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Enhanced Photovoltaic Performance of FASnI3-Based Perovskite Solar Cells with Hydrazinium Chloride Coadditive

  • Md. Emrul Kayesh
    Md. Emrul Kayesh
    Photovoltaic Materials Group, Center for Green Research on Energy and Environmental Materials, National Institute for Materials Science (NIMS), 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan
    Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, Japan
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    • , 
  • Towhid H. Chowdhury
    Towhid H. Chowdhury
    Photovoltaic Materials Group, Center for Green Research on Energy and Environmental Materials, National Institute for Materials Science (NIMS), 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan
    More by Towhid H. Chowdhury
    Orcidhttp://orcid.org/0000-0001-8490-1276
    • , 
  • Kiyoto Matsuishi*
    Kiyoto Matsuishi
    Faculty of Pure and Applied Sciences, University of Tsukuba, Tsukuba, Ibaraki 305-8573, Japan
    *E-mail: [email protected]
    More by Kiyoto Matsuishi
    • , 
  • Ryuji Kaneko
    Ryuji Kaneko
    Photovoltaic Materials Group, Center for Green Research on Energy and Environmental Materials, National Institute for Materials Science (NIMS), 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan
    College of Science and Technology, Nihon University, 1-8-14 Kanda Surugadai, Chiyoda-ku, Tokyo, 101-8308, Japan
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    • , 
  • Said Kazaoui
    Said Kazaoui
    Research Center for Photovoltaics (RCPV), National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8565, Japan
    More by Said Kazaoui
    • , 
  • Jae-Joon Lee
    Jae-Joon Lee
    Department of Energy & Materials Engineering & Research Center for Photoenergy Harvesting and Conversion Technology, Dongguk University, Seoul 04620, Republic of Korea
    More by Jae-Joon Lee
    Orcidhttp://orcid.org/0000-0001-8966-0336
    • , 
  • Takeshi Noda
    Takeshi Noda
    Photovoltaic Materials Group, Center for Green Research on Energy and Environmental Materials, National Institute for Materials Science (NIMS), 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan
    More by Takeshi Noda
    • , and 
  • Ashraful Islam*
    Ashraful Islam
    Photovoltaic Materials Group, Center for Green Research on Energy and Environmental Materials, National Institute for Materials Science (NIMS), 1-2-1 Sengen, Tsukuba, Ibaraki 305-0047, Japan
    *E-mail: [email protected]
    More by Ashraful Islam
    Orcidhttp://orcid.org/0000-0002-1633-1432
Cite this: ACS Energy Lett. 2018, 3, 7, 1584–1589
Publication Date (Web):June 11, 2018
https://doi.org/10.1021/acsenergylett.8b00645
Copyright © 2018 American Chemical Society
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Abstract

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For the fabrication of efficient Sn-based perovskite solar cells (PSCs), deposition of uniform and pinhole-free perovskite films with low Sn4+ content remains a crucial factor. In this work, we present a coadditive engineering process by introduction of hydrazinium chloride (N2H5Cl) in a single precursor solvent system to fabricate FASnI3 perovskite films. The successful integration of N2H5Cl results in reduced concentration of Sn4+ content by 20% in the FASnI3 film leading to suppressed carrier recombination and pinhole-free uniform coverage. These remarkable improvements in the FASnI3 film results in power conversion efficiency (PCE) of Sn-based PSC up to 5.4% due to a significant increase in open-circuit voltage. Moreover, the best PSC without encapsulation showed stable shelf life up to 1000 h while retaining 65% of its initial PCE.

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This article is cited by 61 publications.

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