Pair your accounts.

Export articles to Mendeley

Get article recommendations from ACS based on references in your Mendeley library.

Pair your accounts.

Export articles to Mendeley

Get article recommendations from ACS based on references in your Mendeley library.

You’ve supercharged your research process with ACS and Mendeley!

STEP 1:
Click to create an ACS ID

Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

Please note: If you switch to a different device, you may be asked to login again with only your ACS ID.

MENDELEY PAIRING EXPIRED
Your Mendeley pairing has expired. Please reconnect
ACS Publications. Most Trusted. Most Cited. Most Read
Stretchable Low-Impedance Conductor with Ag–Au–Pt Core–Shell–Shell Nanowires and in Situ Formed Pt Nanoparticles for Wearable and Implantable Device

OR SEARCH CITATIONS

My Activity
Publications
CONTENT TYPES

Figure 1Loading Img
Download Hi-Res ImageDownload to MS-PowerPointCite This:ACS Nano 2023, 17, 8, 7550-7561
    Article

    Stretchable Low-Impedance Conductor with Ag–Au–Pt Core–Shell–Shell Nanowires and in Situ Formed Pt Nanoparticles for Wearable and Implantable Device
    Click to copy article linkArticle link copied!

    • Sung-Hyuk Sunwoo
      Sung-Hyuk Sunwoo
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      Institute of Radiation Medicine, Seoul National University Medical Research Center, Seoul 03080, Republic of Korea
      More by Sung-Hyuk Sunwoo
      Orcidhttps://orcid.org/0000-0002-3925-1275
    • Sang Ihn Han
      Sang Ihn Han
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      Biomaterials Research Center, Biomedical Research Division, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea
      More by Sang Ihn Han
    • Dongjun Jung
      Dongjun Jung
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      More by Dongjun Jung
    • Minseong Kim
      Minseong Kim
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      More by Minseong Kim
    • Seonghyeon Nam
      Seonghyeon Nam
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      More by Seonghyeon Nam
    • Hyunjin Lee
      Hyunjin Lee
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      More by Hyunjin Lee
    • Suji Choi
      Suji Choi
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      Disease Biophysics Group, John A. Paulson School of Engineering and Applied Sciences, Harvard University, Boston, Massachusetts 02134, United States
      More by Suji Choi
    • Hyejeong Kang
      Hyejeong Kang
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      Division of Cardiology, Department of Internal Medicine, Seoul National University Hospital, Seoul 03080, Republic of Korea
      More by Hyejeong Kang
    • Ye Seul Cho
      Ye Seul Cho
      Division of Cardiology, Department of Internal Medicine, Seoul National University Hospital, Seoul 03080, Republic of Korea
      More by Ye Seul Cho
    • Da-Hae Yeom
      Da-Hae Yeom
      Division of Cardiology, Department of Internal Medicine, Seoul National University Hospital, Seoul 03080, Republic of Korea
      More by Da-Hae Yeom
    • Myung-Jin Cha
      Myung-Jin Cha
      Department of Cardiology, Department of Internal Medicine, Asan Medical Center, University of Ulsan College of Medicine, Seoul 05505, Republic of Korea
      More by Myung-Jin Cha
    • Seunghwan Lee
      Seunghwan Lee
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      More by Seunghwan Lee
    • Seung-Pyo Lee*
      Seung-Pyo Lee
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      Division of Cardiology, Department of Internal Medicine, Seoul National University Hospital, Seoul 03080, Republic of Korea
      Department of Internal Medicine, Seoul National University College of Medicine, Seoul 03080, Republic of Korea
      *E-mail: [email protected]
      More by Seung-Pyo Lee
    • Taeghwan Hyeon*
      Taeghwan Hyeon
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      *E-mail: [email protected]
      More by Taeghwan Hyeon
      Orcidhttps://orcid.org/0000-0001-5959-6257
    • Dae-Hyeong Kim*
      Dae-Hyeong Kim
      Center for Nanoparticle Research, Institute for Basic Science (IBS), Seoul 08826, Republic of Korea
      School of Chemical and Biological Engineering, and Institute of Chemical Processes, Seoul National University, Seoul 08826, Republic of Korea
      Department of Materials Science and Engineering, Seoul National University, Seoul 08826, Republic of Korea
      *E-mail: [email protected]
      More by Dae-Hyeong Kim
      Orcidhttps://orcid.org/0000-0002-4722-1893
    Other Access OptionsSupporting Information (1)

