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Ultralow Threshold, Single-Mode InGaAs/GaAs Multiquantum Disk Nanowire Lasers
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    Article

    Ultralow Threshold, Single-Mode InGaAs/GaAs Multiquantum Disk Nanowire Lasers
    Click to copy article linkArticle link copied!

    • Xutao Zhang
      Xutao Zhang
      Key Laboratory of Light Field Manipulation and Information Acquisition, Ministry of Industry and Information Technology, and Shaanxi Key Laboratory of Optical Information Technology, School of Physical Science and Technology, Northwestern Polytechnical University, Xi’an 710129, China
      More by Xutao Zhang
    • Ruixuan Yi
      Ruixuan Yi
      Key Laboratory of Light Field Manipulation and Information Acquisition, Ministry of Industry and Information Technology, and Shaanxi Key Laboratory of Optical Information Technology, School of Physical Science and Technology, Northwestern Polytechnical University, Xi’an 710129, China
      More by Ruixuan Yi
    • Nikita Gagrani
      Nikita Gagrani
      Department of Electronic Materials Engineering, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
    • Ziyuan Li
      Ziyuan Li
      Department of Electronic Materials Engineering, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      More by Ziyuan Li
    • Fanlu Zhang
      Fanlu Zhang
      Department of Electronic Materials Engineering, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      More by Fanlu Zhang
    • Xuetao Gan*
      Xuetao Gan
      Key Laboratory of Light Field Manipulation and Information Acquisition, Ministry of Industry and Information Technology, and Shaanxi Key Laboratory of Optical Information Technology, School of Physical Science and Technology, Northwestern Polytechnical University, Xi’an 710129, China
      *(X.G.) Email: [email protected]
      More by Xuetao Gan
    • Xiaomei Yao
      Xiaomei Yao
      State Key Laboratory for Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, 500 Yutian Road, Shanghai 200083, China
      University of Chinese Academy of Sciences, 19 Yuquan Road, Beijing 100049, China
      More by Xiaomei Yao
    • Xiaoming Yuan
      Xiaoming Yuan
      Hunan Key Laboratory of Nanophotonics and Devices, School of Physics and Electronics, Central South University, 932 South Lushan Road, Changsha, Hunan 410083, P. R. China
    • Naiyin Wang
      Naiyin Wang
      Department of Electronic Materials Engineering, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      More by Naiyin Wang
    • Jianlin Zhao
      Jianlin Zhao
      Key Laboratory of Light Field Manipulation and Information Acquisition, Ministry of Industry and Information Technology, and Shaanxi Key Laboratory of Optical Information Technology, School of Physical Science and Technology, Northwestern Polytechnical University, Xi’an 710129, China
      More by Jianlin Zhao
    • Pingping Chen*
      Pingping Chen
      State Key Laboratory for Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, 500 Yutian Road, Shanghai 200083, China
      University of Chinese Academy of Sciences, 19 Yuquan Road, Beijing 100049, China
      *(P.C.) Email: [email protected]
    • Wei Lu*
      Wei Lu
      State Key Laboratory for Infrared Physics, Shanghai Institute of Technical Physics, Chinese Academy of Sciences, 500 Yutian Road, Shanghai 200083, China
      University of Chinese Academy of Sciences, 19 Yuquan Road, Beijing 100049, China
      School of Physical Science and Technology, ShanghaiTech University, 393 Middle Huaxia Road, Pudong District, Shanghai 201210, China
      *(W.L.) Email: [email protected]
      More by Wei Lu
    • Lan Fu
      Lan Fu
      Department of Electronic Materials Engineering, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      ARC Centre of Excellence for Transformative Meta-Optical Systems, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      More by Lan Fu
    • Hark Hoe Tan
      Hark Hoe Tan
      Department of Electronic Materials Engineering, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      ARC Centre of Excellence for Transformative Meta-Optical Systems, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      More by Hark Hoe Tan
    • Chennupati Jagadish
      Chennupati Jagadish
      Department of Electronic Materials Engineering, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
      ARC Centre of Excellence for Transformative Meta-Optical Systems, Research School of Physics, The Australian National University, Canberra, Australian Capital Territory 2601, Australia
    Other Access OptionsSupporting Information (1)

