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Interfacing a Potential Purely Organic Molecular Quantum Bit with a Real-Life Surface

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    Research Article

    Interfacing a Potential Purely Organic Molecular Quantum Bit with a Real-Life Surface
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    • Francesca Ciccullo
      Francesca Ciccullo
      Institute of Physical and Theoretical Chemistry, University of Tübingen, 72076 Tübingen, Germany
      More by Francesca Ciccullo
    • Arrigo Calzolari
      Arrigo Calzolari
      CNR-NANO Istituto Nanoscienze, Centro S3, 41125 Modena, Italy
      More by Arrigo Calzolari
      Orcidhttp://orcid.org/0000-0002-0244-7717
    • Katharina Bader
      Katharina Bader
      Institute of Physical Chemistry, University of Stuttgart, 70569 Stuttgart, Germany
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    • Petr Neugebauer
      Petr Neugebauer
      Central European Institute of Technology, CEITEC BUT, Purkyňova 656/123, 61600 Brno, Czech Republic
      Institute of Physical Chemistry, University of Stuttgart, 70569 Stuttgart, Germany
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    • Nolan M. Gallagher
      Nolan M. Gallagher
      Department of Chemistry, University of Nebraska−Lincoln, Lincoln, Nebraska 68588-0304, United States
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    • Andrzej Rajca
      Andrzej Rajca
      Department of Chemistry, University of Nebraska−Lincoln, Lincoln, Nebraska 68588-0304, United States
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      Orcidhttp://orcid.org/0000-0002-8856-1536
    • Joris van Slageren
      Joris van Slageren
      Institute of Physical Chemistry, University of Stuttgart, 70569 Stuttgart, Germany
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    • Maria Benedetta Casu*
      Maria Benedetta Casu
      Institute of Physical and Theoretical Chemistry, University of Tübingen, 72076 Tübingen, Germany
      *E-mail: [email protected]
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      Orcidhttp://orcid.org/0000-0002-5659-7040
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    ACS Applied Materials & Interfaces

    Cite this: ACS Appl. Mater. Interfaces 2019, 11, 1, 1571–1578
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    https://doi.org/10.1021/acsami.8b16061
    Published December 6, 2018
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    Abstract

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    By using a multidisciplinary and multitechnique approach, we have addressed the issue of attaching a molecular quantum bit to a real surface. First, we demonstrate that an organic derivative of the pyrene–Blatter radical is a potential molecular quantum bit. Our study of the interface of the pyrene–Blatter radical with a copper-based surface reveals that the spin of the interface layer is not canceled by the interaction with the surface and that the Blatter radical is resistant in presence of molecular water. Although the measured pyrene–Blatter derivative quantum coherence time is not the highest value known, this molecule is known as a “super stable” radical. Conversely, other potential qubits show poor thin film stability upon air exposure. Therefore, we discuss strategies to make molecular systems candidates as qubits competitive, bridging the gap between potential and real applications.

    Copyright © 2018 American Chemical Society

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    • Stoichiometric and experimental elemental ratios for a thicker film and fit results for energy position and relative intensities of the photoemission lines in the C 1s and N 1s spectra for a 78 and 14 Å nominally thick film, respectively, as shown in Figure 2. Relaxed atomic positions of molecule/surface interface resulting from total-energy-and-force optimization (PDF)

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    Cited By

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    This article is cited by 53 publications.

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    ACS Applied Materials & Interfaces

    Cite this: ACS Appl. Mater. Interfaces 2019, 11, 1, 1571–1578
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsami.8b16061
    Published December 6, 2018
    Copyright © 2018 American Chemical Society
    Request reuse permissions

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