    ACS Nano

    Cite this: ACS Nano 2023, 17, 8, 7550–7561
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsnano.2c12659
    Published April 11, 2023
    Copyright © 2023 American Chemical Society
    Request reuse permissions

    Abstract

    Click to copy section linkSection link copied!
    Abstract Image

    Mechanically soft metallic nanocomposites have gained much attention as a key material for intrinsically stretchable biointegrated devices. However, it has been challenging to develop a stretchable conductive nanocomposite with all the desired material characteristics including high conductivity, high stretchability, low cytotoxicity, and low impedance. Here, we present a material strategy for the stretchable conductive nanocomposite, particularly emphasizing low impedance, by combining silver–gold–platinum core–shell–shell nanowires and homogeneously dispersed in situ synthesized platinum nanoparticles (Pt NPs). The highly embossed structure of the outermost Pt shell, together with the intrinsic electrical property of Pt, contributes to minimizing the impedance. The gold–platinum double-layer sheath prevents leaching of cytotoxic Ag ions, thus improving biocompatibility. Homogeneously dispersed Pt NPs, synthesized in situ during fabrication of the nanocomposite, simultaneously enhance conductivity, reduce impedance, and improve stretchability by supporting the percolation network formation. This intrinsically stretchable nanocomposite conductor can be applied to wearable and implantable bioelectronics for recording biosignals and delivering electrical stimulations in vivo.

    Copyright © 2023 American Chemical Society

    Subjects

    what are subjects

    Keywords

    what are keywords

    Read this article

    To access this article, please review the available access options below.

    Get instant access

    Purchase Access

    Read this article for 48 hours. Check out below using your ACS ID or as a guest.

    Recommended

    Access through Your Institution

    You may have access to this article through your institution.

    Your institution does not have access to this content. Add or change your institution or let them know you’d like them to include access.

    Supporting Information

    Click to copy section linkSection link copied!

    The Supporting Information is available free of charge at https://pubs.acs.org/doi/10.1021/acsnano.2c12659.

    • Figures S1–S11 of synthesis of the Ag–Au–Pt NW illustration and SEM, relative resistance variation, characterization of in situ formation of Pt NPs, TEM image of ex situ Pt NP nanocomposite, characterization of Ag–Au NW/Pt NP and Ag–Au–Pt NW/Pt NP nanocomposite, electrical and mechanical properties comparison, illustration of wearable device fabrication process, illustration describing wrist motion, illustration of implantable device fabrication process, in vivo implantation protocol, arrhythmic events recording. (PDF)

    Terms & Conditions

    Most electronic Supporting Information files are available without a subscription to ACS Web Editions. Such files may be downloaded by article for research use (if there is a public use license linked to the relevant article, that license may permit other uses). Permission may be obtained from ACS for other uses through requests via the RightsLink permission system: http://pubs.acs.org/page/copyright/permissions.html.

    Cited By

    Click to copy section linkSection link copied!

    This article is cited by 9 publications.