    ACS Nano

    Cite this: ACS Nano 2021, 15, 5, 9126–9133
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    https://doi.org/10.1021/acsnano.1c02425
    Published May 10, 2021
    Copyright © 2021 American Chemical Society

    Abstract

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    We present single-mode nanowire (NW) lasers with an ultralow threshold in the near-infrared spectral range. To ensure the single-mode operation, the NW diameter and length are reduced specifically to minimize the longitudinal and transverse modes of the NW cavity. Increased optical losses and reduced gain volume by the dimension reduction are compensated by an excellent NW morphology and InGaAs/GaAs multiquantum disks. At 5 K, a threshold low as 1.6 μJ/cm2 per pulse is achieved with a resulting quality factor exceeding 6400. By further passivating the NW with an AlGaAs shell to suppress surface nonradiative recombination, single-mode lasing operation is obtained with a threshold of only 48 μJ/cm2 per pulse at room temperature with a high characteristic temperature of 223 K and power output of ∼0.9 μW. These single-mode, ultralow threshold, high power output NW lasers are promising for the development of near-infrared nanoscale coherent light sources for integrated photonic circuits, sensing, and spectroscopy.

    Copyright © 2021 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acsnano.1c02425.

    • Normalized PL spectral mapping of the InGaAs QDs; energy-dispersive spectroscopy (EDS) analysis; schematic diagram of the experiment setup; transverse mode simulations; lasing power output measurement; emission spectra of a GaAs/InGaAs multi-QD NW; lasing characterization from two different GaAs/InGaAs multi-QD NWs; the spontaneous emission spectra under low pump fluence; lasing characterization from a GaAs/InGaAs multi-QDs NW at 180 K; emission spectra from a GaAs/InGaAs/AlGaAs multi-QD NW at different temperatures; simulations of the polarization dependence; mode hopping analysis; optical image from a GaAs/InGaAs/AlGaAs multi-QD NW; and growth conditions (PDF)

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    Cited By

    Click to copy section linkSection link copied!

    This article is cited by 14 publications.

