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Growth of Quasi-Free-Standing Single-Layer Blue Phosphorus on Tellurium Monolayer Functionalized Au(111)

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    Growth of Quasi-Free-Standing Single-Layer Blue Phosphorus on Tellurium Monolayer Functionalized Au(111)
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    † Department of Chemistry, National University of Singapore, 3 Science Drive 3, 117543 Singapore
    ‡ Hefei National Laboratory for Physical Sciences at the Microscale, CAS Centre for Excellence and Synergetic Innovation Center of Quantum Information & Quantum Physics, University of Science and Technology of China, Hefei 230026, China
    § Department of Physics, National University of Singapore, 2 Science Drive 3, 117542 Singapore
    ∥ SZU-NUS Collaborative Innovation Center for Optoelectronic Science and Technology, Shenzhen University, Shenzhen 518060, China
    ⊥ Institute for Advanced Study and Department of Physics, Nanchang University, 999 Xue Fu Da Dao, Nanchang 330031, China
    # Key Laboratory of Flexible Electronics (KLOFE) & Institute of Advanced Materials (IAM), Jiangsu National Synergetic Innovation Center for Advanced Materials (SICAM), Nanjing Tech University (Nanjing Tech), 30 South Puzhu Road, Nanjing 211816, China
    Institute of Advanced Materials (IAM), Nanjing University of Posts and Telecommunications (NJUPT), 9 Wenyuan Road, Yadong Xincheng Distribution, Nanjing 210023, China
    △ National University of Singapore (Suzhou) Research Institute, 377 Lin Quan Street, Suzhou Industrial Park, Suzhou 215123, China
    ▲ Center for Advanced 2D Materials and Graphene Research Center, National University of Singapore, 3 Science Drive 3, 117546 Singapore
    *E-mail: [email protected]
    *E-mail: [email protected]
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    Cite this: ACS Nano 2017, 11, 5, 4943–4949
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    https://doi.org/10.1021/acsnano.7b01575
    Published May 1, 2017
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    Abstract

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    Blue phosphorus, a newly proposed allotrope of phosphorus, represents a promising 2D material with predicted large tunable band gap and high charge-carrier mobility. Here, we report a simple method for the growth of quasi-free-standing single layer blue phosphorus on tellurium functionalized Au(111) by using black phosphorus as the precursor. In situ low-temperature scanning tunneling microscopy (LT-STM) measurements were used to monitor the growth of the single-layer blue phosphorus, which forms triangular structures arranged hexagonally on the tellurium layer. As revealed by in situ X-ray photoelectron spectroscopy, LT-STM measurements, and density functional theory calculation, the blue phosphorus layer weakly interacts with the underlying tellurium layer.

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