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Rechargeable Aqueous Zn–V2O5 Battery with High Energy Density and Long Cycle Life

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    Rechargeable Aqueous Zn–V2O5 Battery with High Energy Density and Long Cycle Life
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    • Ning Zhang*
      Ning Zhang
      College of Chemistry & Environmental Science, Key Laboratory of Medicinal Chemistry and Molecular Diagnosis (Ministry of Education), Hebei University, Baoding 071002, China
      Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry, Nankai University, Tianjin 300071, China
      *E-mail: [email protected]
      More by Ning Zhang
      Orcidhttp://orcid.org/0000-0002-6176-7278
    • Yang Dong
      Yang Dong
      College of Chemistry & Environmental Science, Key Laboratory of Medicinal Chemistry and Molecular Diagnosis (Ministry of Education), Hebei University, Baoding 071002, China
      More by Yang Dong
    • Ming Jia
      Ming Jia
      College of Chemistry & Environmental Science, Key Laboratory of Medicinal Chemistry and Molecular Diagnosis (Ministry of Education), Hebei University, Baoding 071002, China
      More by Ming Jia
    • Xu Bian
      Xu Bian
      College of Chemistry & Environmental Science, Key Laboratory of Medicinal Chemistry and Molecular Diagnosis (Ministry of Education), Hebei University, Baoding 071002, China
      More by Xu Bian
    • Yuanyuan Wang
      Yuanyuan Wang
      College of Chemistry & Environmental Science, Key Laboratory of Medicinal Chemistry and Molecular Diagnosis (Ministry of Education), Hebei University, Baoding 071002, China
      More by Yuanyuan Wang
    • Mande Qiu
      Mande Qiu
      College of Chemistry & Environmental Science, Key Laboratory of Medicinal Chemistry and Molecular Diagnosis (Ministry of Education), Hebei University, Baoding 071002, China
      More by Mande Qiu
    • Jianzhong Xu
      Jianzhong Xu
      College of Chemistry & Environmental Science, Key Laboratory of Medicinal Chemistry and Molecular Diagnosis (Ministry of Education), Hebei University, Baoding 071002, China
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    • Yongchang Liu*
      Yongchang Liu
      Institute for Advanced Materials and Technology, University of Science and Technology Beijing, Beijing 100083, China
      Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry, Nankai University, Tianjin 300071, China
      *E-mail: [email protected]
      More by Yongchang Liu
    • Lifang Jiao
      Lifang Jiao
      Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry, Nankai University, Tianjin 300071, China
      More by Lifang Jiao
      Orcidhttp://orcid.org/0000-0002-4676-997X
    • Fangyi Cheng
      Fangyi Cheng
      Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry, Nankai University, Tianjin 300071, China
      More by Fangyi Cheng
      Orcidhttp://orcid.org/0000-0002-9400-1500
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    ACS Energy Letters

    Cite this: ACS Energy Lett. 2018, 3, 6, 1366–1372
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    https://doi.org/10.1021/acsenergylett.8b00565
    Published May 16, 2018
    Copyright © 2018 American Chemical Society
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    Abstract

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    We report an aqueous Zn–V2O5 battery chemistry employing commercial V2O5 cathode, Zn anode, and 3 M Zn(CF3SO3)2 electrolyte. We elucidate the Zn-storage mechanism in the V2O5 cathode to be that hydrated Zn2+ can reversibly (de)intercalate through the layered structure. The function of the co-intercalated H2O is revealed to be shielding the electrostatic interactions between Zn2+ and the host framework, accounting for the enhanced kinetics. In addition, the pristine bulk V2O5 gradually evolves into porous nanosheets upon cycling, providing more active sites for Zn2+ storage and thus rendering an initial capacity increase. As a consequence, a reversible capacity of 470 mAh g–1 at 0.2 A g–1 and a long-term cyclability with 91.1% capacity rentention over 4000 cycles at 5 A g–1 are achieved. The combination of the good battery performance, safety, scalable materials synthesis, and facile cell assembly indicates this aqueous Zn–V2O5 system is promising for stationary grid storage applications.

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acsenergylett.8b00565.

    • Experimental section, additional characterization of materials (XRD patterns, SEM images, TEM images, BET data, etc.), additional electrochemical performance (charge–discharge curves, GITT analysis, EIS profiles, cycling performance in diluted aqueous electrolyte and organic electrolyte, cyclability data at high and low temperatures (−10 and 50 °C), etc.) (PDF)

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    Cite this: ACS Energy Lett. 2018, 3, 6, 1366–1372
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