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    Research Article

    Control of Triboelectrification by Engineering Surface Dipole and Surface Electronic State
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    † Samsung Advanced Institute of Technology, Suwon 443-803, Republic of Korea
    ‡ School of Advanced Materials Science and Engineering, Sungkyunkwan University (SKKU), Suwon 440−746, Republic of Korea
    *E-mail: [email protected]
    *E-mail: [email protected]
    *E-mail: [email protected]
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    ACS Applied Materials & Interfaces

    Cite this: ACS Appl. Mater. Interfaces 2016, 8, 28, 18519–18525
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    https://doi.org/10.1021/acsami.6b02802
    Published June 24, 2016
    Copyright © 2016 American Chemical Society
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    Abstract

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    Although triboelectrification is a well-known phenomenon, fundamental understanding of its principle on a material surface has not been studied systematically. Here, we demonstrated that the surface potential, especially the surface dipoles and surface electronic states, governed the triboelectrification by controlling the surface with various electron-donating and -withdrawing functional groups. The functional groups critically affected the surface dipoles and surface electronic states followed by controlling the amount of and even the polarity of triboelectric charges. As a result, only one monolayer with a thickness of less than 1 nm significantly changed the conventional triboelectric series. First-principles simulations confirmed the atomistic origins of triboelectric charges and helped elucidate the triboelectrification mechanism. The simulation also revealed for the first time where charges are retained after triboelectrification. This study provides new insights to understand triboelectrification.

    Copyright © 2016 American Chemical Society

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    • Diffusion of triboelectric charges on various surfaces, triboelectrification in air, triboelectrification of CH3–SiO2 with different carbon chain length, unit cell used in density of functional theory calculations, and output voltage between SAM-modified substrates and the counter materials (PDF)

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    Cite this: ACS Appl. Mater. Interfaces 2016, 8, 28, 18519–18525
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