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Reaction-Mediated Transformation of Working Catalysts

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Download Hi-Res ImageDownload to MS-PowerPointCite This:ACS Catal. 2022, 12, 13, 8007-8018
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    Reaction-Mediated Transformation of Working Catalysts
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    • Gang Wan*
      Gang Wan
      SLAC National Accelerator Laboratory, Menlo Park, California 94025, United States
      *Email for G.W.: [email protected]
      More by Gang Wan
      Orcidhttps://orcid.org/0000-0003-1658-5376
    • Guanghui Zhang*
      Guanghui Zhang
      State Key Laboratory of Fine Chemicals, PSU-DUT Joint Center for Energy Research, School of Chemical Engineering, Dalian University of Technology, Dalian 116024, People’s Republic of China
      Davidson School of Chemical Engineering, Purdue University, West Lafayette, Indiana 47907, United States
      *Email for G.Z.: [email protected]
      More by Guanghui Zhang
      Orcidhttps://orcid.org/0000-0002-5854-6909
    • Johnny Zhu Chen
      Johnny Zhu Chen
      Davidson School of Chemical Engineering, Purdue University, West Lafayette, Indiana 47907, United States
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    • Michael F. Toney*
      Michael F. Toney
      Department of Chemical and Biological Engineering, University of Colorado Boulder, Boulder, Colorado 80309, United States
      *Email for M.F.T.: [email protected]
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    • Jeffrey T. Miller*
      Jeffrey T. Miller
      Davidson School of Chemical Engineering, Purdue University, West Lafayette, Indiana 47907, United States
      *Email for J.T.M.: [email protected]
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    • Christopher J. Tassone*
      Christopher J. Tassone
      SLAC National Accelerator Laboratory, Menlo Park, California 94025, United States
      *Email for C.J.T.: [email protected]
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    ACS Catalysis

    Cite this: ACS Catal. 2022, 12, 13, 8007–8018
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    https://doi.org/10.1021/acscatal.2c01838
    Published June 21, 2022
    Copyright © 2022 American Chemical Society
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    Abstract

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    Catalytic transformations are critical in a variety of thermal and electrochemical processes, including fuel and chemical generation, energy conversion, and decarbonization. Historically, various static assessment factors have been used to examine a wide range of catalytic materials. Surface, interfacial, and nanoscale phenomena have been seen in various catalytic disciplines, which are crucial to major applications. These phenomena sparked extensive discussions on how catalysts operate for reactions and adapt to working environments. With this recognition, the goal of this review is to go beyond the traditional static analysis of working catalysts and provide a perspective on the dynamic insights into structural and redox transformations at catalytic surfaces and electrified interfaces. The correlation between the transformation of working catalysts and their catalytic performance is examined, shedding light on understanding and controlling catalyst redox and structure evolution under operating conditions with properties tailored to thermochemical and electrocatalytic processes.

    Copyright © 2022 American Chemical Society

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    Cited By

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    This article is cited by 4 publications.

    1. Xiaoyu Li, Jinling Cheng, Huaming Hou, Debora M. Meira, Lichen Liu. Reactant-Induced Structural Evolution of Pt Catalysts Confined in Zeolite. JACS Au 2024, 4 (2) , 666-679. https://doi.org/10.1021/jacsau.3c00732
    2. Yao Nian, Xinyuan Huang, Menghui Liu, Jinli Zhang, You Han. Insight into the Dynamic Evolution of Supported Metal Catalysts by In Situ/Operando Techniques and Theoretical Simulations. ACS Catalysis 2023, 13 (16) , 11164-11171. https://doi.org/10.1021/acscatal.3c02370
    3. Steven Chavez, Baraa Werghi, Kenzie M. Sanroman Gutierrez, Ruitian Chen, Supriya Lall, Matteo Cargnello. Studying, Promoting, Exploiting, and Predicting Catalyst Dynamics: the Next Frontier in Heterogeneous Catalysis. The Journal of Physical Chemistry C 2023, 127 (5) , 2127-2146. https://doi.org/10.1021/acs.jpcc.2c06519
    4. Yi Liu, Guanghui Zhang, Shida Liu, Jie Zhu, Jiaxu Liu, Jianyang Wang, Rongtan Li, Mingrui Wang, Qiang Fu, Shuandi Hou, Chunshan Song, Xinwen Guo. Promoting n-Butane Dehydrogenation over PtMn/SiO2 through Structural Evolution Induced by a Reverse Water-Gas Shift Reaction. ACS Catalysis 2022, 12 (21) , 13506-13512. https://doi.org/10.1021/acscatal.2c04471
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    ACS Catalysis

    Cite this: ACS Catal. 2022, 12, 13, 8007–8018
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acscatal.2c01838
    Published June 21, 2022
    Copyright © 2022 American Chemical Society
    Request reuse permissions

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