Dynamic Manipulation in Piezoresponse Force Microscopy: Creating Nonequilibrium Phases with Large Electromechanical ResponseClick to copy article linkArticle link copied!
- Kyle P. Kelley*Kyle P. Kelley*Email: [email protected]Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United StatesMore by Kyle P. Kelley
- Yao RenYao RenDepartment of Materials Science and Engineering, University of Texas at Arlington, Arlington, Texas 76019, United StatesMore by Yao Ren
- Anna N. MorozovskaAnna N. MorozovskaInstitute of Physics, National Academy of Science of Ukraine, Pr. Nauki 46, 03028 Kyiv, UkraineMore by Anna N. Morozovska
- Eugene A. EliseevEugene A. EliseevInstitute for Problems of Materials Science, National Academy of Science of Ukraine, Krjijanovskogo 3, 03142 Kyiv, UkraineMore by Eugene A. Eliseev
- Yoshitaka EharaYoshitaka EharaDepartment of Communications Engineering, National Defense Academy, Hashirimizu, Yokosuka, 239-8686, JapanDepartment of Material Science and Engineering, Tokyo Institute of Technology, Yokohama 226-8502, JapanMore by Yoshitaka Ehara
- Hiroshi FunakuboHiroshi FunakuboDepartment of Material Science and Engineering, Tokyo Institute of Technology, Yokohama 226-8502, JapanMore by Hiroshi Funakubo
- Thierry GiamarchiThierry GiamarchiDepartment of Quantum Matter Physics, University of Geneva, 24 Quai Ernest-Ansermet, CH-1211 Geneva, SwitzerlandMore by Thierry Giamarchi
- Nina BalkeNina BalkeCenter for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United StatesMore by Nina Balke
- Rama K. VasudevanRama K. VasudevanCenter for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United StatesMore by Rama K. Vasudevan
- Ye CaoYe CaoDepartment of Materials Science and Engineering, University of Texas at Arlington, Arlington, Texas 76019, United StatesMore by Ye Cao
- Stephen JesseStephen JesseCenter for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United StatesMore by Stephen Jesse
- Sergei V. Kalinin*Sergei V. Kalinin*Email: [email protected]Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United StatesMore by Sergei V. Kalinin
Abstract
Domain walls and topological defects in ferroelectric materials have emerged as a powerful tool for functional electronic devices including memory and logic. Similarly, wall interactions and dynamics underpin a broad range of mesoscale phenomena ranging from giant electromechanical responses to memory effects. Exploring the functionalities of individual domain walls, their interactions, and controlled modifications of the domain structures is crucial for applications and fundamental physical studies. However, the dynamic nature of these features severely limits studies of their local physics since application of local biases or pressures in piezoresponse force microscopy induce wall displacement as a primary response. Here, we introduce an approach for the control and modification of domain structures based on automated experimentation, whereby real-space image-based feedback is used to control the tip bias during ferroelectric switching, allowing for modification routes conditioned on domain states under the tip. This automated experiment approach is demonstrated for the exploration of domain wall dynamics and creation of metastable phases with large electromechanical response.
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