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Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces

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    Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces
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    † Center for Integrated Nanotechnologies, Sandia National Laboratories, Albuquerque, New Mexico 87185, United States
    ‡ Sandia National Laboratories, Albuquerque, New Mexico 87185, United States
    § Center for Integrated Nanotechnologies, Materials Physics and Applications Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, United States
    *E-mail: [email protected]
    *E-mail: [email protected]
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    ACS Nano

    Cite this: ACS Nano 2017, 11, 6, 6431–6439
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    https://doi.org/10.1021/acsnano.7b02951
    Published May 23, 2017
    Copyright © 2017 American Chemical Society
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    Abstract

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    All-dielectric metasurfaces made from arrays of high index nanoresonators supporting strong magnetic dipole modes have emerged as a low-loss alternative to plasmonic metasurfaces. Here we use oxygen-doped single-walled carbon nanotubes (SWCNTs) as quantum emitters and couple them to silicon metasurfaces to study effects of the magnetic dipole modes of the constituent nanoresonators on the photoluminescence (PL) of individual SWCNTs. We find that when in resonance, the magnetic mode of the silicon nanoresonators can lead to a moderate average PL enhancement of 0.8–4.0 of the SWCNTs, accompanied by an average increase in the radiative decay rate by a factor of 1.5–3.0. More interestingly, single dopant polarization experiments show an anomalous photoluminescence polarization rotation by coupling individual SWCNTs to silicon nanoresonators. Numerical simulations indicate that this is caused by modification of near-field polarization distribution at certain areas in the proximity of the silicon nanoresonators at the excitation wavelength, thus presenting an approach to control emission polarization. These findings indicate silicon nanoresonators as potential building blocks of quantum photonic circuits capable of manipulating PL intensity and polarization of single photon sources.

    Copyright © 2017 American Chemical Society

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    Supporting Information

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    The Supporting Information is available free of charge on the ACS Publications website at DOI: 10.1021/acsnano.7b02951.

    • PL image of oxygen-doped SWCNTs, simulation of radiative decay rate enhancement factors, estimation of η and Purcell factor, simulations of directional scattering of silicon nanoresonators and changes in the collection efficiency, polarization of laser beam on silicon metasurfaces, far field emission polarization simulations, resonance modes in Si360 (PDF)

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    ACS Nano

    Cite this: ACS Nano 2017, 11, 6, 6431–6439
    Click to copy citationCitation copied!
    https://doi.org/10.1021/acsnano.7b02951
    Published May 23, 2017
    Copyright © 2017 American Chemical Society
    Request reuse permissions

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