    1. Hye Jin Kim, Heewon Choi, Dae-Hyeong Kim, Donghee Son. Stretchable Functional Nanocomposites for Soft Implantable Bioelectronics. Nano Letters 2024, 24 (28) , 8453-8464. https://doi.org/10.1021/acs.nanolett.4c01163
    2. Sang Ihn Han, Sung-Hyuk Sunwoo, Chan Soon Park, Seung-Pyo Lee, Taeghwan Hyeon, Dae-Hyeong Kim. Next-Generation Cardiac Interfacing Technologies Using Nanomaterial-Based Soft Bioelectronics. ACS Nano 2024, 18 (19) , 12025-12048. https://doi.org/10.1021/acsnano.4c02171
    3. Sehui Chang, Ja Hoon Koo, Jisu Yoo, Min Seok Kim, Moon Kee Choi, Dae-Hyeong Kim, Young Min Song. Flexible and Stretchable Light-Emitting Diodes and Photodetectors for Human-Centric Optoelectronics. Chemical Reviews 2024, 124 (3) , 768-859. https://doi.org/10.1021/acs.chemrev.3c00548
    4. Shu Gong, Yan Lu, Jialiang Yin, Arie Levin, Wenlong Cheng. Materials-Driven Soft Wearable Bioelectronics for Connected Healthcare. Chemical Reviews 2024, 124 (2) , 455-553. https://doi.org/10.1021/acs.chemrev.3c00502
    5. Rongrong Zhao, Zengdian Zhao, Shasha Song, Yifan Wang. Multifunctional Conductive Double-Network Hydrogel Sensors for Multiscale Motion Detection and Temperature Monitoring. ACS Applied Materials & Interfaces 2023, 15 (51) , 59854-59865. https://doi.org/10.1021/acsami.3c15522
    6. Sangmin Song, Hyejun Hong, Kyung Yeun Kim, Kyun Kyu Kim, Jaewoo Kim, Daeyeon Won, Soyoung Yun, Joonhwa Choi, Young-In Ryu, Kyungwoo Lee, Jaeho Park, Joohyuk Kang, Junhyuk Bang, Hyunseon Seo, Yu-Chan Kim, Daeho Lee, Haechang Lee, Jinwoo Lee, Suk-Won Hwang, Seung Hwan Ko, Hojeong Jeon, Wonryung Lee. Photothermal Lithography for Realizing a Stretchable Multilayer Electronic Circuit Using a Laser. ACS Nano 2023, 17 (21) , 21443-21454. https://doi.org/10.1021/acsnano.3c06207
    7. Luying Yi, Bo Hou, Xiaogang Liu. Optical Integration in Wearable, Implantable and Swallowable Healthcare Devices. ACS Nano 2023, 17 (20) , 19491-19501. https://doi.org/10.1021/acsnano.3c04284
    8. Zongman Zhang, Zhongtai Zhu, Pengcheng Zhou, Yunfan Zou, Jiawei Yang, Hossam Haick, Yan Wang. Soft Bioelectronics for Therapeutics. ACS Nano 2023, 17 (18) , 17634-17667. https://doi.org/10.1021/acsnano.3c02513
    9. Kai Chen, Linyuan Zhang, Kai Wu, Chao Yang, Ruihong Wang, Canhua Xu, Jinyu Zhang, Gang Liu, Jun Sun. Highly Robust and Strain-Resilient Thin Film Conductors Featuring Brittle Materials. Nano Letters 2023, 23 (14) , 6619-6628. https://doi.org/10.1021/acs.nanolett.3c01781
    Download PDF
    Go to ACS Nano
    Get e-Alerts
    Get e-Alerts

    ACS Nano

    Cite this: ACS Nano 2023, 17, 8, 7550–7561
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsnano.2c12659
    Published April 11, 2023
    Copyright © 2023 American Chemical Society
    Request reuse permissions

    Article Views

    3410

    Altmetric

    -

    Citations

    9
    Learn about these metrics

    Article Views are the COUNTER-compliant sum of full text article downloads since November 2008 (both PDF and HTML) across all institutions and individuals. These metrics are regularly updated to reflect usage leading up to the last few days.

    Citations are the number of other articles citing this article, calculated by Crossref and updated daily. Find more information about Crossref citation counts.

    The Altmetric Attention Score is a quantitative measure of the attention that a research article has received online. Clicking on the donut icon will load a page at altmetric.com with additional details about the score and the social media presence for the given article. Find more information on the Altmetric Attention Score and how the score is calculated.