    1. Ruixuan Yi, Xutao Zhang, Xiaoming Yuan, Jianguo Wang, Qiao Zhang, Yong Zhang, Liang Fang, Fanlu Zhang, Lan Fu, Hark Hoe Tan, Chennupati Jagadish, Jianlin Zhao, Xuetao Gan. Integrating a Semiconductor Nanowire Laser in a Silicon Nitride Waveguide. ACS Photonics 2024, 11 (6) , 2471-2479. https://doi.org/10.1021/acsphotonics.4c00393
    2. Xutao Zhang, Ruixuan Yi, Bijun Zhao, Chen Li, Li Li, Ziyuan Li, Fanlu Zhang, Naiyin Wang, Mingwen Zhang, Liang Fang, Jianlin Zhao, Pingping Chen, Wei Lu, Lan Fu, Hark Hoe Tan, Chennupati Jagadish, Xuetao Gan. Vertical Emitting Nanowire Vector Beam Lasers. ACS Nano 2023, 17 (11) , 10918-10924. https://doi.org/10.1021/acsnano.3c02786
    3. Ruixuan Yi, Xutao Zhang, Fanlu Zhang, Linpeng Gu, Qiao Zhang, Liang Fang, Jianlin Zhao, Lan Fu, Hark Hoe Tan, Chennupati Jagadish, Xuetao Gan. Integrating a Nanowire Laser in an on-Chip Photonic Waveguide. Nano Letters 2022, 22 (24) , 9920-9927. https://doi.org/10.1021/acs.nanolett.2c03364
    4. Zachary R. Lindsey, Malachi West, Peter Jacobson, John Robert Ray. Benchtop Electrochemical Growth and Controlled Alloying of Polycrystalline InxGa1–xAs Thin Films. Crystal Growth & Design 2022, 22 (7) , 4228-4235. https://doi.org/10.1021/acs.cgd.2c00241
    5. Yana Suchikova, Sergii Kovachov, Ihor Bohdanov, Anar A. Abdikadirova, Inesh Kenzhina, Anatoli I. Popov. Electrochemical Growth and Structural Study of the AlxGa1−xAs Nanowhisker Layer on the GaAs Surface. Journal of Manufacturing and Materials Processing 2023, 7 (5) , 153. https://doi.org/10.3390/jmmp7050153
    6. Katsuhiro Tomioka, Kazuharu Sugita, Junichi Motohisa. Enhanced Light Extraction of Nano‐Light‐Emitting Diodes with Metal‐Clad Structure Using Vertical GaAs/GaAsP Core–Multishell Nanowires on Si Platform. Advanced Photonics Research 2023, 4 (7) https://doi.org/10.1002/adpr.202200337
    7. Chenyang Li, Xutao Zhang, Ruixuan Yi, Ziyuan Li, Fanlu Zhang, Kaihui Liu, Xuetao Gan, Lan Fu, Fajun Xiao, Jianlin Zhao, Hark Hoe Tan, Chennupati Jagadish. Low‐Threshold Multiwavelength Plasmonic Nanolasing in an “H”‐Shape Cavity. Laser & Photonics Reviews 2023, https://doi.org/10.1002/lpor.202300187
    8. Ruixuan Yi, Xutao Zhang, Chen Li, Bijun Zhao, Jing Wang, Zhiwen Li, Xuetao Gan, Li Li, Ziyuan Li, Fanlu Zhang, Liang Fang, Naiyin Wang, Pingping Chen, Wei Lu, Lan Fu, Jianlin Zhao, Hark Hoe Tan, Chennupati Jagadish. Self-frequency-conversion nanowire lasers. Light: Science & Applications 2022, 11 (1) https://doi.org/10.1038/s41377-022-00807-7
    9. Ankit Udai, Swaroop Ganguly, Pallab Bhattacharya, Dipankar Saha. Real-time observation of delayed excited-state dynamics in InGaN/GaN quantum-wells by femtosecond transient absorption spectroscopy. Nanotechnology 2022, 33 (47) , 475202. https://doi.org/10.1088/1361-6528/ac8a50
    10. Maosheng Liu, Mingming Jiang, Xiangbo Zhou, Caixia Kan, Daning Shi. Performance-enhanced single-mode microlasers in an individual microwire covered by Ag nanowires. Optics & Laser Technology 2022, 155 , 108391. https://doi.org/10.1016/j.optlastec.2022.108391
    11. Jitao Li, Binghui Li, Ming Meng, Lingling Sun, Mingming Jiang. Interface engineering enhanced near-infrared electroluminescence in an n-ZnO microwire/p-GaAs heterojunction. Optics Express 2022, 30 (14) , 24773. https://doi.org/10.1364/OE.459837
    12. Zhen Guo, Dongxu Zhao, Lin Li, Caroline Andreazza‐Vignolle, Pascal Andreazza, Ligong Zhang, Wei Zhang, Lianqun Zhou. Enhanced Ultraviolet Spontaneous and Lasing Emission Through Interface Engineering of Patterned Vertically Aligned ZnO Nanowires. Advanced Materials Interfaces 2022, 9 (19) https://doi.org/10.1002/admi.202200024
    13. Fanlu Zhang, Xutao Zhang, Ziyuan Li, Ruixuan Yi, Zhe Li, Naiyin Wang, Xiaoxue Xu, Zahra Azimi, Li Li, Mykhaylo Lysevych, Xuetao Gan, Yuerui Lu, Hark Hoe Tan, Chennupati Jagadish, Lan Fu. A New Strategy for Selective Area Growth of Highly Uniform InGaAs/InP Multiple Quantum Well Nanowire Arrays for Optoelectronic Device Applications. Advanced Functional Materials 2022, 32 (3) https://doi.org/10.1002/adfm.202103057
    14. Mingming Jiang, Maosheng Liu, Xiangbo Zhou, Caixia Kan, Daning Shi. Performance-Enhanced Single-Mode Microlasers in an Individual Microwire Covered by Ag Nanowires. SSRN Electronic Journal 2022, 16 https://doi.org/10.2139/ssrn.4103686

    ACS Nano

    Cite this: ACS Nano 2021, 15, 5, 9126–9133
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsnano.1c02425
    Published May 10, 2021
    Copyright © 2021 American Chemical Society

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