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Broad Tunability of Carrier Effective Masses in Two-Dimensional Halide Perovskites

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    Broad Tunability of Carrier Effective Masses in Two-Dimensional Halide Perovskites
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    • Mateusz Dyksik
      Mateusz Dyksik
      Laboratoire National des Champs Magnétiques Intenses, UPR 3228, CNRS-UGA-UPS-INSA, Grenoble and Toulouse, France
      Department of Experimental Physics, Faculty of Fundamental Problems of Technology, Wroclaw University of Science and Technology, Wroclaw, Poland
      More by Mateusz Dyksik
    • Herman Duim
      Herman Duim
      Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen, The Netherlands
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    • Xiangzhou Zhu
      Xiangzhou Zhu
      Department of Physics, Technical University of Munich, 85748 Garching, Germany
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    • Zhuo Yang
      Zhuo Yang
      The Institute for Solid State Physics, The University of Tokyo, Kashiwanoha 5-1-5, Kashiwa, Chiba, Japan
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    • Masaki Gen
      Masaki Gen
      The Institute for Solid State Physics, The University of Tokyo, Kashiwanoha 5-1-5, Kashiwa, Chiba, Japan
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    • Yoshimitsu Kohama
      Yoshimitsu Kohama
      The Institute for Solid State Physics, The University of Tokyo, Kashiwanoha 5-1-5, Kashiwa, Chiba, Japan
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    • Sampson Adjokatse
      Sampson Adjokatse
      Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen, The Netherlands
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    • Duncan K. Maude
      Duncan K. Maude
      Laboratoire National des Champs Magnétiques Intenses, UPR 3228, CNRS-UGA-UPS-INSA, Grenoble and Toulouse, France
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    • Maria Antonietta Loi*
      Maria Antonietta Loi
      Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen, The Netherlands
      *[email protected]
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      Orcidhttp://orcid.org/0000-0002-7985-7431
    • David A. Egger*
      David A. Egger
      Department of Physics, Technical University of Munich, 85748 Garching, Germany
      *[email protected]
      More by David A. Egger
      Orcidhttp://orcid.org/0000-0001-8424-902X
    • Michal Baranowski*
      Michal Baranowski
      Department of Experimental Physics, Faculty of Fundamental Problems of Technology, Wroclaw University of Science and Technology, Wroclaw, Poland
      *[email protected]
      More by Michal Baranowski
      Orcidhttp://orcid.org/0000-0002-5974-0850
    • Paulina Plochocka*
      Paulina Plochocka
      Laboratoire National des Champs Magnétiques Intenses, UPR 3228, CNRS-UGA-UPS-INSA, Grenoble and Toulouse, France
      Department of Experimental Physics, Faculty of Fundamental Problems of Technology, Wroclaw University of Science and Technology, Wroclaw, Poland
      *[email protected]
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      Orcidhttp://orcid.org/0000-0002-4019-6138
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    ACS Energy Letters

    Cite this: ACS Energy Lett. 2020, 5, 11, 3609–3616
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    https://doi.org/10.1021/acsenergylett.0c01758
    Published October 27, 2020
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    Abstract

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    The effective mass of charge carriers is a crucial parameter for the design of any optoelectronic device. The estimated values of the effective mass of 2D halide perovskites currently span a broad range, providing an unwelcome source of confusion in this promising material system. Here we highlight how the distortion imposed by the organic spacers, and orbital hybridization effects by the metal cation, govern the effective mass. As a result, the effective mass in 2D halide perovskites can be easily tailored over a wide range. To demonstrate this, we have directly measured the reduced effective mass of charge carriers in phenethylamine (PEA)-based 2D halide perovskites. Combining the experimental results with electronic band-structure calculations, we propose a scaling diagram for the effective mass value versus the distortion of the octahedra imposed by the organic cations.

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    • Transmission spectra of (PEA)2SnI4 in magnetic field, band gap determination for (PEA)2SnI4 and (PEA)2PbI4, reflection spectra of FASnI3 in magnetic field, and temperature dependence of transmission spectra of (PEA)2SnI4 and (PEA)2PbI4 (PDF)

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    Cite this: ACS Energy Lett. 2020, 5, 11, 3609–3616
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