mater. 2020, 3, 3, 1553–1567
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsabm.9b01168
    Published February 6, 2020
    Copyright © 2020 American Chemical Society

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