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Graphene Oxides Used as a New “Dual Role” Binder for Stabilizing Silicon Nanoparticles in Lithium-Ion Battery

  • Changsheng Shan*
    Changsheng Shan
    Physical Chemistry and Applied Spectroscopy (C-PCS), Chemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, United States
    *E-mail: [email protected]
    More by Changsheng Shan
  • , 
  • Kaifeng Wu
    Kaifeng Wu
    State Key Laboratory of Molecular Reaction Dynamics, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian 116023, China
    More by Kaifeng Wu
  • , 
  • Hung-Ju Yen
    Hung-Ju Yen
    Physical Chemistry and Applied Spectroscopy (C-PCS), Chemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, United States
    Institute of Chemistry, Academia Sinica, 128 Academia Road, Section 2, Nankang, Taipei 11529, Taiwan
    More by Hung-Ju Yen
  • , 
  • Claudia Narvaez Villarrubia
    Claudia Narvaez Villarrubia
    Physical Chemistry and Applied Spectroscopy (C-PCS), Chemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, United States
    More by Claudia Narvaez Villarrubia
  • , 
  • Tom Nakotte
    Tom Nakotte
    Physical Chemistry and Applied Spectroscopy (C-PCS), Chemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, United States
    More by Tom Nakotte
  • , 
  • Xiangjie Bo
    Xiangjie Bo
    Key Laboratory of Nanobiosensing and Nanobioanalysis at Universities of Jilin Province, Key Laboratory of Polyoxometalate Science of Ministry of Education, National & Local United Engineering Laboratory for Power Batteries, Department of Chemistry, Northeast Normal University, Changchun, Jilin Province 130024, P.R. China
    More by Xiangjie Bo
    Orcidhttp://orcid.org/0000-0002-0407-0976
  • , 
  • Ming Zhou
    Ming Zhou
    Key Laboratory of Nanobiosensing and Nanobioanalysis at Universities of Jilin Province, Key Laboratory of Polyoxometalate Science of Ministry of Education, National & Local United Engineering Laboratory for Power Batteries, Department of Chemistry, Northeast Normal University, Changchun, Jilin Province 130024, P.R. China
    More by Ming Zhou
    Orcidhttp://orcid.org/0000-0003-2239-9342
  • , 
  • Gang Wu
    Gang Wu
    Department of Chemical and Biological Engineering, University at Buffalo, the State University of New York, Buffalo, New York 14260, United States
    More by Gang Wu
    Orcidhttp://orcid.org/0000-0003-0885-6172
  • , and 
  • Hsing-Lin Wang*
    Hsing-Lin Wang
    Physical Chemistry and Applied Spectroscopy (C-PCS), Chemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, United States
    Department of Materials Science and Engineering, Southern University of Science and Technology, Shenzhen, Guangdong 518055, China
    *E-mail: [email protected]
    More by Hsing-Lin Wang
    Orcidhttp://orcid.org/0000-0002-6379-0519
Cite this: ACS Appl. Mater. Interfaces 2018, 10, 18, 15665–15672
Publication Date (Web):April 23, 2018
https://doi.org/10.1021/acsami.8b00649
Copyright © 2018 American Chemical Society
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    Abstract

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    For the first time, we report that graphene oxide (GO) can be used as a new “dual-role” binder for Si nanoparticles (SiNPs)-based lithium-ion batteries (LIBs). GO not only provides a graphene-like porous 3D framework for accommodating the volume changes of SiNPs during charging/discharging cycles, but also acts as a polymer-like binder that forms strong chemical bonds with SiNPs through its Si–OH functional groups to trap and stabilize SiNPs inside the electrode. Leveraging this unique dual-role of GO binder, we fabricated GO/SiNPs electrodes with remarkably improved performances as compared to using the conventional polyvinylidene fluoride (PVDF) binder. Specifically, the GO/SiNPs electrode showed a specific capacity of 2400 mA h g–1 at the 50th cycle and 2000 mA h g–1 at the 100th cycle, whereas the SiNPs/PVDF electrode only showed 456 mAh g–1 at the 50th cycle and 100 mAh g–1 at 100th cycle. Moreover, the GO/SiNPs film maintained its structural integrity and formed a stable solid–electrolyte interphase (SEI) film after 100 cycles. These results, combined with the well-established facile synthesis of GO, indicate that GO can be an excellent binder for developing high performance Si-based LIBs.

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