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High Spin to Charge Conversion Efficiency in Electron Beam-Evaporated Topological Insulator Bi2Se3

  • Braj Bhusan Singh*
    Braj Bhusan Singh
    Laboratory for Nanomagnetism and Magnetic Materials (LNMM), School of Physical Sciences, National Institute of Science Education and Research (NISER), HBNI, Jatni, Khurda 752050, India
    *Email: [email protected]
  • Sukanta Kumar Jena
    Sukanta Kumar Jena
    Laboratory for Nanomagnetism and Magnetic Materials (LNMM), School of Physical Sciences, National Institute of Science Education and Research (NISER), HBNI, Jatni, Khurda 752050, India
  • Manisha Samanta
    Manisha Samanta
    New Chemistry Unit, Jawaharlal Nehru Centre for Advanced Scientific Research, Jakkur, Bangalore 560064, India
  • Kanishka Biswas
    Kanishka Biswas
    New Chemistry Unit, Jawaharlal Nehru Centre for Advanced Scientific Research, Jakkur, Bangalore 560064, India
  • , and 
  • Subhankar Bedanta*
    Subhankar Bedanta
    Laboratory for Nanomagnetism and Magnetic Materials (LNMM), School of Physical Sciences, National Institute of Science Education and Research (NISER), HBNI, Jatni, Khurda 752050, India
    *Email: [email protected]
Cite this: ACS Appl. Mater. Interfaces 2020, 12, 47, 53409–53415
Publication Date (Web):November 16, 2020
https://doi.org/10.1021/acsami.0c13540
Copyright © 2020 American Chemical Society

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    Abstract

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    Bi2Se3 is a well-established topological insulator (TI) having spin momentum locked Dirac surface states at room temperature and predicted to exhibit high spin to charge conversion efficiency (SCCE) for spintronics applications. The SCCE in TIs is characterized by an inverse Edelstein effect length (λIREE). We report an λIREE of ∼0.36 nm, which is the highest ever observed in Bi2Se3. Here, we performed spin pumping and inverse spin Hall effect (ISHE) in an electron beam-evaporated Bi2Se3/CoFeB bilayer. The Bi2Se3 thickness dependence of λIREE, perpendicular surface anisotropy (KS), spin mixing conductance, and spin Hall angle confirmed that spin to charge conversion is due to spin momentum locked Dirac surface states. We propose that the role of surface states in SCCE can be understood by the evaluation of KS. The SCCE is found to be high when the value of KS is small.

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    16. Rik Dey, Anupam Roy, Leonard F. Register, Sanjay K. Banerjee. Recent progress on measurement of spin–charge interconversion in topological insulators using ferromagnetic resonance. APL Materials 2021, 9 (6) https://doi.org/10.1063/5.0049887

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