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ACS Publications. Most Trusted. Most Cited. Most Read
FeNi Nanoparticles Embedded in Porous Nitrogen-Doped Graphene for Electrocatalytic Evolution of Hydrogen and Oxygen

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Download Hi-Res ImageDownload to MS-PowerPointCite This:ACS Appl. Nano Mater. 2020, 3, 7, 6336-6343
    Article

    FeNi Nanoparticles Embedded in Porous Nitrogen-Doped Graphene for Electrocatalytic Evolution of Hydrogen and Oxygen
    Click to copy article linkArticle link copied!

    • Haixu Wang
      Haixu Wang
      Key Laboratory of Nanobiosensing and Nanobioanalysis at Universities of Jilin Province, Faculty of Chemistry, Northeast Normal University, Changchun 130024, P. R. China
      More by Haixu Wang
    • Xiaogeng Feng
      Xiaogeng Feng
      Key Laboratory of Nanobiosensing and Nanobioanalysis at Universities of Jilin Province, Faculty of Chemistry, Northeast Normal University, Changchun 130024, P. R. China
      More by Xiaogeng Feng
    • Ming Zhou*
      Ming Zhou
      Key Laboratory of Nanobiosensing and Nanobioanalysis at Universities of Jilin Province, Faculty of Chemistry, Northeast Normal University, Changchun 130024, P. R. China
      Guangdong Provincial Key Laboratory of Energy Materials for Electric Power, Southern University of Science and Technology, Shenzhen 518055, Guangdong, China
      *M.Z.: email, [email protected]
      More by Ming Zhou
      Orcidhttp://orcid.org/0000-0003-2239-9342
    • Xiangjie Bo*
      Xiangjie Bo
      Key Laboratory of Nanobiosensing and Nanobioanalysis at Universities of Jilin Province, Faculty of Chemistry, Northeast Normal University, Changchun 130024, P. R. China
      *X.B.: email, [email protected]
      More by Xiangjie Bo
      Orcidhttp://orcid.org/0000-0002-0407-0976
    • Liping Guo*
      Liping Guo
      Key Laboratory of Nanobiosensing and Nanobioanalysis at Universities of Jilin Province, Faculty of Chemistry, Northeast Normal University, Changchun 130024, P. R. China
      *L.G.: email, [email protected]
      More by Liping Guo
      Orcidhttp://orcid.org/0000-0003-2065-387X
    Other Access OptionsSupporting Information (1)

    ACS Applied Nano Materials

    Cite this: ACS Appl. Nano Mater. 2020, 3, 7, 6336–6343
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    https://doi.org/10.1021/acsanm.0c00619
    Published July 1, 2020
    Copyright © 2020 American Chemical Society
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    Abstract

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    The thermal annealing method is regarded as a general and promising method for preparation of carbon-based electrocatalysts. However, this method always suffers from complex and harsh preparative conditions, such as high pyrolysis temperature, protective gas environment, and long synthesis period. Herein, a laser engraving method is introduced for preparation of porous nitrogen-doped graphene layer-enclosed FeNi nanoparticles (FeNi/PNGs), starting with metal organic frameworks (MOFs) as precursors. All the steps were quickly achieved at room temperature and in air environment. Another attractive feature of this method is that FeNi/PNG supported on polyamide (PI) film could directly act as electrocatalytic electrode for hydrogen (HER) and oxygen evolution reaction (OER) without the involvement of dispersion and drop-casting of electrocatalyst ink. The FeNi/PNG shows overpotentials of 132 and 353 mV with Tafel slope of 94 and 80 mV dec–1 for HER and OER catalyses, respectively. This simple and convenient method could be extended to other catalytic systems with carbon-based materials as electrocatalysts.

    Copyright © 2020 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acsanm.0c00619.

    • Details of apparatus and electrochemical measurements, Figures S1–S14, and Table S1 (PDF)

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    Cited By

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    This article is cited by 19 publications.

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    ACS Applied Nano Materials

    Cite this: ACS Appl. Nano Mater. 2020, 3, 7, 6336–6343
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsanm.0c00619
    Published July 1, 2020
    Copyright © 2020 American Chemical Society
    Request reuse permissions

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