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Three-Dimensional Printed Photoluminescent Polymeric Waveguides

  • Francesca Frascella
    Francesca Frascella
    Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino 10129, Italy
  • Gustavo González
    Gustavo González
    Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino 10129, Italy
    Center for Sustainable Future Technologies @Polito, Istituto Italiano di Tecnologia, Corso Trento 21, Torino 10129, Italy
  • Paula Bosch
    Paula Bosch
    Departamento de Química Macromolecular Aplicada, Instituto de Ciencia y Tecnología de Polímeros, Consejo Superior de Investigaciones Científicas (CSIC), C/Juan de la Cierva 3, Madrid 28006, Spain
    More by Paula Bosch
  • Angelo Angelini
    Angelo Angelini
    Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino 10129, Italy
  • Annalisa Chiappone
    Annalisa Chiappone
    Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino 10129, Italy
  • Marco Sangermano
    Marco Sangermano
    Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino 10129, Italy
  • Candido Fabrizio Pirri
    Candido Fabrizio Pirri
    Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino 10129, Italy
    Center for Sustainable Future Technologies @Polito, Istituto Italiano di Tecnologia, Corso Trento 21, Torino 10129, Italy
  • , and 
  • Ignazio Roppolo*
    Ignazio Roppolo
    Department of Applied Science and Technology, Politecnico di Torino, Corso Duca degli Abruzzi 24, Torino 10129, Italy
    *E-mail: [email protected]
Cite this: ACS Appl. Mater. Interfaces 2018, 10, 45, 39319–39326
Publication Date (Web):October 22, 2018
https://doi.org/10.1021/acsami.8b16036
Copyright © 2018 American Chemical Society

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    Abstract

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    In this work, we propose an innovative strategy for obtaining functional objects employing a light-activated three-dimensional (3D) printing process without affecting the materials’ printability. In particular, a dye is a necessary ingredient in a formulation for a digital light processing 3D printing method to obtain precise and complex structures. Here, we use a photoluminescent dye specifically synthesized for this purpose that enables the production of 3D printed waveguides and splitters able to guide the luminescence. Moreover, copolymerizing the dye with the polymeric network during the printing process, we are able to maintain the solvatochromic properties of the dye toward different solvents in the printed structures, enabling the development of solvents’ polarity sensors.

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acsami.8b16036.

    • Scheme of the optical setup, photorheology experiments, ATR spectra of the printed structures, evaluation of the printing precision, optical characterization of the 3D printed structures, and emission spectra of the printed structures in different solvents (PDF)

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