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Full-Color Tunable Fluorescent and Chemiluminescent Supramolecular Nanoparticles for Anti-counterfeiting Inks

  • Minzan Zuo
    Minzan Zuo
    Key Laboratory of Mesoscopic Chemistry of MOE and Collaborative Innovation Center of Chemistry for Life Sciences, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, 210023, China
    More by Minzan Zuo
  • Weirui Qian
    Weirui Qian
    Key Laboratory of Mesoscopic Chemistry of MOE and Collaborative Innovation Center of Chemistry for Life Sciences, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, 210023, China
    More by Weirui Qian
  • Tinghan Li
    Tinghan Li
    Key Laboratory of Mesoscopic Chemistry of MOE and Collaborative Innovation Center of Chemistry for Life Sciences, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, 210023, China
    More by Tinghan Li
  • Xiao-Yu Hu*
    Xiao-Yu Hu
    Key Laboratory of Mesoscopic Chemistry of MOE and Collaborative Innovation Center of Chemistry for Life Sciences, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, 210023, China
    Applied Chemistry Department, School of Material Science and Engineering, Nanjing University of Aeronautics and Astronautics, Nanjing, 211100, China
    *E-mail: [email protected] (X.-Y.H.).
    More by Xiao-Yu Hu
  • Juli Jiang*
    Juli Jiang
    Key Laboratory of Mesoscopic Chemistry of MOE and Collaborative Innovation Center of Chemistry for Life Sciences, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, 210023, China
    *E-mail: [email protected] (J.J.).
    More by Juli Jiang
  • , and 
  • Leyong Wang*
    Leyong Wang
    Key Laboratory of Mesoscopic Chemistry of MOE and Collaborative Innovation Center of Chemistry for Life Sciences, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing, 210023, China
    School of Petrochemical Engineering, Changzhou University, Changzhou, 213164, China
    *E-mail: [email protected] (L.W.).
    More by Leyong Wang
Cite this: ACS Appl. Mater. Interfaces 2018, 10, 45, 39214–39221
Publication Date (Web):October 22, 2018
https://doi.org/10.1021/acsami.8b14110
Copyright © 2018 American Chemical Society
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Abstract

Abstract Image

A drive for anti-counterfeiting technology has attracted considerable interests in developing nanomaterials with a wide range of colors and tunable optical properties in solid state. Herein, with a series of conjugated polymers and based on the host–guest driven self-assembly strategy, a color-tunable supramolecular nanoparticle-based system is reported, in which full-color as well as white fluorescence can be achieved. Moreover, this fluorescent platform exhibits reversible photoswitching between quenching and emission by noncovalently introducing a photoresponsive energy acceptor. In addition, an efficient chemiluminescence system with high intensity can also be obtained in a similar manner by introducing a H2O2-responsive energy donor. Significantly, chemiluminescence is advantageous over fluorescence since there is no need for external light irradiation. More importantly, these acceptor/donor-loaded supramolecular nanoparticles exhibit fluorescence/chemiluminescence modulation ability in both solution and solid state. Therefore, this supramolecular system can be employed as fluorescent security inks for anti-counterfeiting strategies and provide a proof-of-principle application.

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The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acsami.8b14110.

  • Synthesis and relevant characterization details, and supporting photographs (PDF)

  • Supporting Movie 1: Video of the chemiluminescent nanoparticles in PBS solution (AVI)

  • Supporting Movie 2: Video of the chemiluminescent nanoparticles in aqueous solution (AVI)

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